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Hard-Sphere Random Close-Packed Au47Cd2(TBBT)(31) Nanoclusters with a Faradaic Efficiency of Up to 96% for Electrocatalytic CO2 Reduction to CO

文献类型：期刊论文

作者Zhuang, Shengli1,2; Chen, Dong3; Liao, Lingwen1,2; Zhao, Yan1,2; Xia, Nan1,2; Zhang, Wenhao1,2; Wang, Chengming4; Yang, Jun3; Wu, Zhikun1,2
刊名ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
出版日期2020-02-17
卷号59期号:8页码:3073-3077
关键词cadmium CO2 reduction electrocatalysis gold nanoclusters two-phase anti-galvanic reduction
ISSN号1433-7851
DOI10.1002/anie.201912845
英文摘要Metal nanoclusters have recently attracted considerable attention, not only because of their special size range but also because of their well-defined compositions and structures. However, subtly tailoring the compositions and structures of metal nanoclusters for potential applications remains challenging. Now, a two-phase anti-galvanic reduction (AGR) method is presented for precisely tailoring Au-44(TBBT)(28) to produce Au47Cd2(TBBT)(31) nanoclusters with a hard-sphere random close-packed structure, exhibiting Faradaic efficiencies of up to 96% at -0.57 V for the electrocatalytic reduction of CO2 to CO.
WOS关键词ANTI-GALVANIC REDUCTION ; THIOLATE-PROTECTED GOLD ; AU-25 ; CLUSTERS ; ELECTROREDUCTION ; NANOPARTICLES ; ATOMS
资助项目National Natural Science Foundation of China[21829501] ; National Natural Science Foundation of China[21925303] ; National Natural Science Foundation of China[21905284] ; National Natural Science Foundation of China[21771186] ; National Natural Science Foundation of China[21706265] ; National Natural Science Foundation of China[21603234] ; National Natural Science Foundation of China[21573212] ; National Natural Science Foundation of China[21573240] ; National Natural Science Foundation of China[21222301] ; National Natural Science Foundation of China[21171170] ; National Natural Science Foundation of China[21528303] ; China Postdoctoral Science Foundation[Y94G4E356B] ; Key Program of 13th five-year plan, CASHIPS[KP-2017-16] ; Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology[2017FXCX002] ; National Key R&D Program of China[2017YFA0207302] ; Center of Mesosicence, Institute of Process Engineering Chinese Academy of sciences[MPCS-2019-A-09] ; CASHIPS DirectorQs Fund[BJPY2019A02]
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000519891700002
出版者WILEY-V C H VERLAG GMBH
资助机构National Natural Science Foundation of China ; China Postdoctoral Science Foundation ; Key Program of 13th five-year plan, CASHIPS ; Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; National Key R&D Program of China ; Center of Mesosicence, Institute of Process Engineering Chinese Academy of sciences ; CASHIPS DirectorQs Fund
源URL[http://ir.ipe.ac.cn/handle/122111/39777]  
专题中国科学院过程工程研究所
通讯作者Yang, Jun; Wu, Zhikun
作者单位1.Chinese Acad Sci, Key Lab Mat Phys, Anhui Key Lab Nanomat & Nanotechnol, CAS Ctr Excellence Nanosci,Inst Solid State Phys, Hefei 230031, Anhui, Peoples R China
2.Anhui Univ, Inst Phys Sci & Informat Technol, Hefei 230601, Anhui, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
4.Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China
推荐引用方式
GB/T 7714		 Zhuang, Shengli,Chen, Dong,Liao, Lingwen,et al. Hard-Sphere Random Close-Packed Au47Cd2(TBBT)(31) Nanoclusters with a Faradaic Efficiency of Up to 96% for Electrocatalytic CO2 Reduction to CO[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2020,59(8):3073-3077.
APA Zhuang, Shengli.,Chen, Dong.,Liao, Lingwen.,Zhao, Yan.,Xia, Nan.,...&Wu, Zhikun.(2020).Hard-Sphere Random Close-Packed Au47Cd2(TBBT)(31) Nanoclusters with a Faradaic Efficiency of Up to 96% for Electrocatalytic CO2 Reduction to CO.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,59(8),3073-3077.
MLA Zhuang, Shengli,et al."Hard-Sphere Random Close-Packed Au47Cd2(TBBT)(31) Nanoclusters with a Faradaic Efficiency of Up to 96% for Electrocatalytic CO2 Reduction to CO".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 59.8(2020):3073-3077.

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