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Occurrence and spatial distribution of phthalate esters in sediments of the Bohai and Yellow seas

文献类型：期刊论文

作者Mi, LJ; Xie, ZY; Zhao, Z; Zhong, MY; Mi, WY; Ebinghaus, R; Tang, JH
刊名SCIENCE OF THE TOTAL ENVIRONMENT
出版日期2019-02-25
卷号653页码:792-800
关键词Phthalate ester DEHP Sediment Bohai Sea Yellow Sea Marine environment
ISSN号0048-9697
DOI10.1016/j.scitotenv.2018.10.438
产权排序[Mi, Lijie ; Zhong, Mingyu ; Tang, Jianhui] Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China ; [Xie, Zhiyong ; Ebinghaus, Ralf] Helmholtz Zentrum Geesthacht, Inst Coastal Res, Ctr Mat & Coastal Res, D-21502 Geesthacht, Germany ; [Zhao, Zhen] Nankai Univ, Coll Environm Sci & Engn, MOE Key Lab Pollut Proc & Environm Criteria, Tianjin 300350, Peoples R China ; [Mi, Wenying] MINJIE Inst Environm Sci & Hlth Res, D-21502 Geesthacht, Germany
文献子类Article
英文摘要Phthalate esters (PEs) are a class of synthetic chemicals that have been widely used as plasticizers in industrial products and households. The occurrence of PEs in the marine environment has been a concern for many years because of their adverse impacts on marine organisms and human health. In this study, six major PEs, i.e. diethyl phthalate (DEP), di-isobutyl phthalate (DiBP), di-n-butyl phthalate (DnBP), benzylbutyl phthalate (BBP), dicyclohexyl phthalate (DCHP) and di-(2-ethylhexyl) phthalate (DEHP), were analyzed in sediment samples collected in the Bohai and Yellow seas. The sum concentrations of the six PEs ranged from 1.4 to 24.6 ng/g and the average was 9.1 ng/g. The highest concentrations of PEs in the sediment samples were those of DEHP with a median concentration of 3.77 ng/g, followed by DiBP (median, 1.60 ng/g), DnBP (0.91 ng/g), DEP (0.32 ng/g), BBP (0.03 ng/g) and DCHP (0.01 ng/g). Generally, concentrations of PEs in the Bohai Sea are higher than those in the Yellow Sea. The varying spatial distributions of the individual PEs can be the result of discharge sources, regional ocean circulation patterns, and mud areas in the Bohai and Yellow seas. Significant positive correlations were found between total organic carbon content and the concentrations of DiBP, DnBP, and DEHP. It is estimated that the inventories of the Sigma 6PEs were 20.73 tons in the Bohai Sea and 65.87 tons in the Yellow Sea. Both riverine discharge and atmospheric deposition are major input sources for the PE sedimentation, while massive plastic litter and microplastics sinking to the ocean floor can directly release PEs into sediment. This study provides an appropriate data set for the assessment of the risk of PEs to the marine ecosystem. (c) 2018 Elsevier B.V. All rights reserved.
WOS关键词ECOLOGICAL RISK-ASSESSMENT ; ACID-ESTERS ; ORGANIC POLLUTANTS ; COASTAL SEDIMENTS ; SURFACE SEDIMENTS ; KAOHSIUNG HARBOR ; RIVER ESTUARY ; CHINA ; MICROPLASTICS ; SEAWATER
WOS研究方向Environmental Sciences
语种英语
WOS记录号WOS:000458626800080
资助机构Chinese Academy of SciencesChinese Academy of Sciences [KZCX2-EW-QN210, KZZD-EW-14, YZ201161] ; National Natural Science Foundation of ChinaNational Natural Science Foundation of China [40933048, 41073064] ; German BMBFFederal Ministry of Education & Research (BMBF) [03F0786C]
源URL[http://ir.yic.ac.cn/handle/133337/24992]  
专题烟台海岸带研究所_近岸生态与环境实验室
烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
作者单位1.Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China;
2.MINJIE Inst Environm Sci & Hlth Res, D-21502 Geesthacht, Germany
3.Helmholtz Zentrum Geesthacht, Inst Coastal Res, Ctr Mat & Coastal Res, D-21502 Geesthacht, Germany;
4.Nankai Univ, Coll Environm Sci & Engn, MOE Key Lab Pollut Proc & Environm Criteria, Tianjin 300350, Peoples R China;
推荐引用方式
GB/T 7714		 Mi, LJ,Xie, ZY,Zhao, Z,et al. Occurrence and spatial distribution of phthalate esters in sediments of the Bohai and Yellow seas[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2019,653:792-800.
APA Mi, LJ.,Xie, ZY.,Zhao, Z.,Zhong, MY.,Mi, WY.,...&Tang, JH.(2019).Occurrence and spatial distribution of phthalate esters in sediments of the Bohai and Yellow seas.SCIENCE OF THE TOTAL ENVIRONMENT,653,792-800.
MLA Mi, LJ,et al."Occurrence and spatial distribution of phthalate esters in sediments of the Bohai and Yellow seas".SCIENCE OF THE TOTAL ENVIRONMENT 653(2019):792-800.

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来源：烟台海岸带研究所

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