Broadening of the Fluorescence Spectra of Sesquioxide Crystals for Ultrafast Lasers
文献类型：期刊论文
| 作者 | Liu, Wenyu1,5; Lu, Dazhi1,5; Guo, Ruiqi1,5; Wu, Kui6; Pan, Shilie2; Hang, Yin3; Sun, Dunlu4 ; Yu, Haohai1,5; Zhang, Huaijin1,5; Wang, Jiyang1,5
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| 刊名 | CRYSTAL GROWTH & DESIGN
 |
| 出版日期 | 2020-07-01 |
| 卷号 | 20 |
| ISSN号 | 1528-7483 |
| DOI | 10.1021/acs.cgd.0c00473 |
| 通讯作者 | Yu, Haohai(haohaiyu@sdu.edu.cn) ; Zhang, Huaijin(huaijinzhang@sdu.edu.cn) |
| 英文摘要 | Sesquioxide crystals were identified as promising gain media for high-power ultrafast lasers, and the broadening of their fluorescence spectra could shorten the achievable laser pulses, corresponding to the enhancement of the peak powers. In this study, we demonstrate the broadening of the fluorescence spectra of the sesquioxides with the electron-phonon coupling effect and ligand engineering associated with the advantages of the Lu2O3 host in the phonon energy and insensitivity to doping concentrations. The Yb:LuxY2-xO3 (0 <= x <= 2) sesquioxide crystals were grown and characterized. The introduction of Y3+ ions broadens the fluorescence spectra by approximately two times those of Yb:Lu2O3, which could be attributed to the strong electron-phonon coupling effect and octahedral distortion. This work would provide a series of novel laser materials for high-power ultrafast lasers and pave a new route for designing functional materials aimed at the enhancement of the given performance. |
| WOS关键词 | BOND-VALENCE PARAMETERS ; THERMAL-CONDUCTIVITY ; PHONON-SCATTERING ; CONTINUOUS-WAVE ; YB ; POWER ; PERFORMANCE ; CONVERSION ; OPERATION ; LINES |
| 资助项目 | National Key Research and Development Program of China[2016YFB1102301] ; National Natural Science Foundation of China[51772172] |
| WOS研究方向 | Chemistry ; Crystallography ; Materials Science |
| 语种 | 英语 |
| WOS记录号 | WOS:000546699900050 |
| 出版者 | AMER CHEMICAL SOC |
| 资助机构 | National Key Research and Development Program of China ; National Natural Science Foundation of China |
| 源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/71249]  |
| 专题 | 中国科学院合肥物质科学研究院 |
| 通讯作者 | Yu, Haohai; Zhang, Huaijin |
| 作者单位 | 1.Shandong Univ, Inst Crystal Mat, Jinan 250100, Shandong, Peoples R China 2.Chinese Acad Sci, Xinjiang Tech Inst Phys & Chem, Urumqi 830011, Xinjiang, Peoples R China 3.Chinese Acad Sci, Shanghai Inst Opt & Fine Mech, Shanghai 201800, Peoples R China 4.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Shanghai 201800, Peoples R China 5.Shandong Univ, State Key Lab Crystal Mat, Jinan 250100, Shandong, Peoples R China 6.Hebei Univ, Coll Chem & Environm Sci, Baoding 071002, Hebei, Peoples R China |
| 推荐引用方式 GB/T 7714 | Liu, Wenyu,Lu, Dazhi,Guo, Ruiqi,et al. Broadening of the Fluorescence Spectra of Sesquioxide Crystals for Ultrafast Lasers[J]. CRYSTAL GROWTH & DESIGN,2020,20. |
| APA | Liu, Wenyu.,Lu, Dazhi.,Guo, Ruiqi.,Wu, Kui.,Pan, Shilie.,...&Wang, Jiyang.(2020).Broadening of the Fluorescence Spectra of Sesquioxide Crystals for Ultrafast Lasers.CRYSTAL GROWTH & DESIGN,20. |
| MLA | Liu, Wenyu,et al."Broadening of the Fluorescence Spectra of Sesquioxide Crystals for Ultrafast Lasers".CRYSTAL GROWTH & DESIGN 20(2020). |
入库方式： OAI收割
来源：合肥物质科学研究院
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