Silicone Elastomers with High-Permittivity Ionic Liquids Loading
文献类型:期刊论文
作者 | Liu, Xue1,3; Yu, Liyun1; Nie, Yi2,3; Skov, Anne Ladegaard1 |
刊名 | ADVANCED ENGINEERING MATERIALS
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出版日期 | 2019-08-20 |
页码 | 9 |
关键词 | dielectric elastomers ionic liquids permittivity temperature-dependent |
ISSN号 | 1438-1656 |
DOI | 10.1002/adem.201900481 |
英文摘要 | The most obvious challenge facing current dielectric elastomers (DEs) is the high driving voltages necessary to activate them, and so, an effective way to overcome this shortcoming is to increase their dielectric permittivity. Herein, high-permittivity dielectric elastomer materials are prepared by synthesizing silicone elastomer loaded with ionic liquids (ILs). The influence of the structure and the amounts of ILs on the material properties is discussed, and important properties for material applications as DEs, such as dielectric permittivity, gel fraction, and mechanical properties, are also investigated. It is found that 1-butyl-3-methylimidazolium hexafluoroantimonate (BmimSbF(6)) is the most suitable IL for the given system. The dielectric permittivity of the material with 90 parts per hundred rubber (phr) BmimSbF(6) is 3.2 times higher than that of the pristine silicone elastomer, whereas the dielectric permittivity of pure silicone elastomer and elastomer loaded with ILs decreases in line with increased temperature in all cases. Young's modulus decreases in line with the increasing amount of BmimSbF(6) in the elastomer, as expected. A simpler figure of merit (F*(om)) for actuators is used, and F*(om) of the elastomer with a 90 phr IL loading is 10.40, thereby indicating that the material has a great advantage when used in actuators. |
WOS关键词 | DIELECTRIC ELASTOMERS ; HIGH-PERFORMANCE ; IONOGELS ; ACTUATOR ; STRAIN |
资助项目 | Department of Chemical and Biochemical Engineering, Technical University of Denmark ; National Natural Science Foundation of China[21576262] ; National Natural Science Foundation of China[21776276] |
WOS研究方向 | Materials Science |
语种 | 英语 |
WOS记录号 | WOS:000482308800001 |
出版者 | WILEY-V C H VERLAG GMBH |
资助机构 | Department of Chemical and Biochemical Engineering, Technical University of Denmark ; National Natural Science Foundation of China |
源URL | [http://ir.ipe.ac.cn/handle/122111/30631] ![]() |
专题 | 中国科学院过程工程研究所 |
通讯作者 | Nie, Yi; Skov, Anne Ladegaard |
作者单位 | 1.Tech Univ Denmark, Dept Chem & Biochem Engn, Danish Polymer Ctr, Soltofts Plads 227, DK-2800 Lyngby, Denmark 2.Zhengzhou Inst Emerging Ind Technol, Zhengzhou 450000, Peoples R China 3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing Key Lab Ion Liquids Clean Proc,Key Lab Gr, POB 353, Beijing 100190, Peoples R China |
推荐引用方式 GB/T 7714 | Liu, Xue,Yu, Liyun,Nie, Yi,et al. Silicone Elastomers with High-Permittivity Ionic Liquids Loading[J]. ADVANCED ENGINEERING MATERIALS,2019:9. |
APA | Liu, Xue,Yu, Liyun,Nie, Yi,&Skov, Anne Ladegaard.(2019).Silicone Elastomers with High-Permittivity Ionic Liquids Loading.ADVANCED ENGINEERING MATERIALS,9. |
MLA | Liu, Xue,et al."Silicone Elastomers with High-Permittivity Ionic Liquids Loading".ADVANCED ENGINEERING MATERIALS (2019):9. |
入库方式: OAI收割
来源:过程工程研究所
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