中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Efficient Perovskite Light-Emitting Diodes via Tuning Nanoplatelet Distribution and Crystallinity Orientation

文献类型:期刊论文

作者Zou, YT; Huang, Q; Yang, YG; Ban, MY; Li, SY; Han, YJ; Wu, T; Tan, YS; Gao, XY; Song, T
刊名ADVANCED MATERIALS INTERFACES
出版日期2018
卷号5期号:20页码:-
关键词CSPBX3 NANOCRYSTALS I NANOCRYSTALS CS4PBX6 X HALIDE TRANSFORMATION BR SEMICONDUCTORS CONFINEMENT CL
ISSN号2196-7350
DOI10.1002/admi.201801030
文献子类期刊论文
英文摘要Quasi-2D Ruddlesden-Popper (RP) perovskites with quantum-size-tuned nanoplatelet crystallites are particularly attractive for light-emitting diode (LED) applications because of their excellent charge transport, bandgap tunability, and narrow emission peaks. Favorable energy cascade structure in 2D RP perovskites can funnel the photoexcitation from large-bandgap nanoplatelets to the lowest bandgap ones, which promises efficient radiative recombination. However, how to rationally control the nanoplatelet distribution as well as the crystallization characteristics to ensure efficient energy transfer and charge transport in perovskite films is still challenging. Here, a simple path to facilely tune the nanoplatelet distribution as well as the crystal orientation via carefully controlling postannealing condition is provided. With optimizing the thermal annealing time, compact and flat perovskite films with high photoluminescence quantum yield are obtained. Based on the optimized perovskite films, green LED with a current efficiency of 43.7 cd A(-1), corresponding to an external quantum efficiency of 13.9%, is achieved. This work provides a simple path to target highly efficient perovskite LED devices.
语种英语
源URL[http://ir.sinap.ac.cn/handle/331007/30923]  
专题上海应用物理研究所_中科院上海应用物理研究所2011-2017年
作者单位1.Soochow Univ, Jiangsu Key Lab Carbon Based Funct Mat & Devices, Inst Funct Nano & Soft Mat FUNSOM, 199 Renai Rd, Suzhou 215123, Peoples R China
2.Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai Synchrotron Radiat Facil, 239 Zhangheng Rd, Shanghai 201204, Peoples R China
3.Soochow Univ, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, 199 Renai Rd, Suzhou 215123, Peoples R China
推荐引用方式
GB/T 7714
Zou, YT,Huang, Q,Yang, YG,et al. Efficient Perovskite Light-Emitting Diodes via Tuning Nanoplatelet Distribution and Crystallinity Orientation[J]. ADVANCED MATERIALS INTERFACES,2018,5(20):-.
APA Zou, YT.,Huang, Q.,Yang, YG.,Ban, MY.,Li, SY.,...&Sun, BQ.(2018).Efficient Perovskite Light-Emitting Diodes via Tuning Nanoplatelet Distribution and Crystallinity Orientation.ADVANCED MATERIALS INTERFACES,5(20),-.
MLA Zou, YT,et al."Efficient Perovskite Light-Emitting Diodes via Tuning Nanoplatelet Distribution and Crystallinity Orientation".ADVANCED MATERIALS INTERFACES 5.20(2018):-.

入库方式: OAI收割

来源:上海应用物理研究所

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