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Fourier transform infrared time series of tropospheric HCN in eastern China: seasonality, interannual variability, and source attribution

文献类型：期刊论文

作者Sun, Youwen2; Liu, Cheng2,3,4,5,6; Zhang, Lin1; Palm, Mathias7; Notholt, Justus7; Hao, Yin2; Vigouroux, Corinne8; Lutsch, Erik9; Wang, Wei2; Shan, Changong2
刊名ATMOSPHERIC CHEMISTRY AND PHYSICS
出版日期2020-05-11
卷号20
ISSN号1680-7316
DOI10.5194/acp-20-5437-2020
通讯作者Liu, Cheng(chliu81@ustc.edu.cn) ; Zhang, Lin(zhanglg@pku.edu.cn)
英文摘要We analyzed seasonality and interannual variability of tropospheric hydrogen cyanide (HCN) columns in densely populated eastern China for the first time. The results were derived from solar absorption spectra recorded with a ground-based high-spectral-resolution Fourier transform infrared (FTIR) spectrometer in Hefei (31 degrees 54' N, 117 degrees 10' E) between 2015 and 2018. The tropospheric HCN columns over Hefei, China, showed significant seasonal variations with three monthly mean peaks throughout the year. The magnitude of the tropospheric HCN column peaked in May, September, and December. The tropospheric HCN column reached a maximum monthly mean of (9.8 +/- 0.78) x 10(15) molecules cm(-2) in May and a minimum monthly mean of (7.16 +/- 0.75) x 10(15) molecules cm(-2) in November. In most cases, the tropospheric HCN columns in Hefei (32 degrees N) are higher than the FTIR observations in Ny-angstrom lesund (79 degrees N), Kiruna (68 degrees N), Bremen (53 degrees N), Jungfraujoch (47 degrees N), Toronto (44 degrees N), Rikubetsu (43 degrees N), Izana (28 degrees N), Mauna Loa (20 degrees N), La Reunion Maido (21 degrees S), Lauder (45 degrees S), and Arrival Heights (78 degrees S) that are affiliated with the Network for Detection of Atmospheric Composition Change (NDACC). Enhancements of tropospheric HCN column were observed between September 2015 and July 2016 compared to the same period of measurements in other years. The magnitude of the enhancement ranges from 5 % to 46 % with an average of 22 %. Enhancement of tropospheric HCN (Delta HCN) is correlated with the concurrent enhancement of tropospheric CO (Delta CO), indicating that enhancements of tropospheric CO and HCN were due to the same sources. The GEOS-Chem tagged CO simulation, the global fire maps, and the potential source contribution function (PSCF) values calculated using back trajectories revealed that the seasonal maxima in May are largely due to the influence of biomass burning in Southeast Asia (SEAS) (41 +/- 13.1 %), Europe and boreal Asia (EUBA) (21 +/- 9.3 %), and Africa (AF) (22 +/- 4.7 %). The seasonal maxima in September are largely due to the influence of biomass burnings in EUBA (38 +/- 11.3 %), AF (26 +/- 6.7 %), SEAS (14 +/- 3.3 %), and North America (NA) (13.8 +/- 8.4 %). For the seasonal maxima in December, dominant contributions are from AF (36 +/- 7.1 %), EUBA (21 +/- 5.2 %), and NA (18.7 +/- 5.2 %). The tropospheric HCN enhancement between September 2015 and July 2016 at Hefei (32 degrees N) was attributed to an elevated influence of biomass burnings in SEAS, EUBA, and Oceania (OCE) in this period. In particular, an elevated number of fires in OCE in the second half of 2015 dominated the tropospheric HCN enhancement between September and December 2015. An elevated number of fires in SEAS in the first half of 2016 dominated the tropospheric HCN enhancement between January and July 2016.
WOS关键词HIGH-RESOLUTION ; NORTHERN JAPAN ; SPECTROSCOPIC MEASUREMENTS ; ANTHROPOGENIC EMISSIONS ; FTIR MEASUREMENTS ; HYDROGEN-CYANIDE ; CARBON-MONOXIDE ; SURFACE OZONE ; SOLAR SPECTRA ; TRACE GASES
资助项目National High Technology Research and Development Program of China[2019YFC0214802] ; National High Technology Research and Development Program of China[2017YFC0210002] ; National High Technology Research and Development Program of China[2016YFC0203302] ; National High Technology Research and Development Program of China[2018YFC0213201] ; National High Technology Research and Development Program of China[2019YFC0214702] ; National High Technology Research and Development Program of China[2016YFC0200404] ; National Science Foundation of China[41877309] ; National Science Foundation of China[41775025] ; National Science Foundation of China[41575021] ; National Science Foundation of China[51778596] ; National Science Foundation of China[91544212] ; National Science Foundation of China[41722501] ; Sino-German Mobility Programme[M-0036] ; Outstanding Youth Science Foundation[41722501]
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
语种英语
WOS记录号WOS:000531881700001
出版者COPERNICUS GESELLSCHAFT MBH
资助机构National High Technology Research and Development Program of China ; National Science Foundation of China ; Sino-German Mobility Programme ; Outstanding Youth Science Foundation
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/103323]  
专题中国科学院合肥物质科学研究院
通讯作者Liu, Cheng; Zhang, Lin
作者单位1.Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Lab Climate & Ocean Atmosphere Studies, Beijing 100871, Peoples R China
2.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Key Lab Environm Opt & Technol, HFIPS, Hefei 230031, Peoples R China
3.Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China
4.Univ Sci & Technol China, Hefei 230026, Peoples R China
5.Univ Sci & Technol China, Key Lab Precis Sci Instrumentat Anhui Higher Educ, Hefei 230026, Peoples R China
6.Anhui Prov Key Lab Polar Environm & Global Change, Hefei 230026, Peoples R China
7.Univ Bremen, Inst Environm Phys, POB 330440, Bremen 28334, Germany
8.Royal Belgian Inst Space Aeron BIRA IASB, Brussels, Belgium
9.Univ Toronto, Dept Phys, Toronto, ON, Canada
10.Karlsruhe Inst Technol KIT, Inst Meteorol & Climate Res IMK ASF, Karlsruhe, Germany
推荐引用方式
GB/T 7714		 Sun, Youwen,Liu, Cheng,Zhang, Lin,et al. Fourier transform infrared time series of tropospheric HCN in eastern China: seasonality, interannual variability, and source attribution[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2020,20.
APA Sun, Youwen.,Liu, Cheng.,Zhang, Lin.,Palm, Mathias.,Notholt, Justus.,...&Liu, Jianguo.(2020).Fourier transform infrared time series of tropospheric HCN in eastern China: seasonality, interannual variability, and source attribution.ATMOSPHERIC CHEMISTRY AND PHYSICS,20.
MLA Sun, Youwen,et al."Fourier transform infrared time series of tropospheric HCN in eastern China: seasonality, interannual variability, and source attribution".ATMOSPHERIC CHEMISTRY AND PHYSICS 20(2020).

入库方式： OAI收割

来源：合肥物质科学研究院

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