原料和制炭方式对生物炭吸附抗生素的影响
文献类型：期刊论文
| 作者 | 冯丽蓉; 校亮 ; 袁国栋; 毕冬雪; 韦婧
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| 刊名 | 中国环境科学
 |
| 出版日期 | 2020-03-20 |
| 卷号 | 40期号:03页码:1156-1165 |
| 关键词 | 生物炭 制炭方式 土霉素 磺胺甲恶唑 吸附 |
| ISSN号 | 1000-6923 |
| 其他题名 | Biomass feedstocks and carbonization methods affect antibiotic adsorption on biochar |
| 产权排序 | (1) 中国科学院烟台海岸带研究所中国科学院海岸带环境过程与生态修复重点实验室 ; (2) 中国科学院大学 ; (3) 广东省环境健康与资源利用重点实验室 ; (4) 肇庆学院环境与化学工程学院 |
| 文献子类 | 期刊论文 |
| 英文摘要 | Biochar has been reported as a useful adsorbent of organic contaminants. Here, reed, cotton stalk, and bamboo willow were selected as feedstocks to produce biochars via oxygen-limited or aerobic methods for carbonization. The obtained biochars were first characterized for their physical and chemical properties and then investigated for their performance in adsorbing oxytetracycline（OTC） and sulfamethoxazole（SMX）. It was found that both feedstocks and carbonization methods affected OTC and SMX adsorption. Reed and cotton stalks were better carbonized under oxygen-limited conditions to produce biochars（O2-limited biochars）, whereas bamboo willow was suitable to produce biochars via aerobic carbonization（aerobic biochar）. The aerobic biochar adsorbed 11.98 and 10.12 mg/g of OTC and SMX, respectively, from a solution with an initial concentration of 50 mg/L of the biotics. Batch adsorption experiments and the Fourier transform infrared spectroscopic analysis indicated that π-π electron donor-acceptor interaction was the primary mechanisms for OTC and SMX adsorption on the aerobic biochar. Electrostatic attraction further promoted OTC adsorption on aerobic biochar at high pHs, whereas pore filling could contribute to SMX adsorption. This work showed that aerobic biochar were better adsorbents of OTC and SMX than O2-limited biochars, and suggested that biochar adsorbents can be tailor-made for different contaminants by judicious selection of feedstocks and carbonization processes. |
| 语种 | 中文 |
| 资助机构 | 国家重点研发计划项目(2016YFD0200303) ; 烟台市重点研发计划项目(2019XDHZ104) |
| 源URL | [http://ir.yic.ac.cn/handle/133337/25180]  |
| 专题 | 烟台海岸带研究所_近岸生态与环境实验室 |
| 作者单位 | 1.肇庆学院环境与化学工程学院 2.中国科学院烟台海岸带研究所中国科学院海岸带环境过程与生态修复重点实验室; 3.中国科学院大学; 4.广东省环境健康与资源利用重点实验室; |
| 推荐引用方式 GB/T 7714 | 冯丽蓉,校亮,袁国栋,等. 原料和制炭方式对生物炭吸附抗生素的影响[J]. 中国环境科学,2020,40(03):1156-1165. |
| APA | 冯丽蓉,校亮,袁国栋,毕冬雪,&韦婧.(2020).原料和制炭方式对生物炭吸附抗生素的影响.中国环境科学,40(03),1156-1165. |
| MLA | 冯丽蓉,et al."原料和制炭方式对生物炭吸附抗生素的影响".中国环境科学 40.03(2020):1156-1165. |
入库方式： OAI收割
来源：烟台海岸带研究所
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