Activation strategies of water-splitting electrocatalysts
文献类型：期刊论文
| 作者 | Liu, Peng Fei2; Yin, Huajie1; Fu, Huai Qin1,2; Zu, Meng Yang2; Yang, Hua Gui2; Zhao, Huijun1,3 |
| 刊名 | JOURNAL OF MATERIALS CHEMISTRY A
 |
| 出版日期 | 2020-05-28 |
| 卷号 | 8 |
| ISSN号 | 2050-7488 |
| DOI | 10.1039/d0ta01680b |
| 通讯作者 | Yang, Hua Gui(hgyang@ecust.edu.cn) ; Zhao, Huijun(h.zhao@griffith.edu.au) |
| 英文摘要 | Electrocatalysts featuring high activity, selectivity and stability are urgently needed in solar-electricity powered energy-conversion technologies. In the past decade, various electrocatalysts have been demonstrated to be electrocatalytically active toward the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). Despite the significant progress, catalyst discovery is still dominated by "trial-and-error" practice due to the lack of understanding of the origin of electrocatalytic activity, active site structures and key factors determining the operando electrocatalytic performance. Therefore, this critical review focuses on summarizing effective catalyst activation strategies to enable efficient catalyst discovery, on the basis of understanding real active sites for the HER and OER. Meanwhile, theory prediction and operando characterization techniques have also been introduced to identify the origin of electrocatalytic activity and active site structures. Moreover, catalyst atomic structure reconstruction/rearrangement under working conditions and the accompanying catalyst activation strategies have been discussed to address the negative impacts of reaction media. Finally, a brief perspective on the challenges and future directions for predicting, characterizing and understanding operando active sites to discover efficient activation strategies will also be presented. |
| WOS关键词 | HYDROGEN EVOLUTION REACTION ; LAYERED DOUBLE HYDROXIDE ; HIGHLY-ACTIVE ELECTROCATALYST ; AMORPHOUS MOLYBDENUM SULFIDE ; RAY-ABSORPTION SPECTROSCOPY ; ENHANCED CATALYTIC-ACTIVITY ; OXYGEN EVOLUTION ; SINGLE-ATOM ; PEROVSKITE ELECTROCATALYST ; EFFICIENT ELECTROCATALYSTS |
| 资助项目 | Australian Research Council (ARC) Discovery Project[DP170104834] ; National Natural Science Funds for Distinguished Young Scholar[51725201] ; International (Regional) Cooperation and Exchange Projects of the National Natural Science Foundation of China[51920105003] ; Innovation Program of Shanghai Municipal Education Commission[E00014] ; National Natural Science Foundation of China[21573068] ; National Natural Science Foundation of China[51902105] ; Shanghai Engineering Research Center of Hierarchical Nanomaterials[18DZ2252400] ; Shanghai Sailing Program[19YF1411600] ; China Postdoctoral Science Foundation[2018M641938] ; Griffith University Postdoctoral Fellowship |
| WOS研究方向 | Chemistry ; Energy & Fuels ; Materials Science |
| 语种 | 英语 |
| WOS记录号 | WOS:000539350100003 |
| 出版者 | ROYAL SOC CHEMISTRY |
| 资助机构 | Australian Research Council (ARC) Discovery Project ; National Natural Science Funds for Distinguished Young Scholar ; International (Regional) Cooperation and Exchange Projects of the National Natural Science Foundation of China ; Innovation Program of Shanghai Municipal Education Commission ; National Natural Science Foundation of China ; Shanghai Engineering Research Center of Hierarchical Nanomaterials ; Shanghai Sailing Program ; China Postdoctoral Science Foundation ; Griffith University Postdoctoral Fellowship |
| 源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/102983]  |
| 专题 | 中国科学院合肥物质科学研究院 |
| 通讯作者 | Yang, Hua Gui; Zhao, Huijun |
| 作者单位 | 1.Griffith Univ, Ctr Clean Environm & Energy, Gold Coast Campus, Gold Coast, Qld 4222, Australia 2.East China Univ Sci & Technol, Shanghai Engn Res Ctr Hierarch Nanomat, Sch Mat Sci & Engn, Key Lab Ultrafine Mat,Minist Educ, Shanghai 200237, Peoples R China 3.Chinese Acad Sci, Inst Solid State Phys, CAS Ctr Excellence Nanosci, Ctr Environm & Energy Nanomat, Hefei 230031, Peoples R China |
| 推荐引用方式 GB/T 7714 | Liu, Peng Fei,Yin, Huajie,Fu, Huai Qin,et al. Activation strategies of water-splitting electrocatalysts[J]. JOURNAL OF MATERIALS CHEMISTRY A,2020,8. |
| APA | Liu, Peng Fei,Yin, Huajie,Fu, Huai Qin,Zu, Meng Yang,Yang, Hua Gui,&Zhao, Huijun.(2020).Activation strategies of water-splitting electrocatalysts.JOURNAL OF MATERIALS CHEMISTRY A,8. |
| MLA | Liu, Peng Fei,et al."Activation strategies of water-splitting electrocatalysts".JOURNAL OF MATERIALS CHEMISTRY A 8(2020). |
入库方式： OAI收割
来源：合肥物质科学研究院
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