Few-layered mesoporous graphene for high-performance toluene adsorption and regeneration
文献类型：期刊论文
| 作者 | Wang, Yaling2; Li, Zehui2; Tang, Cheng3; Ren, Haixia2; Zhang, Qiang2; Xue, Mo2; Xiong, Jin1; Wang, Dongbin2; Yu, Qian2; He, Zhiyuan4 |
| 刊名 | ENVIRONMENTAL SCIENCE-NANO
 |
| 出版日期 | 2019-10-01 |
| 卷号 | 6期号:10页码:3113-3122 |
| ISSN号 | 2051-8153 |
| DOI | 10.1039/c9en00608g |
| 英文摘要 | The benzene series is one type of volatile organic compounds (VOCs) which causes significant health and environmental issues. Adsorption is an energy-efficient technique for VOC treatment. With a combination of strong pi-pi interaction with the benzene series, large specific surface area (SSA), tunable nanostructure hierarchy and favourable hydrophobicity, three-dimensional porous graphene materials are potentially favorable for high adsorption capacity, low-energy regeneration and good resistance to high humidity. In this work, few-layered mesoporous graphene (FLMG) with a large SSA (1990 m(2) g(-1)) is constructed by chemical vapor deposition on porous magnesium oxide templates. The as-prepared mesoporous graphene presents a high adsorption capacity (260.0 mg g(-1)) for toluene at low toluene concentration (similar to 120 ppm) and a high desorption ratio of 92% for regeneration even at mild heating conditions of 95 degrees C. Additionally, FLMG preserves 80.1% of the initial adsorption capacity even under high humidity (78%). The good adsorption performance of FLMG is due to its high SSA and high mesoporosity, which render a stronger adsorption ability, a larger adsorption accommodation and a more facile desorption behaviour. This work illustrates the further development of advanced graphene materials for enhanced VOC treatment and other environmental applications. |
| WOS关键词 | VOLATILE ORGANIC-COMPOUNDS ; ACTIVATED CARBONS ; SURFACE-AREA ; POROUS GRAPHENE ; CONTACT-ANGLE ; BENZENE ; OXIDE ; VOCS ; DESORPTION ; NITROGEN |
| 资助项目 | National Key RD Plan[2016YFC0200102] |
| WOS研究方向 | Chemistry ; Environmental Sciences & Ecology ; Science & Technology - Other Topics |
| 语种 | 英语 |
| WOS记录号 | WOS:000489724400014 |
| 出版者 | ROYAL SOC CHEMISTRY |
| 资助机构 | National Key RD Plan |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/31284]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Jiang, Jingkun |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, Beijing 100190, Peoples R China 2.Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China 3.Tsinghua Univ, Beijing Key Lab Green Chem React Engn & Technol, Dept Chem Engn, Beijing 100084, Peoples R China 4.Chinese Acad Sci, Inst Chem, Key Lab Green Printing, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Yaling,Li, Zehui,Tang, Cheng,et al. Few-layered mesoporous graphene for high-performance toluene adsorption and regeneration[J]. ENVIRONMENTAL SCIENCE-NANO,2019,6(10):3113-3122. |
| APA | Wang, Yaling.,Li, Zehui.,Tang, Cheng.,Ren, Haixia.,Zhang, Qiang.,...&Jiang, Jingkun.(2019).Few-layered mesoporous graphene for high-performance toluene adsorption and regeneration.ENVIRONMENTAL SCIENCE-NANO,6(10),3113-3122. |
| MLA | Wang, Yaling,et al."Few-layered mesoporous graphene for high-performance toluene adsorption and regeneration".ENVIRONMENTAL SCIENCE-NANO 6.10(2019):3113-3122. |
入库方式： OAI收割
来源：过程工程研究所
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