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Chinese Academy of Sciences Institutional Repositories Grid
Silicone Elastomers with High-Permittivity Ionic Liquids Loading

文献类型:期刊论文

作者Liu, Xue1,3; Yu, Liyun1; Nie, Yi2,3; Skov, Anne Ladegaard1
刊名ADVANCED ENGINEERING MATERIALS
出版日期2019-08-20
页码9
关键词dielectric elastomers ionic liquids permittivity temperature-dependent
ISSN号1438-1656
DOI10.1002/adem.201900481
英文摘要The most obvious challenge facing current dielectric elastomers (DEs) is the high driving voltages necessary to activate them, and so, an effective way to overcome this shortcoming is to increase their dielectric permittivity. Herein, high-permittivity dielectric elastomer materials are prepared by synthesizing silicone elastomer loaded with ionic liquids (ILs). The influence of the structure and the amounts of ILs on the material properties is discussed, and important properties for material applications as DEs, such as dielectric permittivity, gel fraction, and mechanical properties, are also investigated. It is found that 1-butyl-3-methylimidazolium hexafluoroantimonate (BmimSbF(6)) is the most suitable IL for the given system. The dielectric permittivity of the material with 90 parts per hundred rubber (phr) BmimSbF(6) is 3.2 times higher than that of the pristine silicone elastomer, whereas the dielectric permittivity of pure silicone elastomer and elastomer loaded with ILs decreases in line with increased temperature in all cases. Young's modulus decreases in line with the increasing amount of BmimSbF(6) in the elastomer, as expected. A simpler figure of merit (F*(om)) for actuators is used, and F*(om) of the elastomer with a 90 phr IL loading is 10.40, thereby indicating that the material has a great advantage when used in actuators.
WOS关键词DIELECTRIC ELASTOMERS ; HIGH-PERFORMANCE ; IONOGELS ; ACTUATOR ; STRAIN
资助项目Department of Chemical and Biochemical Engineering, Technical University of Denmark ; National Natural Science Foundation of China[21576262] ; National Natural Science Foundation of China[21776276]
WOS研究方向Materials Science
语种英语
WOS记录号WOS:000482308800001
出版者WILEY-V C H VERLAG GMBH
资助机构Department of Chemical and Biochemical Engineering, Technical University of Denmark ; National Natural Science Foundation of China
源URL[http://ir.ipe.ac.cn/handle/122111/30631]  
专题中国科学院过程工程研究所
通讯作者Nie, Yi; Skov, Anne Ladegaard
作者单位1.Tech Univ Denmark, Dept Chem & Biochem Engn, Danish Polymer Ctr, Soltofts Plads 227, DK-2800 Lyngby, Denmark
2.Zhengzhou Inst Emerging Ind Technol, Zhengzhou 450000, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing Key Lab Ion Liquids Clean Proc,Key Lab Gr, POB 353, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Liu, Xue,Yu, Liyun,Nie, Yi,et al. Silicone Elastomers with High-Permittivity Ionic Liquids Loading[J]. ADVANCED ENGINEERING MATERIALS,2019:9.
APA Liu, Xue,Yu, Liyun,Nie, Yi,&Skov, Anne Ladegaard.(2019).Silicone Elastomers with High-Permittivity Ionic Liquids Loading.ADVANCED ENGINEERING MATERIALS,9.
MLA Liu, Xue,et al."Silicone Elastomers with High-Permittivity Ionic Liquids Loading".ADVANCED ENGINEERING MATERIALS (2019):9.

入库方式: OAI收割

来源:过程工程研究所

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