Easy-separative MoS2-glue sponges with high-efficient dye adsorption and excellent reusability for convenient water treatment
文献类型：期刊论文
| 作者 | Fang, Yueyun3,4; Huang, Qizhang3,4; Liu, Pengyi1; Shi, Jifu1 ; Xu, Gang2,3
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| 刊名 | COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
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| 出版日期 | 2018-03-05 |
| 卷号 | 540页码:11 |
| ISSN号 | 0927-7757 |
| 关键词 | MoS2-glue sponges Easy-separative Dye adsorption Rhodamine B Reusability |
| DOI | 10.1016/j.colsurfa.2018.01.001 |
| 通讯作者 | Shi, Jifu(shijf@ms.giec.ac.cn) ; Xu, Gang(xugang@ms.giec.ac.cn) |
| 英文摘要 | This study demonstrated high-efficient dye adsorption for wastewater using MoS2-glue sponge as an easy-separative and regenerative adsorbent. Flower-like molybdenum disulfide (MoS2) nanopowders with rich polar edge sites were firstly synthesized by a facile one-pot hydrothermal method. Chemical and morphological features of MoS2 nanoflowers were then examined by XRD, XPS, SEM and TEM. Afterwards, different concentrations of the MoS2-glue sponges with easy separability were successfully fabricated by a convenient two-step dipcoating method. The adsorption performance was estimated by the removal of Rhodamine B (RhB) dyes. The results proved that the maximum adsorption capacity of MoS2-glue sponge was 127.39 mg RhB/g product in 60 min. The RhB uptake behaviors can be well described by the Sips isotherm model and pseudo-second-order kinetic model, indicating a multilayer and chemical adsorption process. The adsorption mechanism proposed that the zwitterionic RhB molecules in aqueous solution would aggregate on the surface of negative charged MoS2 in a head-to-tail way through electrostatic interaction. Furthermore, RhB dyes could desorb easily from MoS2-glue sponges when changing the polarity of solvent and the reusability experiment showed that the MoS2-3% glue sponge could be reused for 15 times with above 85.8% of the adsorption capacity retained. Thus, the novel MoS2-glue sponge is considered as a competitive adsorbent for treatment of dyestuff waste water. |
| WOS关键词 | LAYERED DOUBLE HYDROXIDE ; DISULFIDE MOS2 NANOSHEETS ; WASTE-WATER ; MOLYBDENUM-DISULFIDE ; ORGANIC-DYES ; RHODAMINE-B ; METHYL-ORANGE ; ANIONIC DYES ; REMOVAL ; NANOCOMPOSITES |
| 资助项目 | National Natural Science Foundation of China[21673243] ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China[2014B050505015] ; Special Support Program of Guangdong Province, China[2014TQ01N610] ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences[KFJ-STS-QYZD-010] ; Tibet Autonomous Region Major Special Projects[ZD20170017] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| 出版者 | ELSEVIER SCIENCE BV |
| WOS记录号 | WOS:000424954100014 |
| 资助机构 | National Natural Science Foundation of China ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China ; Special Support Program of Guangdong Province, China ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences ; Tibet Autonomous Region Major Special Projects |
| 源URL | [http://ir.giec.ac.cn/handle/344007/23365]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Shi, Jifu; Xu, Gang |
| 作者单位 | 1.Jinan Univ, Dept Phys, Siyuan Lab, Guangzhou 510632, Guangdong, Peoples R China 2.Tibet New Energy Res & Demonstrat Ctr, Lhasa 85000, Tibet, Peoples R China 3.Chinese Acad Sci, Guangdong Prov Key Lab New & Renewable Energy Res, Key Lab Renewable Energy, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Fang, Yueyun,Huang, Qizhang,Liu, Pengyi,et al. Easy-separative MoS2-glue sponges with high-efficient dye adsorption and excellent reusability for convenient water treatment[J]. COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS,2018,540:11. |
| APA | Fang, Yueyun,Huang, Qizhang,Liu, Pengyi,Shi, Jifu,&Xu, Gang.(2018).Easy-separative MoS2-glue sponges with high-efficient dye adsorption and excellent reusability for convenient water treatment.COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS,540,11. |
| MLA | Fang, Yueyun,et al."Easy-separative MoS2-glue sponges with high-efficient dye adsorption and excellent reusability for convenient water treatment".COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS 540(2018):11. |
入库方式： OAI收割
来源：广州能源研究所
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