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Isolation and radiocarbon analysis of elemental carbon in atmospheric aerosols using hydropyrolysis

文献类型：期刊论文

作者Zhang, Xiangyun; Li, Jun; Mo, Yangzhi; Shen, Chengde; Ding, Ping; Wang, Ning; Zhu, Sanyuan; Cheng, Zhineng; He, Jiazhuo; Tian, Yankuan
刊名ATMOSPHERIC ENVIRONMENT
出版日期2019-02-01
卷号198页码:381-386
关键词Elemental carbon Atmospheric aerosols Hydropyrolysis Radiocarbon
ISSN号1352-2310
DOI10.1016/j.atmosenv.2018.11.005
产权排序[Zhang, Xiangyun ; Li, Jun ; Mo, Yangzhi ; Zhu, Sanyuan ; Cheng, Zhineng ; He, Jiazhuo ; Tian, Yankuan ; Gao, Shutao ; Zhou, Qin ; Zhang, Gan] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China ; [Shen, Chengde ; Ding, Ping ; Wang, Ning] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Isotope Geochem, Guangzhou 510640, Guangdong, Peoples R China ; [Tian, Chongguo] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Peoples R China ; [Chen, Yingjun] Tongji Univ, Coll Environm Sci & Engn, Shanghai 200092, Peoples R China ; [Zhang, Xiangyun ; Mo, Yangzhi] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
文献子类Article
英文摘要Radiocarbon (C-14) analysis is a powerful tool that can unambiguously distinguish fossil and non-fossil sources of carbonaceous particles. However, one of the big challenges of this method is to isolate elemental carbon (EC) or black carbon (BC) for C-14 analysis. Hydropyrolysis (hypy) has proven to be an effective method for separating BC in environmental matrices. The potential of hypy for isolation of EC from atmospheric aerosols is evaluated using typical combustion products from non-fossil (biomass), fossil fuel (coal and petroleum), and ambient aerosol samples collected in Beijing and Guangzhou. Using solid state nuclear magnetic resonance (NMR) along with measurement of carbon content and C-14, hypy conditions of 15 MPa hydrogen pressure and 550 degrees C temperature was confirmed to effectively separate EC from aerosol samples. Consequently, a comparison study of EC C-14 in aerosol samples separated using the two-step heating method (CTO-375), thermal-optical method and hypy was conducted. The results show that hypy is an effective and stable approach for matrix-independent C-14 quantification of EC in aerosols.
WOS关键词NON-FOSSIL SOURCES ; SOURCE APPORTIONMENT ; ORGANIC-CARBON ; BLACK CARBON ; PYROGENIC CARBON ; C-14 ANALYSIS ; HAZE EVENTS ; QUANTIFICATION ; BIOCHAR ; SYSTEM
WOS研究方向Environmental Sciences ; Meteorology & Atmospheric Sciences
语种英语
WOS记录号WOS:000455693900034
资助机构National Natural Science Foundation of China (NSFC) [41430645, 41473101] ; State Key Laboratory of Organic Geochemistry [SKLOGA201603A, SKLOGC201604] ; Guangzhou Institute of Geochemistry, Chinese Academy of Sciences [GIG-GNKF201603]
源URL[http://ir.yic.ac.cn/handle/133337/24629]  
专题烟台海岸带研究所_近岸生态与环境实验室
烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
作者单位1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Peoples R China;
2.Tongji Univ, Coll Environm Sci & Engn, Shanghai 200092, Peoples R China;
3.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China;
4.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Isotope Geochem, Guangzhou 510640, Guangdong, Peoples R China;
5.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714		 Zhang, Xiangyun,Li, Jun,Mo, Yangzhi,et al. Isolation and radiocarbon analysis of elemental carbon in atmospheric aerosols using hydropyrolysis[J]. ATMOSPHERIC ENVIRONMENT,2019,198:381-386.
APA Zhang, Xiangyun.,Li, Jun.,Mo, Yangzhi.,Shen, Chengde.,Ding, Ping.,...&Zhang, Gan.(2019).Isolation and radiocarbon analysis of elemental carbon in atmospheric aerosols using hydropyrolysis.ATMOSPHERIC ENVIRONMENT,198,381-386.
MLA Zhang, Xiangyun,et al."Isolation and radiocarbon analysis of elemental carbon in atmospheric aerosols using hydropyrolysis".ATMOSPHERIC ENVIRONMENT 198(2019):381-386.

入库方式： OAI收割

来源：烟台海岸带研究所

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