Regulation of intrinsic physicochemical properties of metal oxide nanomaterials for energy conversion and environmental detection applications
文献类型：期刊论文
| 作者 | Chen, Li1,2; Liu, Zhonggang1,2; Guo, Zheng1,2; Huang, Xing-Jiu1,2,3,4
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| 刊名 | JOURNAL OF MATERIALS CHEMISTRY A
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| 出版日期 | 2020-09-14 |
| 卷号 | 8 |
| ISSN号 | 2050-7488 |
| DOI | 10.1039/d0ta05539e |
| 通讯作者 | Guo, Zheng(zhguo@ahu.edu.cn) ; Huang, Xing-Jiu(xingjiuhuang@iim.ac.cn) |
| 英文摘要 | In response to the global energy crisis and damage to humans by environmental issues, metal oxide nanomaterials (nonprecious) represent an important class of materials for energy conversion and environmental detection on account of their natural abundance, easy synthesis, low cost, and excellent stability. A majority of pristine metal oxide nanomaterials have certain shortcomings in catalysis and sensing, such as poor conductivity and wide bandgap. Fortunately, the regulation of the intrinsic physicochemical properties of metal oxide nanomaterials is a very promising approach for improving their catalytic and sensing properties for energy conversion and environmental detection. In this review, we will mainly discuss the regulation of the intrinsic physicochemical properties, namely, shape and size, defects, crystal facets, and ion cycles of metal oxide nanomaterials, with a majority of applications involving photocatalytic water splitting and CO2 reduction, electrocatalytic water splitting, heavy metal ion (HMI) detection, and metal oxide gas sensors. Density functional theory (DFT) calculations and X-ray absorption fine-structure (XAFS) spectroscopy analysis have been used to evaluate the effects of regulation of the intrinsic physicochemical properties of metal oxide nanomaterials, as well as to further identify the relationship between the intrinsic physicochemical properties and their enhanced catalytic and sensing properties with regard to energy conversion and environmental detection. Finally, some unresolved problems associated with future perspectives in this field are discussed, inspiring further development of the intrinsic physicochemical properties of metal oxide nanomaterials. |
| WOS关键词 | CORE-SHELL NANOWIRES ; GAS-SENSING PROPERTIES ; SENSITIVE ELECTROCHEMICAL DETECTION ; PHOTOCATALYTIC OXYGEN EVOLUTION ; HIGH-YIELD SYNTHESIS ; VISIBLE-LIGHT ; CONTROLLABLE SYNTHESIS ; ANATASE TIO2 ; FACILE SYNTHESIS ; EXPOSED 001 |
| 资助项目 | National Natural Science Foundation of China[21735005] ; National Natural Science Foundation of China[21802145] ; National Natural Science Foundation of China[61774159] ; National Natural Science Foundation of China[21904001] ; Anhui Provincial Natural Science Foundation[2008085QF320] ; Anhui Provincial Natural Science Foundation[2008085QF288] ; Science and Technology Research Project of Anhui Province[1704c0402195] ; Key Program of 13th.ve-year plan ; CASHIPS |
| WOS研究方向 | Chemistry ; Energy & Fuels ; Materials Science |
| 语种 | 英语 |
| WOS记录号 | WOS:000566092600049 |
| 出版者 | ROYAL SOC CHEMISTRY |
| 资助机构 | National Natural Science Foundation of China ; Anhui Provincial Natural Science Foundation ; Science and Technology Research Project of Anhui Province ; Key Program of 13th.ve-year plan ; CASHIPS |
| 源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/102897]  |
| 专题 | 中国科学院合肥物质科学研究院 |
| 通讯作者 | Guo, Zheng; Huang, Xing-Jiu |
| 作者单位 | 1.Anhui Univ, Inst Phys Sci, Hefei 230601, Peoples R China 2.Anhui Univ, Inst Phys Sci, Informat Mat & Intelligent Sensing Lab Anhui Prov, Hefei 230601, Anhui, Peoples R China 3.Chinese Acad Sci, Inst Intelligent Machines, Hefei 230031, Peoples R China 4.Univ Sci & Technol China, Dept Chem, Hefei 230026, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Li,Liu, Zhonggang,Guo, Zheng,et al. Regulation of intrinsic physicochemical properties of metal oxide nanomaterials for energy conversion and environmental detection applications[J]. JOURNAL OF MATERIALS CHEMISTRY A,2020,8. |
| APA | Chen, Li,Liu, Zhonggang,Guo, Zheng,&Huang, Xing-Jiu.(2020).Regulation of intrinsic physicochemical properties of metal oxide nanomaterials for energy conversion and environmental detection applications.JOURNAL OF MATERIALS CHEMISTRY A,8. |
| MLA | Chen, Li,et al."Regulation of intrinsic physicochemical properties of metal oxide nanomaterials for energy conversion and environmental detection applications".JOURNAL OF MATERIALS CHEMISTRY A 8(2020). |
入库方式： OAI收割
来源：合肥物质科学研究院
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