Characterization of urban CO2 column abundance with a portable low resolution spectrometer (PLRS): Comparisons with GOSAT and GEOS-Chem model data
文献类型:期刊论文
作者 | Tian, Yuan2,3; Sun, Youwen1,3![]() ![]() ![]() ![]() |
刊名 | SCIENCE OF THE TOTAL ENVIRONMENT
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出版日期 | 2018-01-15 |
卷号 | 612期号:无页码:1593-1609 |
关键词 | Remote sensing Carbon dioxide City emission Seasonal cycle GOSAT GEOS-Chem |
ISSN号 | 0048-9697 |
DOI | 10.1016/j.scitotenv.2016.12.005 |
英文摘要 | We presented the characterization of urban CO2 column abundance (XCO2) in Hefei, China using a portable low resolution spectrometer (PLRS). An optimized correction spectrum was introduced in the spectral fitting to improve CO2 retrieval. A pronounced seasonal cycle and diurnal variation were observed with a precision of similar to 0.12%. The CO2 concentrations in winter are about 5-10 ppm higher than those in summer. Most diurnal variations exhibited downward trends. The measurement in the early morning is about 2-5 ppm higher than the late afternoon observation. The causes of the seasonal and diurnal trends were systematic analyzed. The coincident CO2 time series were compared with the Greenhouse Gases Observing SATellite (GOSAT) data and the GEOS-Chem global 3-D tropospheric chemistry model data. We found the ground based (g-b) PLRS data are systematically higher than the GOSAT and the GEOS-Chem data. Compared to the GOSAT data, the g-b PLRS data are 0.26 ppm (0.07%) higher with a standard deviation of 1.70 ppm (0.43%). Compared to the smoothed GEOS-Chem model data, the g-b PLRS data shows a 1.31 ppm (0.33%) higher with a standard deviation of 5.30 ppm (0.87%). The g-b PLRS generally reproduced the seasonal cycle observed by GOSAT and GEOS-Chem model with correlation coefficients (r) of 0.82 and 0.64, respectively. (C) 2016 Published by Elsevier B.V. |
WOS关键词 | SOLAR ABSORPTION-SPECTROSCOPY ; CARBON-DIOXIDE OBSERVATIONS ; ATMOSPHERIC CO2 ; RETRIEVAL ALGORITHM ; INFRARED-SPECTROSCOPY ; FTIR SPECTROMETERS ; OBSERVING NETWORK ; AVERAGED METHANE ; AIRCRAFT ; CALIBRATION |
资助项目 | National Natural Science Foundation of China[41575021] ; National Natural Science Foundation of China[91544212] ; Anhui Province Natural Science Foundation of China[1308085MD79] ; National Natural Science Foundation of China[41530644] ; National Natural Science Foundation of China[41571130023] ; National Natural Science Foundation of China[41275038] ; National Natural Science Foundation of China[41605018] ; National Natural Science Foundation of China[41405134] ; National Key Technology R&D Program of China[2014BAC22B00] ; National Key Technology R&D Program of China[2016YFC0200800] ; National High Technology Research and Development Program of China[2014AA06A508] ; National High Technology Research and Development Program of China[2014AA06A511] ; Scientific and Technological Project of Anhui Province[1301022083] ; Special Project of Environmental Nonprofit Industry Research China[201409006] |
WOS研究方向 | Environmental Sciences & Ecology |
语种 | 英语 |
WOS记录号 | WOS:000413313700156 |
出版者 | ELSEVIER SCIENCE BV |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/35866] ![]() |
专题 | 合肥物质科学研究院_中科院安徽光学精密机械研究所 |
通讯作者 | Liu, Cheng |
作者单位 | 1.Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Urban Atmospher Environm, Xiamen 361021, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Key Lab Environm Optic & Technol, Hefei 230031, Anhui, Peoples R China 4.Univ Sci & Technol China, Sch Earth & Space Sci, Hefei 230026, Anhui, Peoples R China 5.Ludwig Maximilians Univ Munchen, Meteorol Inst, Munich, Germany |
推荐引用方式 GB/T 7714 | Tian, Yuan,Sun, Youwen,Liu, Cheng,et al. Characterization of urban CO2 column abundance with a portable low resolution spectrometer (PLRS): Comparisons with GOSAT and GEOS-Chem model data[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2018,612(无):1593-1609. |
APA | Tian, Yuan.,Sun, Youwen.,Liu, Cheng.,Xie, Pinhua.,Chan, Kalok.,...&Liu, Jianguo.(2018).Characterization of urban CO2 column abundance with a portable low resolution spectrometer (PLRS): Comparisons with GOSAT and GEOS-Chem model data.SCIENCE OF THE TOTAL ENVIRONMENT,612(无),1593-1609. |
MLA | Tian, Yuan,et al."Characterization of urban CO2 column abundance with a portable low resolution spectrometer (PLRS): Comparisons with GOSAT and GEOS-Chem model data".SCIENCE OF THE TOTAL ENVIRONMENT 612.无(2018):1593-1609. |
入库方式: OAI收割
来源:合肥物质科学研究院
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