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Spatial distribution and seasonal variation of four current-use pesticides (CUPs) in air and surface water of the Bohai Sea, China

文献类型：期刊论文

作者Liu, Lin; Tang, Jianhui; Zhong, Guangcai; Zhen, Xiaomei; Pan, Xiaohui; Tian, Chongguo
刊名SCIENCE OF THE TOTAL ENVIRONMENT
出版日期2018-04-15
卷号621页码:516-523
关键词Current-use pesticides (CUPs) Chlorpyrifos Chlorothalonil Dicofol Bohai Sea Air-sea exchange
ISSN号0048-9697
DOI10.1016/j.scitotenv.2017.11.282
产权排序[Liu, Lin ; Tang, Jianhui ; Zhen, Xiaomei ; Pan, Xiaohui ; Tian, Chongguo] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China ; [Zhong, Guangcai ; Zhen, Xiaomei] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China ; [Liu, Lin ; Zhen, Xiaomei] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
文献子类Article
英文摘要Current-use pesticides (CUPs) arewidely used in agriculture, and some are listed as persistent organic pollutants (POPs) due to their bioaccumulative and toxic properties. China is one of the largest producers and users of pesticides in the world. However, very limited data are available about the environmental fates of CUPs. Four CUPs (trifluralin, chlorothalonil, chlorpyrifos, and dicofol) in surface seawater and lowatmospheric samples taken during research cruises on the Bohai Sea in August and December 2016 and February 2017 were analyzed, we added the spring data sampled in May 2012 to the discussion of seasonal variation. In our study, chlorpyrifos was the most abundant CUPs in the gas phase with a mean abundance of 59.06 +/- 126.94 pg m(-3), and dicofol had the highest concentration dissolved in seawater (mean: 115.94 +/- 123.16 pg L-1). The concentrations of all target compounds were higher during May and August due to intensive use and relatively high temperatures in the spring and summer. Backward trajectories indicated that air masses passing through the eastern coast of the Bohai Sea contained high concentrations of pollutants, while the air masses from the Bohai and Yellow Seas were less polluted. The high concentration of pollutants in seawater was not only influenced by high yields from the source region of production or usage, but also by input from polluted rivers. Volatilization from surface water was found to be an important source of trifluralin and chlorpyrifos in the air. Air-sea gas exchange of chlorothalonil underwent strong net deposition (mean FRs: 51.67), which was driven by higher concentrations in air and indicates that the Bohai Sea acted as a sink for chlorothalonil. (C) 2017 Elsevier B.V. All rights reserved.
WOS关键词POLYCYCLIC AROMATIC-HYDROCARBONS ; ORGANIC-COMPOUNDS SOCS ; CANADIAN AGRICULTURAL REGIONS ; TEFLON MEMBRANE FILTERS ; HISTORIC-USE PESTICIDES ; QUARTZ FIBER FILTERS ; ORGANOCHLORINE PESTICIDES ; RISK-ASSESSMENT ; GAS-EXCHANGE ; NORTH-SEA
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000424196800054
资助机构National Science Foundation of China [41773138] ; Chinese Academy of Sciences [XDA11020401, 2013T2Z0032, 13337KYSB20130013]
源URL[http://ir.yic.ac.cn/handle/133337/24376]  
专题烟台海岸带研究所_近岸生态与环境实验室
烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
作者单位1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
2.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China;
3.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China;
推荐引用方式
GB/T 7714		 Liu, Lin,Tang, Jianhui,Zhong, Guangcai,et al. Spatial distribution and seasonal variation of four current-use pesticides (CUPs) in air and surface water of the Bohai Sea, China[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2018,621:516-523.
APA Liu, Lin,Tang, Jianhui,Zhong, Guangcai,Zhen, Xiaomei,Pan, Xiaohui,&Tian, Chongguo.(2018).Spatial distribution and seasonal variation of four current-use pesticides (CUPs) in air and surface water of the Bohai Sea, China.SCIENCE OF THE TOTAL ENVIRONMENT,621,516-523.
MLA Liu, Lin,et al."Spatial distribution and seasonal variation of four current-use pesticides (CUPs) in air and surface water of the Bohai Sea, China".SCIENCE OF THE TOTAL ENVIRONMENT 621(2018):516-523.

入库方式： OAI收割

来源：烟台海岸带研究所

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