High Phase-Purity 1T-MoS2 Ultrathin Nanosheets by a Spatially Confined Template
文献类型：期刊论文
| 作者 | Chen, Xiaoyu3; Wang, Zumin1; Wei, Yanze3; Zhang, Xing3; Zhang, Qinghua5; Gu, Lin5; Zhang, Lijuan1; Yang, Nailiang1,2; Yu, Ranbo3,4 |
| 刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
 |
| 出版日期 | 2019-10-23 |
| 页码 | 5 |
| 关键词 | hydrogen evolution reaction intercalation metastable phases molybdenum disulfide nanosheets |
| ISSN号 | 1433-7851 |
| DOI | 10.1002/anie.201909879 |
| 英文摘要 | The crystal phase plays an important role in controlling the properties of a nanomaterial; however, it is a great challenge to obtain a nanomaterial with high purity of the metastable phase. For instance, the large-scale synthesis of the metallic phase MoS2 (1T-MoS2) is important for enhancing electrocatalytic reaction, but it can only be obtained under harsh conditions. Herein, a spatially confined template method is proposed to synthesize high phase-purity MoS2 with a 1T content of 83%. Moreover, both the confined space and the structure of template will affect the purity of 1T-MoS2; in this case, this approach was extended to other similar spatially confined templates to obtain the high-purity material. The obtained ultrathin nanosheets exhibit good electrocatalytic activity and excellent stability in the hydrogen evolution reaction. |
| WOS关键词 | LAYERED DOUBLE HYDROXIDES ; MOS2 NANOSHEETS ; HYDROGEN EVOLUTION ; TRANSITION ; 1T ; ELECTRODE ; CLOTH |
| 资助项目 | National Natural Science Foundation of China[21671016] ; National Natural Science Foundation of China[51872024] ; National Natural Science Foundation of China[51932001] ; National Natural Science Foundation of China[21971244] ; China Postdoctoral Science Foundation[2019M650849] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000494204400001 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | National Natural Science Foundation of China ; China Postdoctoral Science Foundation |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/39075]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Yang, Nailiang; Yu, Ranbo |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, 1 North 2nd St, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 10049, Peoples R China 3.Univ Sci & Technol Beijing, Sch Met & Ecol Engn, Dept Phys Chem, 30 Xueyuan Rd, Beijing 100083, Peoples R China 4.Zhengzhou Univ, Minist Educ, Key Lab Adv Mat Proc & Mold, Zhengzhou 450002, Henan, Peoples R China 5.Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Xiaoyu,Wang, Zumin,Wei, Yanze,et al. High Phase-Purity 1T-MoS2 Ultrathin Nanosheets by a Spatially Confined Template[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2019:5. |
| APA | Chen, Xiaoyu.,Wang, Zumin.,Wei, Yanze.,Zhang, Xing.,Zhang, Qinghua.,...&Yu, Ranbo.(2019).High Phase-Purity 1T-MoS2 Ultrathin Nanosheets by a Spatially Confined Template.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,5. |
| MLA | Chen, Xiaoyu,et al."High Phase-Purity 1T-MoS2 Ultrathin Nanosheets by a Spatially Confined Template".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019):5. |
入库方式： OAI收割
来源：过程工程研究所
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