Partial Oxidation of Filter Cake Particles from Biomass Gasification Process in the Simulated Product Gas Environment
文献类型：期刊论文
| 作者 | Jiang, Jun-fei2; Lang, Lin2 ; Lin, Le-teng1; Liu, Hua-cai2; Yin, Xiu-li2; Wu, Chuang-zhi2
|
| 刊名 | ENERGY & FUELS
 |
| 出版日期 | 2018-02-01 |
| 卷号 | 32期号:2页码:1703-1710 |
| ISSN号 | 0887-0624 |
| DOI | 10.1021/acs.energyfuels.7b01100 |
| 通讯作者 | Lang, Lin(langlin@ms.giec.ac.cn) |
| 英文摘要 | Filtration failure occurs when filter media are blocked by accumulated solid particles. Suitable operating conditions were investigated for cake cleaning by partial oxidation of filter-cake particles (FCPs) during biomass gasification. The mechanism of the FCP partial oxidation was investigated in a ceramic filter and by using thermogravimetric analysis through a temperature-programmed route in a 2 vol % O-2-N-2 environment. Partial oxidation of the FCPs in the simulated product gas environment was examined at 300-600 degrees C in a ceramic filter that was set and heated in a laboratory-scale fixed reactor. Four reaction stages, namely, drying, preoxidation, complex oxidation, and nonoxidation, occurred in the FCP partial oxidation when the temperature increased from 30 to 800 degrees C in a 2 vol % O-2-N-2 environment. Partial oxidation was more effective for FCP mass loss from 275 to 725 degrees C. Experimental results obtained in a ceramic filter indicated that the best operating temperature and FCP loading occurred at 400 degrees C and 1.59 g/cm(2), respectively. The FCPs were characterized before and after partial oxidation by Fourier-transform infrared spectroscopy, scanning electron microscopy, and Brunaeur Emmett Teller analysis. Fourier transform infrared spectroscopy analysis revealed that partial oxidation of the FCPs can result in a significant decrease in C Fin (alkyl and aromatic) groups and an increase in C=O (carboxylic acids) groups. The scanning electron microscopy and Brunaeur Emmett Teller analyses suggest that, during partial oxidation, the FCPs underwent pore or pit formation, expansion, amalgamation, and destruction. |
| WOS关键词 | HIGH-TEMPERATURE ; FILTRATION ; CORROSION ; CANDLES ; SYNGAS ; AIR |
| 资助项目 | National Natural Science Foundation of China[51676192] ; National Natural Science Foundation of China[51661145022] ; Science and Technology Program of Guangzhou[201707010237] |
| WOS研究方向 | Energy & Fuels ; Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000426015000073 |
| 出版者 | AMER CHEMICAL SOC |
| 资助机构 | National Natural Science Foundation of China ; Science and Technology Program of Guangzhou |
| 源URL | [http://ir.giec.ac.cn/handle/344007/23480]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Lang, Lin |
| 作者单位 | 1.Linnaeus Univ, Built Environm & Energy Technol, Vaxjo, Sweden 2.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Guangdong, Peoples R China |
| 推荐引用方式 GB/T 7714 | Jiang, Jun-fei,Lang, Lin,Lin, Le-teng,et al. Partial Oxidation of Filter Cake Particles from Biomass Gasification Process in the Simulated Product Gas Environment[J]. ENERGY & FUELS,2018,32(2):1703-1710. |
| APA | Jiang, Jun-fei,Lang, Lin,Lin, Le-teng,Liu, Hua-cai,Yin, Xiu-li,&Wu, Chuang-zhi.(2018).Partial Oxidation of Filter Cake Particles from Biomass Gasification Process in the Simulated Product Gas Environment.ENERGY & FUELS,32(2),1703-1710. |
| MLA | Jiang, Jun-fei,et al."Partial Oxidation of Filter Cake Particles from Biomass Gasification Process in the Simulated Product Gas Environment".ENERGY & FUELS 32.2(2018):1703-1710. |
入库方式： OAI收割
来源：广州能源研究所
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