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A bifunctional luminescent coordination polymer as recyclable sensor for detecting TNP and Fe3+ with high selectivity and sensitivity

文献类型：期刊论文

作者Zhang, Xiaolong1; Hu, Jinsong1,2,3; Li, Jinsong1; Liu, Tingting1; Wang, Jie1; Ma, Xiangmei1
刊名INORGANICA CHIMICA ACTA
出版日期2019-02-24
卷号486页码:556-561
ISSN号0020-1693
关键词Coordination polymer Nitro aromatic explosives Metal ions Fluorescence sensing Selectivity and sensitivity
DOI10.1016/j.ica.2018.11.015
通讯作者Hu, Jinsong(jshu@aust.edu.cn)
英文摘要A thermo-stable three dimensional network [Cd-2(BPDPE)(2)(1,2-H(2)bdc)(2)](n) (1) (1,2-H(2)bdc = 1,2 benzenedicarboxylic acid, BPDPE = 4,4'-bis(pyridyl)diphenyl ether) with blue fluorescence was successfully synthesized and characterized. Complex 1 is a two-dimensional layer constructed by BPDPE connecting [Cd(1,2-bdc)](n) one-dimensional chains, then a three-dimensional network is finally formed via pi center dot center dot center dot pi interactions. Importantly, Complex 1 presents an excellent fluorescent MOF sensor for highly sensitive and selective detecting TNP, the K-sv, is up to 1.03 x 10(5) M-1. Further more, complex 1 can be quickly regenerated by simple washing, exhibiting good recyclability for detecting TNP. In addition, complex 1 shows higher sensitive fluorescent sensor for detecting Fe3+ cation than other metal ions. the K-sv is calculated to be 1.84 x 10(5) M-1. Furthermore, the quenching mechanisms of complex 1 as bifunctional sensor were studied as well.
WOS关键词METAL-ORGANIC FRAMEWORK ; 2,4,6-TRINITROPHENOL TNP ; PORTABLE PROTOTYPE ; LEVEL DETECTION ; POLLUTANT TNP ; MOF ; IONS ; NITROBENZENE ; FABRICATION ; ADSORPTION
资助项目Natural Science Foundation of China[21501002] ; Natural Science Foundation of China[21671004] ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities[KJ2016A196] ; Key Research and Development Project in Anhui Province[1804a09020090]
WOS研究方向Chemistry
语种英语
出版者ELSEVIER SCIENCE SA
WOS记录号WOS:000454151300069
资助机构Natural Science Foundation of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province ; Natural Science Foundation of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province ; Natural Science Foundation of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province ; Natural Science Foundation of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Laboratory of Photochemical Conversion and Optoelectronic Material, TIPC, CAS ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Open Fundation of the Key Lab of Photovoltaic and Energy Conservation Materials, The Key Project of Natural Science Research in Anhui Colleges and Universities ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province ; Key Research and Development Project in Anhui Province
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/41294]  
专题中国科学院合肥物质科学研究院
通讯作者Hu, Jinsong
作者单位1.Anhui Univ Sci & Technol, Sch Chem Engn, Huainan 232001, Peoples R China
2.Chinese Acad Sci, Key Lab Photovolta & Energy Conservat Mat, Hefei Inst Phys Sci, Beijing, Peoples R China
3.Chinese Acad Sci, TIPC, Key Lab Photochem Convers & Optoelect Mat, Beijing, Peoples R China
推荐引用方式
GB/T 7714		 Zhang, Xiaolong,Hu, Jinsong,Li, Jinsong,et al. A bifunctional luminescent coordination polymer as recyclable sensor for detecting TNP and Fe3+ with high selectivity and sensitivity[J]. INORGANICA CHIMICA ACTA,2019,486:556-561.
APA Zhang, Xiaolong,Hu, Jinsong,Li, Jinsong,Liu, Tingting,Wang, Jie,&Ma, Xiangmei.(2019).A bifunctional luminescent coordination polymer as recyclable sensor for detecting TNP and Fe3+ with high selectivity and sensitivity.INORGANICA CHIMICA ACTA,486,556-561.
MLA Zhang, Xiaolong,et al."A bifunctional luminescent coordination polymer as recyclable sensor for detecting TNP and Fe3+ with high selectivity and sensitivity".INORGANICA CHIMICA ACTA 486(2019):556-561.

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来源：合肥物质科学研究院

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