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  4. 中科院安徽光学精密机械研究所
Ozone seasonal evolution and photochemical production regime in the polluted troposphere in eastern China derived from high-resolution Fourier transform spectrometry (FTS) observations

文献类型：期刊论文

作者Sun, Youwen7; Liu, Cheng1,5,6,7; Palm, Mathias2; Vigouroux, Corinne3; Notholt, Justus2; Hui, Qihou7; Jones, Nicholas4; Wang, Wei7; Su, Wenjing6; Zhang, Wenqiang6
刊名ATMOSPHERIC CHEMISTRY AND PHYSICS
出版日期2018-10-11
卷号18期号:19页码:14569-14583
ISSN号1680-7316
DOI10.5194/acp-18-14569-2018
通讯作者Liu, Cheng(chliu81@ustc.edu.cn)
英文摘要The seasonal evolution of O-3 and its photochemical production regime in a polluted region of eastern China between 2014 and 2017 has been investigated using observations. We used tropospheric ozone (O-3), carbon monoxide (CO), and formaldehyde (HCHO, a marker of VOCs (volatile organic compounds)) partial columns derived from high-resolution Fourier transform spectrometry (FTS); tropospheric nitrogen dioxide (NO2, a marker of NOx (nitrogen oxides)) partial column deduced from the Ozone Monitoring Instrument (OMI); surface meteorological data; and a back trajectory cluster analysis technique. A broad O-3 maximum during both spring and summer (MAM/JJA) is observed; the day-to-day variations in MAM/JJA are generally larger than those in autumn and winter (SON/DJF). Tropospheric O-3 columns in June are 1.55 x 10(18) molecules cm(-2) (56 DU (Dobson units)), and in December they are 1.05 x 10(18) molecules cm(-2) (39 DU). Tropospheric O-3 columns in June were similar to 50 % higher than those in December. Compared with the SON/DJF season, the observed tropospheric O-3 levels in MAMMA are more influenced by the transport of air masses from densely populated and industrialized areas, and the high O-3 level and variability in MAMMA is determined by the photochemical O-3 production. The tropospheric-column HCHO/NO2 ratio is used as a proxy to investigate the photochemical O-3 production rate (PO3). The results show that the PO3 is mainly nitrogen oxide (MX) limited in MAM/JJA, while it is mainly VOC or mixed VOC-NOx-limited in SON/DJF. Statistics show that NOx-limited, mixed VOC-NOx-limited, and VOC-limited PO3 accounts for 60.1 %, 28.7 %, and 11 % of days, respectively. Considering most of PO3 is NOx limited or mixed VOC-NOx-limited, reductions in NOx would reduce O-3 pollution in eastern China.
WOS关键词MAX-DOAS OBSERVATIONS ; GROUND-BASED FTIR ; SURFACE OZONE ; PRODUCTION SENSITIVITY ; TOTAL COLUMNS ; FORMALDEHYDE ; SATELLITE ; NOX ; TEMPERATURE ; RETRIEVALS
资助项目National High Technology Research and Development Program of China[2016YFC0200800] ; National High Technology Research and Development Program of China[2018YFC0213104] ; National High Technology Research and Development Program of China[2017YFC0210002] ; National High Technology Research and Development Program of China[2016YFC0203302] ; National Science Foundation of China[41605018] ; National Science Foundation of China[41877309] ; National Science Foundation of China[41405134] ; National Science Foundation of China[41775025] ; National Science Foundation of China[41575021] ; National Science Foundation of China[51778596] ; National Science Foundation of China[91544212] ; National Science Foundation of China[41722501] ; Anhui Province Natural Science Foundation of China[1608085MD79] ; Outstanding Youth Science Foundation[41722501] ; German Federal Ministry of Education and Research (BMBF)[01LG1214A] ; Belgian Science Policy Office
WOS研究方向Meteorology & Atmospheric Sciences
语种英语
WOS记录号WOS:000447008300003
出版者COPERNICUS GESELLSCHAFT MBH
资助机构National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; National Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Anhui Province Natural Science Foundation of China ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; Outstanding Youth Science Foundation ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; German Federal Ministry of Education and Research (BMBF) ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office ; Belgian Science Policy Office
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/39360]  
专题合肥物质科学研究院_中科院安徽光学精密机械研究所
通讯作者Liu, Cheng
作者单位1.USTC, Anhui Prov Key Lab Polar Environm & Global Change, Hefei 230026, Anhui, Peoples R China
2.Univ Bremen, Inst Environm Phys, POB 330440, D-28334 Bremen, Germany
3.Royal Belgian Inst Space Aeron BIRA IASB, Brussels, Belgium
4.Univ Wollongong, Sch Chem, Northfields Ave, Wollongong, NSW 2522, Australia
5.Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China
6.Univ Sci & Technol China, Sch Earth & Space Sci, Hefei 230026, Anhui, Peoples R China
7.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Key Lab Environm Opt & Technol, Hefei 230031, Anhui, Peoples R China
推荐引用方式
GB/T 7714		 Sun, Youwen,Liu, Cheng,Palm, Mathias,et al. Ozone seasonal evolution and photochemical production regime in the polluted troposphere in eastern China derived from high-resolution Fourier transform spectrometry (FTS) observations[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(19):14569-14583.
APA Sun, Youwen.,Liu, Cheng.,Palm, Mathias.,Vigouroux, Corinne.,Notholt, Justus.,...&Liu, Jianguo.(2018).Ozone seasonal evolution and photochemical production regime in the polluted troposphere in eastern China derived from high-resolution Fourier transform spectrometry (FTS) observations.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(19),14569-14583.
MLA Sun, Youwen,et al."Ozone seasonal evolution and photochemical production regime in the polluted troposphere in eastern China derived from high-resolution Fourier transform spectrometry (FTS) observations".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.19(2018):14569-14583.

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来源：合肥物质科学研究院

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