NOx Emission Flux Measurements with Multiple Mobile-DOAS Instruments in Beijing
文献类型:期刊论文
作者 | Huang, Yeyuan2,5; Li, Ang5![]() ![]() ![]() |
刊名 | REMOTE SENSING
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出版日期 | 2020-08-01 |
卷号 | 12 |
关键词 | NOX emission flux mobile-DOAS mega-city |
DOI | 10.3390/rs12162527 |
通讯作者 | Li, Ang(angli@aiofm.ac.cn) |
英文摘要 | NOX(NOX= NO + NO2) emissions measurements in Beijing are of great significance because they can aid in understanding how NOX pollution develops in mega-cities throughout China. However, NO(X)emissions in mega-cities are difficult to measure due to changes in wind patterns and moving sources on roads during measurement. To obtain good spatial coverage on different ring roads in Beijing over a short amount of time, two mobile differential optical absorption spectroscopy (DOAS) instruments were used to measure NOX emission flux from April 18th to 26th, 2018. In addition, a wind profile radar provided simultaneous wind field measurements for altitudes between 50 m and 1 km for each ring road measurement. We first determined NOX emission flux of different ring roads using wind field averages from measured wind data. The results showed that the NO(X)emission flux of Beijing's fifth ring road, which represented the urban part, varied from (19.29 +/- 5.26) x 10(24) molec./s to (36.46 +/- 12.86) x 10(24)molec./s. On April 20th, NOX emission flux for the third ring was slightly higher than the fourth ring because the two ring roads were measured at different time periods. We then analyzed the NO(X)emission flux error budget and error sensitivity. The main error source was the wind field uncertainty. For some measurements, the main emission flux error source was either wind speed uncertainty or wind direction uncertainty, but not both. As Beijing's NOX emissions came from road vehicle exhaust, we found that emission flux error had a more diverse sensitivity to wind direction uncertainty, which improved our knowledge on this topic. The NOX emission flux error sensitivity study indicated that more accurate measurements of the wind field are crucial for effective NOX emission flux measurements in Chinese mega-cities. Obtaining actual time and high resolved wind measurements is an advantage for mega-cities' NOX emission flux measurements. The emission flux errors caused by wind direction and wind speed uncertainties were clearly distinguished. Other sensitivity studies indicated that NOX/NO2 ratio uncertainty dominated flux errors when the NOX/NO2 ratio uncertainty was >0.4. Using two mobile-DOAS and wind profile radars to measure NOx emission flux improved the quality of the emission flux measuring results. This approach could be applied to many other mega-cities in China and in others countries. |
WOS关键词 | TROPOSPHERIC NO2 ; MINI-DOAS ; SO2 ; CHINA ; OMI ; AREA ; QUANTIFICATION ; STATISTICS ; VALIDATION ; POLLUTION |
资助项目 | National Natural Science Foundation of China[:41775029] ; National Natural Science Foundation of China[91644110] ; National Natural Science Foundation of China[41530644] ; National Natural Science Foundation of China[41975037] ; National Key Research and Development Project of China[2018YFC0213201] ; National Key Research and Development Project of China[2017YFC0209902] ; Science and Technology Commission of Shanghai Municipality[17DZ1203102] |
WOS研究方向 | Remote Sensing |
语种 | 英语 |
WOS记录号 | WOS:000565443100001 |
出版者 | MDPI |
资助机构 | National Natural Science Foundation of China ; National Key Research and Development Project of China ; Science and Technology Commission of Shanghai Municipality |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/92724] ![]() |
专题 | 中国科学院合肥物质科学研究院 |
通讯作者 | Li, Ang |
作者单位 | 1.Chinese Acad Meteorol Sci, Beijing 100081, Peoples R China 2.Univ Sci & Technol China, Hefei 230026, Peoples R China 3.Chinese Acad Sci, CAS Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361000, Peoples R China 4.Beijing Municipal Climate Ctr, Beijing 100089, Peoples R China 5.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Hefei Inst Phys Sci, Key Lab Environm Opt & Technol, Hefei 230031, Peoples R China |
推荐引用方式 GB/T 7714 | Huang, Yeyuan,Li, Ang,Xie, Pinhua,et al. NOx Emission Flux Measurements with Multiple Mobile-DOAS Instruments in Beijing[J]. REMOTE SENSING,2020,12. |
APA | Huang, Yeyuan.,Li, Ang.,Xie, Pinhua.,Hu, Zhaokun.,Xu, Jin.,...&Dang, Bing.(2020).NOx Emission Flux Measurements with Multiple Mobile-DOAS Instruments in Beijing.REMOTE SENSING,12. |
MLA | Huang, Yeyuan,et al."NOx Emission Flux Measurements with Multiple Mobile-DOAS Instruments in Beijing".REMOTE SENSING 12(2020). |
入库方式: OAI收割
来源:合肥物质科学研究院
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