Micro-nano-engineered nitrogenous bone biochar developed with a ball-milling technique for high-efficiency removal of aquatic Cd(II), Cu(II) and Pb(II)
文献类型：期刊论文
| 作者 | Xiao, Jiang2; Hu, Rui1; Chen, Guangcai2 |
| 刊名 | JOURNAL OF HAZARDOUS MATERIALS
 |
| 出版日期 | 2020-04-05 |
| 卷号 | 387 |
| 关键词 | Engineered bone biochar Ball-milling Heavy metals Adsorption Complexing mechanism |
| ISSN号 | 0304-3894 |
| DOI | 10.1016/j.jhazmat.2019.121980 |
| 通讯作者 | Hu, Rui(ruihu@mtek.cas.cn) ; Chen, Guangcai(guangcaichen@sohu.com) |
| 英文摘要 | A cost-effective and eco-friendly engineering method to improve biochar's physicochemical and sorption performance is critical in various environmental applications. In this study, micro-nano-engineered nitrogenous biochars derived from cow bone meal pyrolyzed at different temperatures and were engineered with the assistance of a ball-milling technique. The ball-milled bone biochars were natural composites combined with plant biochars and hydroxyapatite components on the micro-nanoscale. Both the micropore area and the external specific surface area of the bone biochars were significantly improved after ball-milling. The sorption capacities for heavy metal ions were heavy metal ions were MBC-600 > MBC-450 > BC-600 > MBC-300 > BC-450 > BC-300, consistent with the variation tendency in the specific surface areas of the bone biochars. The adsorption capacities of MBC-600 for Cd(II), Cu(II) and Pb(II) were 165.77, 287.58 and 558.88 mg/g, respectively (T 298K, pH 5.0), representing increases of 93.91.%, 75.56% and 64.61% compared with the un-milled preparation. Surface complexation, cation exchange, chemical precipitation, electrostatic interaction and cation-n bonding were responsible for the removal of heavy metal ions by bone biochar materials. Taken together, the results show that micro-nano-engineered nitrogenous bone biochar prepared using ball-milling technology is a promising material for the remediation of heavy metals-bearing aquatic environments. |
| WOS关键词 | STRAW-DERIVED BIOCHAR ; HEAVY-METAL IONS ; COMPETITIVE ADSORPTION ; AQUEOUS-SOLUTIONS ; MILLED BIOCHAR ; LEAD ; CARBON ; MECHANISMS ; WATER ; SOIL |
| 资助项目 | Key Research and Development Program of Zhejiang Province[2018C03047] ; China Postdoctoral Science Foundation[2018M640200] ; China Postdoctoral Science Foundation[2019T120154] ; CAS Pioneer Hundred Talents Program ; CASHIPS Director's Fund[YZJJ2018QN20] ; National Natural Science Foundation of China[21875257] |
| WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:000514758500020 |
| 出版者 | ELSEVIER |
| 资助机构 | Key Research and Development Program of Zhejiang Province ; China Postdoctoral Science Foundation ; CAS Pioneer Hundred Talents Program ; CASHIPS Director's Fund ; National Natural Science Foundation of China |
| 源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/103981]  |
| 专题 | 中国科学院合肥物质科学研究院 |
| 通讯作者 | Hu, Rui; Chen, Guangcai |
| 作者单位 | 1.Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Hefei 230088, Peoples R China 2.Chinese Acad Forestry, Res Inst Subtrop Forestry, Hangzhou 311400, Zhejiang, Peoples R China |
| 推荐引用方式 GB/T 7714 | Xiao, Jiang,Hu, Rui,Chen, Guangcai. Micro-nano-engineered nitrogenous bone biochar developed with a ball-milling technique for high-efficiency removal of aquatic Cd(II), Cu(II) and Pb(II)[J]. JOURNAL OF HAZARDOUS MATERIALS,2020,387. |
| APA | Xiao, Jiang,Hu, Rui,&Chen, Guangcai.(2020).Micro-nano-engineered nitrogenous bone biochar developed with a ball-milling technique for high-efficiency removal of aquatic Cd(II), Cu(II) and Pb(II).JOURNAL OF HAZARDOUS MATERIALS,387. |
| MLA | Xiao, Jiang,et al."Micro-nano-engineered nitrogenous bone biochar developed with a ball-milling technique for high-efficiency removal of aquatic Cd(II), Cu(II) and Pb(II)".JOURNAL OF HAZARDOUS MATERIALS 387(2020). |
入库方式： OAI收割
来源：合肥物质科学研究院
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