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Adsorption of 17 beta-estradiol from aqueous solutions by a novel hierarchically nitrogen-doped porous carbon

文献类型：期刊论文

作者Duan, Qingyun2,3; Li, Xuede2,3; Wu, Zheng2,3; Alsaedi, Ahmed4; Hayat, Tasawar4; Chen, Changlun1,4; Li, Jie2,3
刊名JOURNAL OF COLLOID AND INTERFACE SCIENCE
出版日期2019
卷号533页码:700-708
关键词17 beta-estradiol Hierarchically nitrogen-doped porous carbon Capture Water chemistry Interaction mechanisms
ISSN号0021-9797
DOI10.1016/j.jcis.2018.09.007
通讯作者Chen, Changlun(clchen@ipp.ac.cn) ; Li, Jie(lijie314@ahau.edu.cn)
英文摘要A novel interconnected hierarchically nitrogen-doped porous carbon (IHNPC) derived from metal-organic framework-based composites was obtained via a facile method and applied as a superior material for the capture of 17 beta-estradiol (E2) from aqueous solution. The adsorption kinetic and isotherm behaviors were well described by the pseudo-second-order and Langmuir models. Various thermodynamic parameters uncovered that E2 adsorption onto IHNPC was spontaneous and exothermic. Moreover, the adsorption rate of E2 by IHNPC didn't decrease with increasing water salinity in the presence of electrolyte ions and humic acids. Naturally occurring aquatic particles can enhance (i.e., Al2O3), decrease (i.e., kaolin and SiO2) or have no obvious effects (i.e., montmorillonite) on the adsorption rate of E2 by IHNPC. The high adsorption capacity and remarkable adsorption selectivity of IHNPC highlighted the application of IHNPC for the capture of E2 and provided understanding of the fate and transport of E2 in natural aquatic environments. (C) 2018 Elsevier Inc. All rights reserved.
WOS关键词METAL-ORGANIC FRAMEWORKS ; GRAPHENE OXIDE ; BISPHENOL-A ; INORGANIC NANOPARTICLES ; ESTROGEN CONTAMINANTS ; ACTIVATED-SLUDGE ; MAGNETIC BIOCHAR ; REMOVAL ; NANOTUBES ; WATER
资助项目National Natural Science Foundation of China[21806001] ; Natural Project of Anhui Provincial Department of Education[KJ2018A0126] ; Youth Science Fund of Anhui Agricultural University[2017zd03] ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000447815200072
出版者ACADEMIC PRESS INC ELSEVIER SCIENCE
资助机构National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Natural Project of Anhui Provincial Department of Education ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; Youth Science Fund of Anhui Agricultural University ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences ; CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Chinese Academy of Sciences
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/39934]  
专题合肥物质科学研究院_中科院等离子体物理研究所
通讯作者Chen, Changlun; Li, Jie
作者单位1.Chinese Acad Sci, Inst Plasma Phys, CAS Key Lab Photovolta & Energy Conservat Mat, POB 1126, Hefei 230031, Anhui, Peoples R China
2.Anhui Agr Univ, Sch Resources & Environm, Hefei 230036, Anhui, Peoples R China
3.Minist Agr, Hefei Sci Observing & Expt Stn Agroenvironm, Hefei, Anhui, Peoples R China
4.King Abdulaziz Univ, NAAM Res Grp, Jeddah 21589, Saudi Arabia
推荐引用方式
GB/T 7714		 Duan, Qingyun,Li, Xuede,Wu, Zheng,et al. Adsorption of 17 beta-estradiol from aqueous solutions by a novel hierarchically nitrogen-doped porous carbon[J]. JOURNAL OF COLLOID AND INTERFACE SCIENCE,2019,533:700-708.
APA Duan, Qingyun.,Li, Xuede.,Wu, Zheng.,Alsaedi, Ahmed.,Hayat, Tasawar.,...&Li, Jie.(2019).Adsorption of 17 beta-estradiol from aqueous solutions by a novel hierarchically nitrogen-doped porous carbon.JOURNAL OF COLLOID AND INTERFACE SCIENCE,533,700-708.
MLA Duan, Qingyun,et al."Adsorption of 17 beta-estradiol from aqueous solutions by a novel hierarchically nitrogen-doped porous carbon".JOURNAL OF COLLOID AND INTERFACE SCIENCE 533(2019):700-708.

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来源：合肥物质科学研究院

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