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Facile synthesis of chiral epsilon-sultams via an organocatalytic aza-Friedel-Crafts reaction

文献类型：期刊论文

作者Zhao, Zi-Biao1,2; Shi, Lei2; Li, Yaming2; Meng, Fan-Jie2; Zhou, Yong-Gui1,2
刊名ORGANIC & BIOMOLECULAR CHEMISTRY
出版日期2019-07-14
卷号17期号:26页码:6364-6368
ISSN号1477-0520
DOI10.1039/c9ob01158g
通讯作者Shi, Lei(shileichem@dlut.edu.cn) ; Zhou, Yong-Gui(ygzhou@dicp.ac.cn)
英文摘要Chiral epsilon-sultams, with their unique strain cyclic structure, are a type of molecule with important biological activities. A facile enantioselective aza-Friedel-Crafts reaction of seven-membered cyclic N-sulfonylimines with naphthols was developed with a cinchona alkaloid-based bifunctional organocatalyst, giving chiral epsilon-sultams with an enantiomeric excess of up to 92%.
WOS关键词INDOLES ; ALKYLATION ; IMINES ; SULFONAMIDES ; DERIVATIVES ; MODULATORS ; NAPHTHOLS ; REAGENTS ; PBTDS
资助项目National Natural Science Foundation of China[21772195] ; Dalian Bureau of Science and Technology[2016RD07] ; Chinese Academy of Sciences[XDB17020300] ; Chinese Academy of Sciences[QYZDJ-SSW-SLH035]
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000474089200008
出版者ROYAL SOC CHEMISTRY
资助机构National Natural Science Foundation of China ; National Natural Science Foundation of China ; Dalian Bureau of Science and Technology ; Dalian Bureau of Science and Technology ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Dalian Bureau of Science and Technology ; Dalian Bureau of Science and Technology ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Dalian Bureau of Science and Technology ; Dalian Bureau of Science and Technology ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Dalian Bureau of Science and Technology ; Dalian Bureau of Science and Technology ; Chinese Academy of Sciences ; Chinese Academy of Sciences
源URL[http://cas-ir.dicp.ac.cn/handle/321008/175130]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Shi, Lei; Zhou, Yong-Gui
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Dalian Univ Technol, Zhang Dayu Sch Chem, State Key Lab Fine Chem, 2 Linggong Rd, Dalian 116024, Peoples R China
推荐引用方式
GB/T 7714		 Zhao, Zi-Biao,Shi, Lei,Li, Yaming,et al. Facile synthesis of chiral epsilon-sultams via an organocatalytic aza-Friedel-Crafts reaction[J]. ORGANIC & BIOMOLECULAR CHEMISTRY,2019,17(26):6364-6368.
APA Zhao, Zi-Biao,Shi, Lei,Li, Yaming,Meng, Fan-Jie,&Zhou, Yong-Gui.(2019).Facile synthesis of chiral epsilon-sultams via an organocatalytic aza-Friedel-Crafts reaction.ORGANIC & BIOMOLECULAR CHEMISTRY,17(26),6364-6368.
MLA Zhao, Zi-Biao,et al."Facile synthesis of chiral epsilon-sultams via an organocatalytic aza-Friedel-Crafts reaction".ORGANIC & BIOMOLECULAR CHEMISTRY 17.26(2019):6364-6368.

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来源：大连化学物理研究所

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