Solvent-free engineering of Fe-0/Fe3C nanoparticles encased in nitrogen-doped carbon nanoshell materials for highly efficient removal of uranyl ions from acidic solution
文献类型：期刊论文
| 作者 | Zhu, Kairuo2,3; Song, Gang1 ; Ren, Xuemei3; Chen, Changlun2,3
|
| 刊名 | JOURNAL OF COLLOID AND INTERFACE SCIENCE
 |
| 出版日期 | 2020-09-01 |
| 卷号 | 575 |
| 关键词 | Fe-0/Fe3C nanoparticles Nitrogen-doped carbon U(VI) removal |
| ISSN号 | 0021-9797 |
| DOI | 10.1016/j.jcis.2020.04.091 |
| 通讯作者 | Chen, Changlun(clchen@ipp.ac.cn) |
| 英文摘要 | In this work, nitrogen-doped carbon nanoshell structure with the encased Fe-0/Fe3C nanoparticles (Fe@NC) was synthesized with a solvent-free method via direct carbonizing the ground mixture of dicyandiamide and ferric chloride hexahydrate. The morphology, structure, and surface properties of as-synthesized Fe@NC were characterized systematically, and the removal performance of Fe@NC towards U(VI) was studied in detail. The results manifested that the Fe@NC possessed large surface area (127.0 m(2)/g) with mesoporosity and the encapsulated Fe-0/Fe3C nanoparticles were concentrated at the tip of N-doped carbon nanotubes. Moreover, the Fe@NC hybrid material exhibited the maximum removal capacities of 0.85 and 0.44 mg/m(2) at pH 4.5 and 1.5, respectively. The mechanism of U(VI) removal by the Fe@NC was attributed to the synergistic effects of adsorption via nitrogen/oxygen-containing groups and redox reaction between Fe-0/Fe2+ and U(VI). (C) 2020 Elsevier Inc. All rights reserved. |
| WOS关键词 | ZERO-VALENT IRON ; AQUEOUS-SOLUTION ; CATALYTIC DEGRADATION ; INTERACTION MECHANISM ; U(VI) ADSORPTION ; URANIUM ; NANOTUBES ; COMPOSITE ; ENCAPSULATION ; MICROSPHERES |
| 资助项目 | National Natural Science Foundation of China[21976184] ; Research Fund Program of Guangdong Provincial Key Laboratory of Radionuclides Pollution Control and Resources[2017B030314182] ; China Postdoctoral Science Foundation[2019M652228] ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000538935500002 |
| 出版者 | ACADEMIC PRESS INC ELSEVIER SCIENCE |
| 资助机构 | National Natural Science Foundation of China ; Research Fund Program of Guangdong Provincial Key Laboratory of Radionuclides Pollution Control and Resources ; China Postdoctoral Science Foundation ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences |
| 源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/102993]  |
| 专题 | 中国科学院合肥物质科学研究院 |
| 通讯作者 | Chen, Changlun |
| 作者单位 | 1.Guangzhou Univ, Sch Environm Sci & Engn, Guangdong Prov Key Lab Radionuclides Pollut Contr, Guangzhou 510006, Peoples R China 2.Soochow Univ, Collaborat Innovat Ctr Radiat Med Jiangsu Higher, Suzhou 215123, Peoples R China 3.Chinese Acad Sci, Inst Plasma Phys, Key Lab Photovolta & Energy Conservat Mat, POB 1126, Hefei 230031, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhu, Kairuo,Song, Gang,Ren, Xuemei,et al. Solvent-free engineering of Fe-0/Fe3C nanoparticles encased in nitrogen-doped carbon nanoshell materials for highly efficient removal of uranyl ions from acidic solution[J]. JOURNAL OF COLLOID AND INTERFACE SCIENCE,2020,575. |
| APA | Zhu, Kairuo,Song, Gang,Ren, Xuemei,&Chen, Changlun.(2020).Solvent-free engineering of Fe-0/Fe3C nanoparticles encased in nitrogen-doped carbon nanoshell materials for highly efficient removal of uranyl ions from acidic solution.JOURNAL OF COLLOID AND INTERFACE SCIENCE,575. |
| MLA | Zhu, Kairuo,et al."Solvent-free engineering of Fe-0/Fe3C nanoparticles encased in nitrogen-doped carbon nanoshell materials for highly efficient removal of uranyl ions from acidic solution".JOURNAL OF COLLOID AND INTERFACE SCIENCE 575(2020). |
入库方式： OAI收割
来源：合肥物质科学研究院
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