High-Temperature CO2 Electrolysis in Solid Oxide Electrolysis Cells: Developments, Challenges, and Prospects
文献类型：期刊论文
| 作者 | Song, Yuefeng2,3; Zhang, Xiaomin2; Xie, Kui1; Wang, Guoxiong2; Bao, Xinhe2 |
| 刊名 | ADVANCED MATERIALS
 |
| 出版日期 | 2019-07-07 |
| 页码 | 18 |
| ISSN号 | 0935-9648 |
| 关键词 | CO2 electrolysis perovskites solid oxide electrolysis cells |
| DOI | 10.1002/adma.201902033 |
| 通讯作者 | Wang, Guoxiong(wanggx@dicp.ac.cn) ; Bao, Xinhe(xhbao@dicp.ac.cn) |
| 英文摘要 | High-temperature CO2 electrolysis in solid-oxide electrolysis cells (SOECs) could greatly assist in the reduction of CO2 emissions by electrochemically converting CO2 to valuable fuels through effective electrothermal activation of the stable C(sic)O bond. If powered by renewable energy resources, it could also provide an advanced energy-storage method for their intermittent output. Compared to low-temperature electrochemical CO2 reduction, CO2 electrolysis in SOECs at high temperature exhibits higher current density and energy efficiency and has thus attracted much recent attention. The history of its development and its fundamental mechanisms, cathode materials, oxygen-ion-conducting electrolyte materials, and anode materials are highlighted. Electrode, electrolyte, and electrode-electrolyte interface degradation issues are comprehensively summarized. Fuel-assisted SOECs with low-cost fuels applied to the anode to decrease the overpotential and electricity consumption are introduced. Furthermore, the challenges and prospects for future research into high-temperature CO2 electrolysis in SOECs are included. |
| WOS关键词 | OXYGEN ELECTRODES ; CARBON-DIOXIDE ; FUEL-CELL ; ELECTROCHEMICAL PERFORMANCE ; INTERMEDIATE-TEMPERATURE ; STEAM ELECTROLYSIS ; ELECTROCATALYTIC REDUCTION ; ELIMINATING DEGRADATION ; RUDDLESDEN-POPPER ; SYNGAS PRODUCTION |
| 资助项目 | National Key R&D Program of China[2017YFA0700102] ; National Natural Science Foundation of China[21573222] ; National Natural Science Foundation of China[91545202] ; National Natural Science Foundation of China[21703237] ; Dalian National Laboratory for Clean Energy[DNL180404] ; Dalian Institute of Chemical Physics[DICP DMTO201702] ; Dalian Outstanding Young Scientist Foundation[2017RJ03] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDB17020200] ; CAS Youth Innovation Promotion[2015145] |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| 语种 | 英语 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| WOS记录号 | WOS:000474479400001 |
| 资助机构 | National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy ; Dalian Institute of Chemical Physics ; Dalian Institute of Chemical Physics ; Dalian Outstanding Young Scientist Foundation ; Dalian Outstanding Young Scientist Foundation ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; CAS Youth Innovation Promotion ; CAS Youth Innovation Promotion ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy ; Dalian Institute of Chemical Physics ; Dalian Institute of Chemical Physics ; Dalian Outstanding Young Scientist Foundation ; Dalian Outstanding Young Scientist Foundation ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; CAS Youth Innovation Promotion ; CAS Youth Innovation Promotion ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy ; Dalian Institute of Chemical Physics ; Dalian Institute of Chemical Physics ; Dalian Outstanding Young Scientist Foundation ; Dalian Outstanding Young Scientist Foundation ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; CAS Youth Innovation Promotion ; CAS Youth Innovation Promotion ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy ; Dalian Institute of Chemical Physics ; Dalian Institute of Chemical Physics ; Dalian Outstanding Young Scientist Foundation ; Dalian Outstanding Young Scientist Foundation ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; CAS Youth Innovation Promotion ; CAS Youth Innovation Promotion |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/175347]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Wang, Guoxiong; Bao, Xinhe |
| 作者单位 | 1.Chinese Acad Sci, Fujian Inst Res Struct Matter, Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, State Key Lab Catalysis,CAS Ctr Excellence Nanosc, Dalian 116023, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100039, Peoples R China |
| 推荐引用方式 GB/T 7714 | Song, Yuefeng,Zhang, Xiaomin,Xie, Kui,et al. High-Temperature CO2 Electrolysis in Solid Oxide Electrolysis Cells: Developments, Challenges, and Prospects[J]. ADVANCED MATERIALS,2019:18. |
| APA | Song, Yuefeng,Zhang, Xiaomin,Xie, Kui,Wang, Guoxiong,&Bao, Xinhe.(2019).High-Temperature CO2 Electrolysis in Solid Oxide Electrolysis Cells: Developments, Challenges, and Prospects.ADVANCED MATERIALS,18. |
| MLA | Song, Yuefeng,et al."High-Temperature CO2 Electrolysis in Solid Oxide Electrolysis Cells: Developments, Challenges, and Prospects".ADVANCED MATERIALS (2019):18. |
入库方式： OAI收割
来源：大连化学物理研究所
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