Magnetically Recyclable MoS2/Fe3O4 Hybrid Composite as Visible Light Responsive Photocatalyst with Enhanced Photocatalytic Performance
文献类型：期刊论文
| 作者 | Lin, Xiaozi1,3; Wang, Xi3; Zhou, Qingwei4,5; Wen, Chengyan6; Su, Shaoqiang1; Xiang, Jie1; Cheng, Pengfei1; Hu, Xianbiao1; Li, Ye1; Wang, Xin2 |
| 刊名 | ACS SUSTAINABLE CHEMISTRY & ENGINEERING
 |
| 出版日期 | 2019-01-07 |
| 卷号 | 7期号:1页码:1673-1682 |
| ISSN号 | 2168-0485 |
| 关键词 | Fe3O4 NPs MoS2 photocatalyst magnetical recyclability visible light responsive |
| DOI | 10.1021/acssuschemeng.8b05440 |
| 通讯作者 | Zhang, Zhang(zzhang@scnu.edu.cn) |
| 英文摘要 | Photocatalysis is one of the most promising technologies in wastewater treatment. However, the inactivity to visible light and the inconvenience to recycle severely limit its practical application. In this work, via a facile hydrothermal method, Fe3O4 NPs were integrated onto the surfaces of 3D ball-flower-like MoS2 microspheres as efficiently visible light responsive and magnetically recyclable photocatalysts. Experimental results indicate that, an optimal loading amount (20 wt %) of Fe3O4 NPs can not only effectively enhance the photocatalytic ability of the MoS2/Fe3O4 (MF) hybrid composite with approximately 2 times better than pure MoS2, but also make it conveniently recycle from water by an external magnetic field. The photoelectrochemical studies also reveal that the incorporation of Fe3O4 NPs can effectively enhance the charge transfer rate and accelerate separation of photoinduced charge carriers. The surface catalytic mechanism of MF hybrid composite was also explored through XPS spectra. With both the excellent photocatalytic performance and magnetical recyclability, the 20 wt %-MF hybrid composite is considered to be a promising and competitive photocatalyst for wastewater treatment utilizing solar energy. |
| WOS关键词 | HYDROTHERMAL SYNTHESIS ; TIO2 NANOPARTICLES ; FACILE SYNTHESIS ; MOS2 NANOSHEETS ; DEGRADATION ; GRAPHENE ; HETEROJUNCTION ; FABRICATION ; MECHANISM ; EVOLUTION |
| 资助项目 | National Key R&D Program of China[2016YFB0401501] ; Program for Chang Jiang Scholars and Innovative Research Teams in Universities[IRT_17R40] ; Cultivation project of National Engineering Technology Center[2017B090903008] ; Xijiang RD Team ; Guangdong National Science Foundation[2018A030313377] |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Engineering |
| 语种 | 英语 |
| 出版者 | AMER CHEMICAL SOC |
| WOS记录号 | WOS:000455288800177 |
| 资助机构 | National Key R&D Program of China ; Program for Chang Jiang Scholars and Innovative Research Teams in Universities ; Cultivation project of National Engineering Technology Center ; Xijiang RD Team ; Guangdong National Science Foundation |
| 源URL | [http://ir.giec.ac.cn/handle/344007/24548]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Zhang, Zhang |
| 作者单位 | 1.South China Normal Univ, South China Acad Adv Optoelect, Inst Adv Mat, Guangzhou 510006, Guangdong, Peoples R China 2.South China Normal Univ, South China Acad Adv Optoelect, Natl Ctr Int Res Green Optoelect, Guangzhou 510006, Guangdong, Peoples R China 3.South China Normal Univ, Guangdong Prov Key Lab Funct Mat Environm Protect, Guangdong Prov Engn Res Ctr Drinking Water Safety, Sch Chem & Environm, Guangzhou 510006, Guangdong, Peoples R China 4.Nanjing Univ, Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China 5.Nanjing Univ, Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China 6.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lin, Xiaozi,Wang, Xi,Zhou, Qingwei,et al. Magnetically Recyclable MoS2/Fe3O4 Hybrid Composite as Visible Light Responsive Photocatalyst with Enhanced Photocatalytic Performance[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2019,7(1):1673-1682. |
| APA | Lin, Xiaozi.,Wang, Xi.,Zhou, Qingwei.,Wen, Chengyan.,Su, Shaoqiang.,...&Liu, Junming.(2019).Magnetically Recyclable MoS2/Fe3O4 Hybrid Composite as Visible Light Responsive Photocatalyst with Enhanced Photocatalytic Performance.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,7(1),1673-1682. |
| MLA | Lin, Xiaozi,et al."Magnetically Recyclable MoS2/Fe3O4 Hybrid Composite as Visible Light Responsive Photocatalyst with Enhanced Photocatalytic Performance".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 7.1(2019):1673-1682. |
入库方式： OAI收割
来源：广州能源研究所
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