中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Poly(ionic liquid)s as a distinct receptor material to create a highly-integrated sensing platform for efficiently identifying numerous saccharides

文献类型:期刊论文

作者Zhang, Wanlin1,2; Li, Yao3; Liang, Yun2; Gao, Ning2; Liu, Chengcheng2; Wang, Shiqiang2; Yin, Xianpeng1; Li, Guangtao2
刊名CHEMICAL SCIENCE
出版日期2019-07-21
卷号10期号:27页码:6617-6623
ISSN号2041-6520
DOI10.1039/c9sc02266j
英文摘要Saccharides have strong hydrophilicities, and are complex molecular structures with subtle structure differences, and tremendous structural variations. The creation of one sensing platform capable of efficiently identifying such target systems presents a huge challenge. Using the integration of unique multiple noncovalent interactions simultaneously occurring in poly(ionic liquid)s (PILs) with multiple signaling channels, in this research an aggregation-induced emission (AIE)-doped photonic structured PIL sphere is constructed. It is found that such a sphere can serve as a highly integrated platform to provide abundant fingerprints for directly sensing numerous saccharides with an unprecedented efficiency. As a demonstration, 23 saccharides can be conveniently identified using only one sphere. More importantly, by using simple ion-exchanges of PIL receptors or/and increasing the AIE signaling channels, this platform is able to perform, on demand, different sensing tasks very efficiently. This is demonstrated by using it for the detection of difficult targets, such as greatly extended saccharides as well as mixed targets, in real-life examples on one or two spheres. The findings show that this new class of platform is very promising for addressing the challenges of identifying saccharides.
WOS关键词FLUORESCENT SENSOR ARRAY ; IONIC LIQUIDS ; DISCRIMINATION ; GLUCOSE ; IDENTIFICATION ; BINDING ; MONOSACCHARIDES ; DISSOLUTION ; AGGREGATION ; RECOGNITION
资助项目NSF China[21773135] ; NSF China[21473098] ; NSF China[21121004] ; NSF China[21421064] ; MOST[2017YFA0204501] ; MOST[2013CB834502] ; Deutsche Forschungsgemeinschaft DFG[TRR61]
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000477947800001
出版者ROYAL SOC CHEMISTRY
资助机构NSF China ; MOST ; Deutsche Forschungsgemeinschaft DFG
源URL[http://ir.ipe.ac.cn/handle/122111/30439]  
专题中国科学院过程工程研究所
通讯作者Li, Guangtao
作者单位1.Aerosp Res Inst Special Mat & Proc Technol, Beijing 100074, Peoples R China
2.Tsinghua Univ, Dept Chem, Key Lab Organ Optoelect & Mol Engn, Beijing 100084, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Wanlin,Li, Yao,Liang, Yun,et al. Poly(ionic liquid)s as a distinct receptor material to create a highly-integrated sensing platform for efficiently identifying numerous saccharides[J]. CHEMICAL SCIENCE,2019,10(27):6617-6623.
APA Zhang, Wanlin.,Li, Yao.,Liang, Yun.,Gao, Ning.,Liu, Chengcheng.,...&Li, Guangtao.(2019).Poly(ionic liquid)s as a distinct receptor material to create a highly-integrated sensing platform for efficiently identifying numerous saccharides.CHEMICAL SCIENCE,10(27),6617-6623.
MLA Zhang, Wanlin,et al."Poly(ionic liquid)s as a distinct receptor material to create a highly-integrated sensing platform for efficiently identifying numerous saccharides".CHEMICAL SCIENCE 10.27(2019):6617-6623.

入库方式: OAI收割

来源:过程工程研究所

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