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When hollow multishelled structures (HoMSs) meet metal-organic frameworks (MOFs)

文献类型：期刊论文

作者Wang, Zumin2; Yang, Nailiang1,2; Wang, Dan1,2
刊名CHEMICAL SCIENCE
出版日期2020-06-07
卷号11期号:21页码:5359-5368
ISSN号2041-6520
DOI10.1039/d0sc01284j
英文摘要Hollow multishelled structures (HoMSs) have distinguished advantages, such as a large effective surface area, an optimized mass transport route, and a high loading capacity, but the fabrication of HoMSs has been a big challenge. In 2009, we developed a universal and facile method for HoMS fabrication, i.e., the sequential templating approach (STA). Progress in the synthetic methodology has enabled the study of HoMSs to develop and has made it a research hotspot in materials science. To date, HoMSs have shown their advantages in a wide range of applications, including catalysis, energy conversion and storage, drug delivery, etc. Based on the understanding in this field, we recently revealed the unique temporal-spatial ordering properties of HoMSs. Furthermore, we have been wondering if the structure of a HoMS can be modulated at the molecular level. Encouragingly, metal-organic frameworks (MOFs) are star materials with clearly defined molecular structures. The compositions, geometries, functionalities and topologies of MOFs have been well tuned by rational design. Integrating the unique properties of MOFs and HoMS could realize the systemic design of materials from the molecular to the micro-level, which would provide a series of advantages for various applications, such as developing high performance catalysts for cascade and/or selective catalysis, combining the reaction and separation process for multiple reactions, releasing drugs in a certain environment for smart medicine, and so on. We believe it is time to summarize the recent progress in the integration of MOFs and HoMSs, including HoMSs coated with MOFs, MOF-derived HoMSs, and MOFs with a hollow multishelled structure, and we also put forward our personal outlook in relation to the future opportunities and challenges in this emerging yet promising research field.
WOS关键词CRYSTAL ; MICROSPHERES ; COORDINATION ; PERFORMANCE ; SPHERES ; BATTERIES ; CATALYST ; DESIGN ; ANODES ; SNO2
资助项目National Natural Science Foundation of China[21590795] ; National Natural Science Foundation of China[21820102002] ; National Natural Science Foundation of China[21971244] ; Scientific Instrument Developing Project of the Chinese Academy of Sciences[YZ201623]
WOS研究方向Chemistry
语种英语
出版者ROYAL SOC CHEMISTRY
WOS记录号WOS:000538158300001
资助机构National Natural Science Foundation of China ; Scientific Instrument Developing Project of the Chinese Academy of Sciences
源URL[http://ir.ipe.ac.cn/handle/122111/40922]  
专题中国科学院过程工程研究所
通讯作者Wang, Dan
作者单位1.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 100049, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, 1 North 2nd St, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714		 Wang, Zumin,Yang, Nailiang,Wang, Dan. When hollow multishelled structures (HoMSs) meet metal-organic frameworks (MOFs)[J]. CHEMICAL SCIENCE,2020,11(21):5359-5368.
APA Wang, Zumin,Yang, Nailiang,&Wang, Dan.(2020).When hollow multishelled structures (HoMSs) meet metal-organic frameworks (MOFs).CHEMICAL SCIENCE,11(21),5359-5368.
MLA Wang, Zumin,et al."When hollow multishelled structures (HoMSs) meet metal-organic frameworks (MOFs)".CHEMICAL SCIENCE 11.21(2020):5359-5368.

入库方式： OAI收割

来源：过程工程研究所

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