Giant electrocaloric response in compositional manipulated BaTiO3 relaxor-ferroelectric system
文献类型:期刊论文
作者 | Hou, Ying1; Li, Jiacheng1; Ding, Junfeng3; Ye, Tingting3; Liang, Ruihong2 |
刊名 | JOURNAL OF APPLIED PHYSICS |
出版日期 | 2020-02-14 |
卷号 | 127 |
ISSN号 | 0021-8979 |
DOI | 10.1063/1.5142635 |
通讯作者 | Hou, Ying(houying@ecust.edu.cn) |
英文摘要 | The compositional manipulation of the multiphase coexistence in relaxor-ferroelectrics has been reported to be an effective approach to generate the giant electrocaloric effect. In this work, we systemically investigate the temperature-dependent electrocaloric effect in BaZr0.18Ti0.82O3-BaSn0.11Ti0.89O3 relaxors, where Zr and Sn are introduced into BaTiO3 to develop the multiphase coexistence at the ferroelectric-paraelectric transition. Through the direct measurement by the heat flux sensor, a large temperature change around 4 K under an electric field of 10 MV m(-1), combined with a broad temperature span (20 degrees C-60 degrees C), has been observed. For comparison, the electrocaloric properties are also indirectly deduced based on Maxwell equations and Landau-Ginzburg-Devonshire phenomenological theory, and the validity of the indirect methods in this relaxor-ferroelectric system has been discussed. This work would shed light on developing giant electrocaloric materials with a wide operating temperature range. Published under license by AIP Publishing. |
WOS关键词 | TEMPERATURE ; NANOCOMPOSITES ; EFFICIENT ; FILMS |
资助项目 | Natural Science Foundation of Shanghai[19ZR1411900] ; National Natural Science Foundation of China[91963116] ; National Natural Science Foundation of China[51303053] ; Chen-guang Talent Foundation of the Shanghai Education and Development Committee[14CG28] ; Key Laboratory of Inorganic Functional Materials and Devices, Chinese Academy of Sciences[KLIFMD201707] ; Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences[2018KLMP01] |
WOS研究方向 | Physics |
语种 | 英语 |
出版者 | AMER INST PHYSICS |
WOS记录号 | WOS:000522036200015 |
资助机构 | Natural Science Foundation of Shanghai ; National Natural Science Foundation of China ; Chen-guang Talent Foundation of the Shanghai Education and Development Committee ; Key Laboratory of Inorganic Functional Materials and Devices, Chinese Academy of Sciences ; Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/103621] |
专题 | 中国科学院合肥物质科学研究院 |
通讯作者 | Hou, Ying |
作者单位 | 1.East China Univ Sci & Technol, Dept Phys, Shanghai 200237, Peoples R China 2.Chinese Acad Sci, Shanghai Inst Ceram, Key Lab Inorgan Funct Mat & Devices, Shanghai 201899, Peoples R China 3.Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Peoples R China |
推荐引用方式 GB/T 7714 | Hou, Ying,Li, Jiacheng,Ding, Junfeng,et al. Giant electrocaloric response in compositional manipulated BaTiO3 relaxor-ferroelectric system[J]. JOURNAL OF APPLIED PHYSICS,2020,127. |
APA | Hou, Ying,Li, Jiacheng,Ding, Junfeng,Ye, Tingting,&Liang, Ruihong.(2020).Giant electrocaloric response in compositional manipulated BaTiO3 relaxor-ferroelectric system.JOURNAL OF APPLIED PHYSICS,127. |
MLA | Hou, Ying,et al."Giant electrocaloric response in compositional manipulated BaTiO3 relaxor-ferroelectric system".JOURNAL OF APPLIED PHYSICS 127(2020). |
入库方式: OAI收割
来源:合肥物质科学研究院
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