中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Characterization of urban CO2 column abundance with a portable low resolution spectrometer (PLRS): Comparisons with GOSAT and GEOS-Chem model data

文献类型:期刊论文

作者Tian, Yuan2,3; Sun, Youwen1,3; Liu, Cheng1,3,4; Xie, Pinhua3; Chan, Kalok5; Xu, Jin3; Wang, Wei3; Liu, Jianguo3
刊名SCIENCE OF THE TOTAL ENVIRONMENT
出版日期2018-01-15
卷号612期号:页码:1593-1609
关键词Remote sensing Carbon dioxide City emission Seasonal cycle GOSAT GEOS-Chem
ISSN号0048-9697
DOI10.1016/j.scitotenv.2016.12.005
英文摘要

We presented the characterization of urban CO2 column abundance (XCO2) in Hefei, China using a portable low resolution spectrometer (PLRS). An optimized correction spectrum was introduced in the spectral fitting to improve CO2 retrieval. A pronounced seasonal cycle and diurnal variation were observed with a precision of similar to 0.12%. The CO2 concentrations in winter are about 5-10 ppm higher than those in summer. Most diurnal variations exhibited downward trends. The measurement in the early morning is about 2-5 ppm higher than the late afternoon observation. The causes of the seasonal and diurnal trends were systematic analyzed. The coincident CO2 time series were compared with the Greenhouse Gases Observing SATellite (GOSAT) data and the GEOS-Chem global 3-D tropospheric chemistry model data. We found the ground based (g-b) PLRS data are systematically higher than the GOSAT and the GEOS-Chem data. Compared to the GOSAT data, the g-b PLRS data are 0.26 ppm (0.07%) higher with a standard deviation of 1.70 ppm (0.43%). Compared to the smoothed GEOS-Chem model data, the g-b PLRS data shows a 1.31 ppm (0.33%) higher with a standard deviation of 5.30 ppm (0.87%). The g-b PLRS generally reproduced the seasonal cycle observed by GOSAT and GEOS-Chem model with correlation coefficients (r) of 0.82 and 0.64, respectively. (C) 2016 Published by Elsevier B.V.

WOS关键词SOLAR ABSORPTION-SPECTROSCOPY ; CARBON-DIOXIDE OBSERVATIONS ; ATMOSPHERIC CO2 ; RETRIEVAL ALGORITHM ; INFRARED-SPECTROSCOPY ; FTIR SPECTROMETERS ; OBSERVING NETWORK ; AVERAGED METHANE ; AIRCRAFT ; CALIBRATION
资助项目National Natural Science Foundation of China[41575021] ; National Natural Science Foundation of China[91544212] ; Anhui Province Natural Science Foundation of China[1308085MD79] ; National Natural Science Foundation of China[41530644] ; National Natural Science Foundation of China[41571130023] ; National Natural Science Foundation of China[41275038] ; National Natural Science Foundation of China[41605018] ; National Natural Science Foundation of China[41405134] ; National Key Technology R&D Program of China[2014BAC22B00] ; National Key Technology R&D Program of China[2016YFC0200800] ; National High Technology Research and Development Program of China[2014AA06A508] ; National High Technology Research and Development Program of China[2014AA06A511] ; Scientific and Technological Project of Anhui Province[1301022083] ; Special Project of Environmental Nonprofit Industry Research China[201409006]
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000413313700156
出版者ELSEVIER SCIENCE BV
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/35866]  
专题合肥物质科学研究院_中科院安徽光学精密机械研究所
通讯作者Liu, Cheng
作者单位1.Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Urban Atmospher Environm, Xiamen 361021, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Key Lab Environm Optic & Technol, Hefei 230031, Anhui, Peoples R China
4.Univ Sci & Technol China, Sch Earth & Space Sci, Hefei 230026, Anhui, Peoples R China
5.Ludwig Maximilians Univ Munchen, Meteorol Inst, Munich, Germany
推荐引用方式
GB/T 7714
Tian, Yuan,Sun, Youwen,Liu, Cheng,et al. Characterization of urban CO2 column abundance with a portable low resolution spectrometer (PLRS): Comparisons with GOSAT and GEOS-Chem model data[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2018,612(无):1593-1609.
APA Tian, Yuan.,Sun, Youwen.,Liu, Cheng.,Xie, Pinhua.,Chan, Kalok.,...&Liu, Jianguo.(2018).Characterization of urban CO2 column abundance with a portable low resolution spectrometer (PLRS): Comparisons with GOSAT and GEOS-Chem model data.SCIENCE OF THE TOTAL ENVIRONMENT,612(无),1593-1609.
MLA Tian, Yuan,et al."Characterization of urban CO2 column abundance with a portable low resolution spectrometer (PLRS): Comparisons with GOSAT and GEOS-Chem model data".SCIENCE OF THE TOTAL ENVIRONMENT 612.无(2018):1593-1609.

入库方式: OAI收割

来源:合肥物质科学研究院

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