中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
NOx Emission Flux Measurements with Multiple Mobile-DOAS Instruments in Beijing

文献类型:期刊论文

作者Huang, Yeyuan2,5; Li, Ang5; Xie, Pinhua2,3,5; Hu, Zhaokun5; Xu, Jin5; Fang, Xiaoyi1; Ren, Hongmei2,5; Li, Xiaomei2,5; Dang, Bing4
刊名REMOTE SENSING
出版日期2020-08-01
卷号12
关键词NOX emission flux mobile-DOAS mega-city
DOI10.3390/rs12162527
通讯作者Li, Ang(angli@aiofm.ac.cn)
英文摘要

NOX(NOX= NO + NO2) emissions measurements in Beijing are of great significance because they can aid in understanding how NOX pollution develops in mega-cities throughout China. However, NO(X)emissions in mega-cities are difficult to measure due to changes in wind patterns and moving sources on roads during measurement. To obtain good spatial coverage on different ring roads in Beijing over a short amount of time, two mobile differential optical absorption spectroscopy (DOAS) instruments were used to measure NOX emission flux from April 18th to 26th, 2018. In addition, a wind profile radar provided simultaneous wind field measurements for altitudes between 50 m and 1 km for each ring road measurement. We first determined NOX emission flux of different ring roads using wind field averages from measured wind data. The results showed that the NO(X)emission flux of Beijing's fifth ring road, which represented the urban part, varied from (19.29 +/- 5.26) x 10(24) molec./s to (36.46 +/- 12.86) x 10(24)molec./s. On April 20th, NOX emission flux for the third ring was slightly higher than the fourth ring because the two ring roads were measured at different time periods. We then analyzed the NO(X)emission flux error budget and error sensitivity. The main error source was the wind field uncertainty. For some measurements, the main emission flux error source was either wind speed uncertainty or wind direction uncertainty, but not both. As Beijing's NOX emissions came from road vehicle exhaust, we found that emission flux error had a more diverse sensitivity to wind direction uncertainty, which improved our knowledge on this topic. The NOX emission flux error sensitivity study indicated that more accurate measurements of the wind field are crucial for effective NOX emission flux measurements in Chinese mega-cities. Obtaining actual time and high resolved wind measurements is an advantage for mega-cities' NOX emission flux measurements. The emission flux errors caused by wind direction and wind speed uncertainties were clearly distinguished. Other sensitivity studies indicated that NOX/NO2 ratio uncertainty dominated flux errors when the NOX/NO2 ratio uncertainty was >0.4. Using two mobile-DOAS and wind profile radars to measure NOx emission flux improved the quality of the emission flux measuring results. This approach could be applied to many other mega-cities in China and in others countries.

WOS关键词TROPOSPHERIC NO2 ; MINI-DOAS ; SO2 ; CHINA ; OMI ; AREA ; QUANTIFICATION ; STATISTICS ; VALIDATION ; POLLUTION
资助项目National Natural Science Foundation of China[:41775029] ; National Natural Science Foundation of China[91644110] ; National Natural Science Foundation of China[41530644] ; National Natural Science Foundation of China[41975037] ; National Key Research and Development Project of China[2018YFC0213201] ; National Key Research and Development Project of China[2017YFC0209902] ; Science and Technology Commission of Shanghai Municipality[17DZ1203102]
WOS研究方向Remote Sensing
语种英语
WOS记录号WOS:000565443100001
出版者MDPI
资助机构National Natural Science Foundation of China ; National Key Research and Development Project of China ; Science and Technology Commission of Shanghai Municipality
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/92724]  
专题中国科学院合肥物质科学研究院
通讯作者Li, Ang
作者单位1.Chinese Acad Meteorol Sci, Beijing 100081, Peoples R China
2.Univ Sci & Technol China, Hefei 230026, Peoples R China
3.Chinese Acad Sci, CAS Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361000, Peoples R China
4.Beijing Municipal Climate Ctr, Beijing 100089, Peoples R China
5.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Hefei Inst Phys Sci, Key Lab Environm Opt & Technol, Hefei 230031, Peoples R China
推荐引用方式
GB/T 7714
Huang, Yeyuan,Li, Ang,Xie, Pinhua,et al. NOx Emission Flux Measurements with Multiple Mobile-DOAS Instruments in Beijing[J]. REMOTE SENSING,2020,12.
APA Huang, Yeyuan.,Li, Ang.,Xie, Pinhua.,Hu, Zhaokun.,Xu, Jin.,...&Dang, Bing.(2020).NOx Emission Flux Measurements with Multiple Mobile-DOAS Instruments in Beijing.REMOTE SENSING,12.
MLA Huang, Yeyuan,et al."NOx Emission Flux Measurements with Multiple Mobile-DOAS Instruments in Beijing".REMOTE SENSING 12(2020).

入库方式: OAI收割

来源:合肥物质科学研究院

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