Simultaneous Removal of NOx and SO2 by MgO Combined with O-3 Oxidation: The Influencing Factors and O-3 Consumption Distributions
文献类型：期刊论文
| 作者 | Zou, Yang2,4; Liu, Xiaolong2; Zhu, Tingyu2,3; Tian, Mengkui4; Cai, Maoyu2,4; Zhao, Ziwei2; Wu, Heng1,2 |
| 刊名 | ACS OMEGA
 |
| 出版日期 | 2019-12-17 |
| 卷号 | 4期号:25页码:21091-21099 |
| ISSN号 | 2470-1343 |
| DOI | 10.1021/acsomega.9b02502 |
| 英文摘要 | Simultaneous removal of NOx and SO2 by MgO combined with O-3 oxidation was studied. The effects of the O-3/NO molar ratio, oxidation temperature, and oxidation residence time on N2O5 decomposition and O-3 consumption distributions were systematically illustrated, which is of great significance for improving NOx removal efficiency and reducing O-3 consumption in practical application. When the O-3/NO molar ratio was greater than 1.0, the highest N2O5 yield was achieved at 90 degrees C. The NOx removal efficiency reached 96.5% at an O-3/NO molar ratio of 1.8. The oxidation temperature increased from 90 to 130 degrees C, resulting in the decrease of N2O5 yield, the improvement of O-3-ICC (O-3 invalid cycle consumption) caused by N2O5 decomposition, and the decrease of NOx removal efficiency from 96.5 to 76%. Besides, the effects of pH, SO2 concentration, and MgSO3 addition on NOx removal efficiency were also investigated. The results showed that the removal efficiency of NO(x )decreased with the increase of SO2 concentration, while MgSO3 addition into MgO slurry could promote the absorption of NO2 due to the reaction between NO2 and SO32-. |
| WOS关键词 | SELECTIVE CATALYTIC-REDUCTION ; FLUE-GAS ; OZONE INJECTION ; SIMULTANEOUS ABSORPTION ; AIR-POLLUTION ; KINETICS ; SYSTEMS ; PRODUCT ; AMMONIA ; OXIDES |
| 资助项目 | National key research and development program of China[2017YFC0210600] ; National Natural Science Foundation of China[51978644] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000503370500027 |
| 出版者 | AMER CHEMICAL SOC |
| 资助机构 | National key research and development program of China ; National Natural Science Foundation of China |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/38664]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Liu, Xiaolong; Zhu, Tingyu |
| 作者单位 | 1.Kunming Univ Sci & Technol, Environm Sci & Engn, Kunming 650500, Yunnan, Peoples R China 2.Chinese Acad Sci, Beijing Engn Res Ctr Proc Pollut Control, Natl Engn Lab Hydromet Cleaner Prod Technol, Inst Proc Engn, Beijing 100190, Peoples R China 3.Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Fujian, Peoples R China 4.Guizhou Univ, Chem & Chem Engn, Guiyang 550025, Guizhou, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zou, Yang,Liu, Xiaolong,Zhu, Tingyu,et al. Simultaneous Removal of NOx and SO2 by MgO Combined with O-3 Oxidation: The Influencing Factors and O-3 Consumption Distributions[J]. ACS OMEGA,2019,4(25):21091-21099. |
| APA | Zou, Yang.,Liu, Xiaolong.,Zhu, Tingyu.,Tian, Mengkui.,Cai, Maoyu.,...&Wu, Heng.(2019).Simultaneous Removal of NOx and SO2 by MgO Combined with O-3 Oxidation: The Influencing Factors and O-3 Consumption Distributions.ACS OMEGA,4(25),21091-21099. |
| MLA | Zou, Yang,et al."Simultaneous Removal of NOx and SO2 by MgO Combined with O-3 Oxidation: The Influencing Factors and O-3 Consumption Distributions".ACS OMEGA 4.25(2019):21091-21099. |
入库方式： OAI收割
来源：过程工程研究所
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