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  4. 中科院固体物理研究所
N-doping nanoporous carbon microspheres derived from MOFs for highly efficient removal of formaldehyde

文献类型：期刊论文

作者Li, Xinyang1; Sun, Yiqiang1,2; Zhang, Tao1,2; Bai, Yu1; Lyu, Xianjun3; Cai, Weiping1; Li, Yue1
刊名NANOTECHNOLOGY
出版日期2019-03-08
卷号30期号:10页码:10
关键词metal-organic framework N-doped nanoporous carbon formaldehyde adsorption
ISSN号0957-4484
DOI10.1088/1361-6528/aaf75b
通讯作者Li, Yue(yueli@issp.ac.cn)
英文摘要Indoor formaldehyde (HCHO) removal is very important to reduce public health risk. Herein, we report a facile method for preparing N-doped nanoporous carbon through direct carbonization of metal-organic frameworks (ZIF-8) to remove harmful formaldehyde. The prepared N-doped nanoporous carbon exhibited uniform morphology and large specific surface area. Moreover, the type of N-functional groups on the N-doped nanoporous carbon had a dominant effect on its HCHO adsorption activity. As a result, HCHO adsorption capacity of the optimized N-doped nanoporous carbon was approximately five times higher than that of the commercially activated carbon. The detailed HCHO adsorption process, including physical adsorption and chemical adsorption, was also confirmed through in situ diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS). In addition, it should be noted that the N-doped nanoporous carbon exhibited high stability for HCHO adsorption, even after six adsorption cycles, indicating its good recyclability for long-term application. This study is expected to pave a way for expanding the environmental applications of the N-doped nanoporous carbon.
WOS关键词THERMAL-CONVERSION ; NITROGEN ; PERFORMANCE ; ADSORPTION ; OXIDATION ; IDENTIFICATION ; DECOMPOSITION ; TEMPERATURE ; ADSORBENT ; COMPOSITE
资助项目National Natural Science Foundation of China[51501186] ; National Natural Science Foundation of China[51601191] ; National Natural Science Foundation of China[51571189] ; National Key Research and Development Program of China[2017YFA0207101] ; Anhui Provincial Natural Science Foundation[1508085JGD07] ; Cross-disciplinary Collaborative Teams Program in CAS ; CAS/SAFEA International Partnership Program for Creative Research Teams
WOS研究方向Science & Technology - Other Topics ; Materials Science ; Physics
语种英语
WOS记录号WOS:000455934700002
出版者IOP PUBLISHING LTD
资助机构National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Foundation ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; Cross-disciplinary Collaborative Teams Program in CAS ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams ; CAS/SAFEA International Partnership Program for Creative Research Teams
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/41500]  
专题合肥物质科学研究院_中科院固体物理研究所
通讯作者Li, Yue
作者单位1.Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Anhui Key Lab Nanomat & Nanotechnol, Hefei 230031, Anhui, Peoples R China
2.Univ Sci & Technol China, Hefei 230026, Anhui, Peoples R China
3.Shandong Univ Sci & Technol, Coll Chem & Environm Engn, Qingdao 266590, Shandong, Peoples R China
推荐引用方式
GB/T 7714		 Li, Xinyang,Sun, Yiqiang,Zhang, Tao,et al. N-doping nanoporous carbon microspheres derived from MOFs for highly efficient removal of formaldehyde[J]. NANOTECHNOLOGY,2019,30(10):10.
APA Li, Xinyang.,Sun, Yiqiang.,Zhang, Tao.,Bai, Yu.,Lyu, Xianjun.,...&Li, Yue.(2019).N-doping nanoporous carbon microspheres derived from MOFs for highly efficient removal of formaldehyde.NANOTECHNOLOGY,30(10),10.
MLA Li, Xinyang,et al."N-doping nanoporous carbon microspheres derived from MOFs for highly efficient removal of formaldehyde".NANOTECHNOLOGY 30.10(2019):10.

入库方式： OAI收割

来源：合肥物质科学研究院

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