Real-time monitoring of the dissolution of silver nanoparticles by using a solid-contact Ag+-selective electrode
文献类型：期刊论文
| 作者 | Yin, TJ ; Han, TT; Li, CB; Qin, W; Bobacka, J
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| 刊名 | ANALYTICA CHIMICA ACTA
 |
| 出版日期 | 2020-03-08 |
| 卷号 | 1101页码:50-57 |
| ISSN号 | 0003-2670 |
| 关键词 | Solid-contact Ag+-selective electrode Mesoporous carbon Spontaneous dissolution Stimulated dissolution Ag+ |
| DOI | 10.1016/j.aca.2019.12.022 |
| 产权排序 | [Yin, Tanji ; Qin, Wei] Chinese Acad Sci, Shandong Key Lab Coastal Environm Proc, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res YIC,YICCAS, Yantai 264003, Shandong, Peoples R China ; [Yin, Tanji ; Han, Tingting ; Li, Changbai ; Bobacka, Johan] Abo Akad Univ, Johan Gadolin Proc Chem Ctr, Lab Mol Sci & Engn, Biskopsgatan 8, FIN-20500 Turku, Finland ; [Yin, Tanji ; Qin, Wei] Pilot Natl Lab Marine Sci & Technol, Lab Marine Biol & Biotechnol, Qingdao 266200, Peoples R China |
| 文献子类 | Article |
| 英文摘要 | The dissolution kinetics of silver nanoparticles (Ag NPs) to Ag+ ions is a critical factor determining the toxicity of silver nanoparticles. In this work, a solid-contact Ag+-selective electrode (Ag+-ISE) is fabricated and used to monitor the dissolution of Ag NPs. Ordered mesoporous carbon is compared with disordered mesoporous carbon as the solid-contact material for the Ag+-ISE. The ordered mesoporous carbon based solid-contact Ag+-ISE shows a linear potential response in the range of 1.0 x 10(-6)-1.0 x 10(-3) M AgNO3 with the slope of 55.6 +/- 0.8 mV/dec (n = 7) and the detection limit of 10(-6.8) M. The solid-contact Ag+-ISE is used to monitor the concentration changes of Ag+ during spontaneous dissolution of Ag NPs in deionized water, and the dissolution kinetics of Ag NPs is consistent with that obtained by inductively coupled plasma-mass spectrometry (ICP-MS). Stimulated dissolution of Ag NPs induced by addition of H2O2 to the Ag NP solution is also investigated by the proposed solid-contact Ag+-ISE. This work provides a fast tool for charactering the dissolution of Ag NPs to Ag+ in real time, which is important for studying the toxicology of nanoparticles. (C) 2019 Elsevier B.V. All rights reserved. |
| WOS关键词 | MESOPOROUS CARBON ; TOXICITY ; STABILITY ; IONS ; SPECIATION ; IMPACT |
| WOS研究方向 | Chemistry, Analytical |
| 语种 | 英语 |
| WOS记录号 | WOS:000510835500006 |
| 资助机构 | Johan Gadolin Scholarship by the Johan Gadolin Process Chemistry Centre at Abo Akademi University ; National Natural Science Foundation of ChinaNational Natural Science Foundation of China [41706110] |
| 源URL | [http://ir.yic.ac.cn/handle/133337/24740]  |
| 专题 | 烟台海岸带研究所_近岸生态与环境实验室 烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室 |
| 作者单位 | 1.Chinese Acad Sci, Shandong Key Lab Coastal Environm Proc, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res YIC,YICCAS, Yantai 264003, Shandong, Peoples R China; 2.Pilot Natl Lab Marine Sci & Technol, Lab Marine Biol & Biotechnol, Qingdao 266200, Peoples R China 3.Abo Akad Univ, Johan Gadolin Proc Chem Ctr, Lab Mol Sci & Engn, Biskopsgatan 8, FIN-20500 Turku, Finland; |
| 推荐引用方式 GB/T 7714 | Yin, TJ,Han, TT,Li, CB,et al. Real-time monitoring of the dissolution of silver nanoparticles by using a solid-contact Ag+-selective electrode[J]. ANALYTICA CHIMICA ACTA,2020,1101:50-57. |
| APA | Yin, TJ,Han, TT,Li, CB,Qin, W,&Bobacka, J.(2020).Real-time monitoring of the dissolution of silver nanoparticles by using a solid-contact Ag+-selective electrode.ANALYTICA CHIMICA ACTA,1101,50-57. |
| MLA | Yin, TJ,et al."Real-time monitoring of the dissolution of silver nanoparticles by using a solid-contact Ag+-selective electrode".ANALYTICA CHIMICA ACTA 1101(2020):50-57. |
入库方式： OAI收割
来源：烟台海岸带研究所
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