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Copper-catalyzed asymmetric tandem double Michael reactions of diethylzinc to alpha,beta-unsaturated ketones followed by trapping with nitroolefins

文献类型：期刊论文

作者Wang, Qiang1; Li, Shuang1; Hou, Chuan-Jin1; Chu, Ting-Ting1; Hu, Xiang-Ping2
刊名TETRAHEDRON
出版日期2019-07-19
卷号75期号:29页码:3943-3950
ISSN号0040-4020
关键词Chiral P,N-ligands Asymmetric tandem reactions Double Michael reactions Enolate trapping Nitroolefins
DOI10.1016/j.tet.2019.06.032
通讯作者Hou, Chuan-Jin(houcj@dlpu.edu.cn) ; Hu, Xiang-Ping(xiangping@dicp.ac.cn)
英文摘要A copper catalyzed asymmetric tandem double Michael addition of diethylzinc to alpha,beta-unsaturated ketones followed by trapping with nitroolefins has been developed using chiral P,N-ligands. The tandem products were obtained in good yields and excellent enantioselectivities with three contiguous stereocenters. (C) 2019 Elsevier Ltd. All rights reserved.
WOS关键词ENANTIOSELECTIVE CONJUGATE ADDITION ; ORGANOMETALLIC REAGENTS ; EFFICIENT ; ZINC ; 1,4-ADDITION ; LIGANDS ; DIALKYLZINCS ; CARBONYL ; ENONES ; ACCESS
资助项目National Natural Science Foundation of China[21403022] ; National Natural Science Foundation of China[21572226] ; National Natural Science Foundation of China[21772196] ; Program of Star of Dalian Youth Science and Technology[2016RQ062] ; Fundamental Research Funds for the Higher Education of Liaoning Province[2017J027] ; Liaoning BaiQianWan Talents Program[201892153]
WOS研究方向Chemistry
语种英语
出版者PERGAMON-ELSEVIER SCIENCE LTD
WOS记录号WOS:000474678000011
资助机构National Natural Science Foundation of China ; National Natural Science Foundation of China ; Program of Star of Dalian Youth Science and Technology ; Program of Star of Dalian Youth Science and Technology ; Fundamental Research Funds for the Higher Education of Liaoning Province ; Fundamental Research Funds for the Higher Education of Liaoning Province ; Liaoning BaiQianWan Talents Program ; Liaoning BaiQianWan Talents Program ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Program of Star of Dalian Youth Science and Technology ; Program of Star of Dalian Youth Science and Technology ; Fundamental Research Funds for the Higher Education of Liaoning Province ; Fundamental Research Funds for the Higher Education of Liaoning Province ; Liaoning BaiQianWan Talents Program ; Liaoning BaiQianWan Talents Program ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Program of Star of Dalian Youth Science and Technology ; Program of Star of Dalian Youth Science and Technology ; Fundamental Research Funds for the Higher Education of Liaoning Province ; Fundamental Research Funds for the Higher Education of Liaoning Province ; Liaoning BaiQianWan Talents Program ; Liaoning BaiQianWan Talents Program ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Program of Star of Dalian Youth Science and Technology ; Program of Star of Dalian Youth Science and Technology ; Fundamental Research Funds for the Higher Education of Liaoning Province ; Fundamental Research Funds for the Higher Education of Liaoning Province ; Liaoning BaiQianWan Talents Program ; Liaoning BaiQianWan Talents Program
源URL[http://cas-ir.dicp.ac.cn/handle/321008/175098]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Hou, Chuan-Jin; Hu, Xiang-Ping
作者单位1.Dalian Polytech Univ, Sch Light Ind & Chem Engn, Dalian 116034, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714		 Wang, Qiang,Li, Shuang,Hou, Chuan-Jin,et al. Copper-catalyzed asymmetric tandem double Michael reactions of diethylzinc to alpha,beta-unsaturated ketones followed by trapping with nitroolefins[J]. TETRAHEDRON,2019,75(29):3943-3950.
APA Wang, Qiang,Li, Shuang,Hou, Chuan-Jin,Chu, Ting-Ting,&Hu, Xiang-Ping.(2019).Copper-catalyzed asymmetric tandem double Michael reactions of diethylzinc to alpha,beta-unsaturated ketones followed by trapping with nitroolefins.TETRAHEDRON,75(29),3943-3950.
MLA Wang, Qiang,et al."Copper-catalyzed asymmetric tandem double Michael reactions of diethylzinc to alpha,beta-unsaturated ketones followed by trapping with nitroolefins".TETRAHEDRON 75.29(2019):3943-3950.

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来源：大连化学物理研究所

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