中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Tungsten nitride/carbide nanocomposite encapsulated in nitrogen-doped carbon shell as an effective and durable catalyst for hydrogen evolution reaction

文献类型:期刊论文

作者Xu, Shihao1,2; Chu, Suyun1,2; Yang, Liang2; Chen, Yao1,2; Wang, Zhenyang1,2; Jiang, Changlong1,2
刊名NEW JOURNAL OF CHEMISTRY
出版日期2018-12-21
卷号42期号:24页码:19557-19563
ISSN号1144-0546
DOI10.1039/c8nj04663h
英文摘要

Replacement of noble-metal platinum catalysts with low-cost, durability, and highly efficient electrocatalysts holds huge potential for hydrogen evolution reaction (HER). Transition-metal carbides and nitrides have attracted much attention on account of their specific noble-metal-like d-state density electron structure. Herein, we synthesized WN-W2C nanocomposites uniformly encapsulated in nitrogen-doped (4.21 atom%) carbon shell through in situ carbonized WOX/aniline hybrid nanoparticles. The catalysts displayed remarkable performance with a low overpotential of only 242 mV at 10 mA cm(-2) and an excellent long-term durability performance i.e., 5000 cycles owing to the protection of the carbon shell. The enhanced catalytic activities arose from the synergistic effect of tungsten nitride (WN) and tungsten carbide (W2C) nanocrystals and abundant nitrogen content. The current study might inspire the design of advanced and performance-oriented metal carbide and nitride-hybrid based electrocatalysts for wider applications in hydrogen evolution reaction.

WOS关键词METAL-ORGANIC FRAMEWORKS ; OXYGEN REDUCTION ; HIGHLY EFFICIENT ; ACTIVE-SITES ; ELECTROCATALYST ; PERFORMANCE ; NANOTUBES ; ELECTRODE ; FOAM
资助项目National Basic Research Program of China[2015CB932002] ; China-Singapore Joint Project[2015DFG92510] ; National Natural Science Foundation of China[21371174] ; National Natural Science Foundation of China[21335006] ; National Natural Science Foundation of China[21275145] ; National Natural Science Foundation of China[21277145] ; National Natural Science Foundation of China[21375131] ; National Natural Science Foundation of China[21475135]
WOS研究方向Chemistry
语种英语
出版者ROYAL SOC CHEMISTRY
WOS记录号WOS:000456501100027
资助机构National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; National Basic Research Program of China ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; China-Singapore Joint Project ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/41491]  
专题合肥物质科学研究院_中科院合肥智能机械研究所
通讯作者Jiang, Changlong
作者单位1.Univ Sci & Technol China, Dept Chem, Hefei 230026, Anhui, Peoples R China
2.Chinese Acad Sci, Inst Intelligent Machines, Hefei 230031, Anhui, Peoples R China
推荐引用方式
GB/T 7714
Xu, Shihao,Chu, Suyun,Yang, Liang,et al. Tungsten nitride/carbide nanocomposite encapsulated in nitrogen-doped carbon shell as an effective and durable catalyst for hydrogen evolution reaction[J]. NEW JOURNAL OF CHEMISTRY,2018,42(24):19557-19563.
APA Xu, Shihao,Chu, Suyun,Yang, Liang,Chen, Yao,Wang, Zhenyang,&Jiang, Changlong.(2018).Tungsten nitride/carbide nanocomposite encapsulated in nitrogen-doped carbon shell as an effective and durable catalyst for hydrogen evolution reaction.NEW JOURNAL OF CHEMISTRY,42(24),19557-19563.
MLA Xu, Shihao,et al."Tungsten nitride/carbide nanocomposite encapsulated in nitrogen-doped carbon shell as an effective and durable catalyst for hydrogen evolution reaction".NEW JOURNAL OF CHEMISTRY 42.24(2018):19557-19563.

入库方式: OAI收割

来源:合肥物质科学研究院

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