Formation and toxicity of polycyclic aromatic hydrocarbons during CaO assisted hydrothermal carbonization of swine manure
文献类型：期刊论文
| 作者 | Lang, Qianqian2,3; Zhang, Bo1; Li, Yi4; Liu, Zhengang2,3; Jiao, Wentao2,3 |
| 刊名 | WASTE MANAGEMENT
 |
| 出版日期 | 2019-12-01 |
| 卷号 | 100页码:84-90 |
| 关键词 | Hydrothermal carbonization Swine manure CaO introduction Polycyclic aromatic hydrocarbons Soil amendment |
| ISSN号 | 0956-053X |
| DOI | 10.1016/j.wasman.2019.09.010 |
| 英文摘要 | The effects of temperature and Ca0 introduction on polycyclic aromatic hydrocarbons (PAHs) contents, distribution patterns and toxicity of the products from hydrothermal carbonization (HTC) of swine manure (SM) were investigated in this study for the first time. The results indicated that increasing temperature decreased total PAHs content of the hydrochar, while the PAHs toxicity firstly decreased and then increased during HTC of SM. For the aqueous product, the total PAHs content and toxicity gradually decreased with increasing temperature. CaO introduction during HTC of SM significantly suppressed the PAHs formation and promoted the transformation from higher molecular weight PAHs into lower molecular weight PAHs in HTC products, resulting in the remarkably decreased content and toxicity of PAHs. The lowest total PAHs content (1428.57 mu g/kg) and TEQ value (21.33 mu g/kg) of the hydrochar were obtained by 15% CaO introduction at 200 degrees C and 180 degrees C, respectively, and compared to SM, they were decreased by 73.73% and 79.51%, respectively. Moreover, 3-ring PAHs were the predominant PAHs in HTC products regardless of CaO introduction. The present study demonstrated that CaO assisted HTC at temperature lower than 220 degrees C was effective to reduce the total content and toxicity of PAHs in SM, and the prepared hydrochar was a promising soil amendment in view of the elimination of PAHs toxicity. (C) 2019 Elsevier Ltd. All rights reserved. |
| WOS关键词 | SEWAGE-SLUDGE ; HYDROCHAR ; PYROLYSIS ; PAHS ; SOIL ; BIOMASS ; WATER ; IDENTIFICATION ; GASIFICATION ; TEMPERATURE |
| 资助项目 | "100 Talents" Program of the Chinese Academy of Sciences[Y5N41I1C01] ; Science and Technology Department of Sichuan Province[2018YZ0016] |
| WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:000494887900010 |
| 出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
| 资助机构 | "100 Talents" Program of the Chinese Academy of Sciences ; Science and Technology Department of Sichuan Province |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/38948]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Liu, Zhengang; Jiao, Wentao |
| 作者单位 | 1.Shandong Prov Environm Technol Serv Ctr, Jinan 250102, Shandong, Peoples R China 2.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Beijing 100085, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 4.Chinese Acad Sci, IPE, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lang, Qianqian,Zhang, Bo,Li, Yi,et al. Formation and toxicity of polycyclic aromatic hydrocarbons during CaO assisted hydrothermal carbonization of swine manure[J]. WASTE MANAGEMENT,2019,100:84-90. |
| APA | Lang, Qianqian,Zhang, Bo,Li, Yi,Liu, Zhengang,&Jiao, Wentao.(2019).Formation and toxicity of polycyclic aromatic hydrocarbons during CaO assisted hydrothermal carbonization of swine manure.WASTE MANAGEMENT,100,84-90. |
| MLA | Lang, Qianqian,et al."Formation and toxicity of polycyclic aromatic hydrocarbons during CaO assisted hydrothermal carbonization of swine manure".WASTE MANAGEMENT 100(2019):84-90. |
入库方式： OAI收割
来源：过程工程研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。