A review of oxygen reduction mechanisms for metal-free carbon-based electrocatalysts
文献类型：期刊论文
| 作者 | Ma, Ruguang; Lin, Gaoxin; Zhou, Yao; Liu, Qian; Zhang, Tao; Shan, Guangcun; Yang, Minghui; Wang, Jiacheng |
| 刊名 | NPJ COMPUTATIONAL MATERIALS
 |
| 出版日期 | 2019-07-19 |
| 卷号 | 5 |
| ISSN号 | 2057-3960 |
| DOI | 10.1038/s41524-019-0210-3 |
| 文献子类 | Review |
| 英文摘要 | The sluggish kinetics of Oxygen Reduction Reaction (ORR) at the cathode in proton exchange membrane fuel cells or metal-air batteries requires highly effective and stable electrocatalysts to boost the reaction. The low abundance and high price of Pt-based electrocatalysts hamper the widespread application of proton exchange membrane fuel cells and metal-air batteries. As promising alternatives, metal-free carbon materials, especially upon doping heteroatoms or creating defects demonstrated excellent ORR activity, which is as efficient as or even superior to commercial platinum on carbon. Significant progress on the development of advanced carbon materials as highly stable and durable catalysts has been achieved, but the catalytic mechanisms of these materials still remain undistinguished. In present review, we summarized the up-to-date progress in the studies of carbon materials, and emphasized on the combination of experiment and theory to clarify the underlying mechanisms of these materials. At last, we proposed the perspectives on the proper strategies of elucidating the mechanisms of carbon materials as electrocatalysts towards ORR. |
| WOS研究方向 | Chemistry ; Materials Science |
| 语种 | 英语 |
| 出版者 | SPRINGERNATURE |
| 源URL | [http://ir.sic.ac.cn/handle/331005/26972]  |
| 专题 | 中国科学院上海硅酸盐研究所 |
| 推荐引用方式 GB/T 7714 | Ma, Ruguang,Lin, Gaoxin,Zhou, Yao,et al. A review of oxygen reduction mechanisms for metal-free carbon-based electrocatalysts[J]. NPJ COMPUTATIONAL MATERIALS,2019,5. |
| APA | Ma, Ruguang.,Lin, Gaoxin.,Zhou, Yao.,Liu, Qian.,Zhang, Tao.,...&Wang, Jiacheng.(2019).A review of oxygen reduction mechanisms for metal-free carbon-based electrocatalysts.NPJ COMPUTATIONAL MATERIALS,5. |
| MLA | Ma, Ruguang,et al."A review of oxygen reduction mechanisms for metal-free carbon-based electrocatalysts".NPJ COMPUTATIONAL MATERIALS 5(2019). |
入库方式： OAI收割
来源：上海硅酸盐研究所
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