Catalyst deactivation and regeneration during CO2 reforming of bio-oil
文献类型：期刊论文
| 作者 | Xu Qingli1; Feng Peng1; Qi Wei2 ; Huang Kai3; Xin Shanzhi4; Yan Yongjie1
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| 刊名 | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
 |
| 出版日期 | 2019-04-23 |
| 卷号 | 44期号:21页码:10277-10285 |
| 关键词 | CO2 reforming Bio-oil Hydrogen Deactivation Regeneration |
| ISSN号 | 0360-3199 |
| DOI | 10.1016/j.ijhydene.2019.02.156 |
| 通讯作者 | Xu Qingli(xuqingli@ecust.edu.cn) ; Qi Wei(qiwei@ms.giec.ac.cn) |
| 英文摘要 | Catalyst deactivation and regeneration during CO2 reforming of bio-oil were researched in this paper. The results of XRD, TG and SEM analyses showed that the catalyst deactivation was a combination of carbon deposition and sintering. There were amorphous carbon and filamentous carbon on the catalyst surface, but amorphous carbon was the main carbon product, which was the main reason for the catalyst deactivation. The activity and stability of steam regeneration catalyst is superior to that of CO2 and air regeneration catalyst, but steam regeneration process will consume much quantity of steam, which can be increased production cost. Air regeneration method is easy to sinter the center of catalyst. CO2 regeneration process not only produces useful gases (C + CO2 = 2CO), but also makes good use of greenhouse gases, which has an industrial application prospect. However, with the cycle of catalyst increasing, the activity and stability catalyst will decrease gradually during the CO2 reforming process. (C) 2019 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved. |
| WOS关键词 | MODEL COMPOUNDS ; FAST-PYROLYSIS ; HYDROGEN-PRODUCTION ; NI/LA2O3-ALPHA-AL2O3 CATALYST ; OPERATING-CONDITIONS ; STEAM GASIFICATION ; ACETIC-ACID ; ETHANOL ; NI ; BIOMASS |
| 资助项目 | National Natural Science Foundation of China[51676193] ; National Natural Science Foundation of China[21376084] ; Hubei Science and Technology Department Project[2017CFB370] |
| WOS研究方向 | Chemistry ; Electrochemistry ; Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:000466618300013 |
| 出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
| 资助机构 | National Natural Science Foundation of China ; Hubei Science and Technology Department Project |
| 源URL | [http://ir.giec.ac.cn/handle/344007/24939]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Xu Qingli; Qi Wei |
| 作者单位 | 1.East China Univ Sci & Technol, Key Lab Coal Gasificat & Energy Chem Engn, Minist Educ, Res Ctr Biomass Energy, Shanghai, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou, Guangdong, Peoples R China 3.Guangxi Acad Sci, Natl Engn Res Ctr Nonfood Biorefinery, Guangxi Key Lab Biorefinery, Nanning, Peoples R China 4.Jianghan Univ, Hubei Key Lab Ind Fume & Dust Pollut Control, Wuhan, Hubei, Peoples R China |
| 推荐引用方式 GB/T 7714 | Xu Qingli,Feng Peng,Qi Wei,et al. Catalyst deactivation and regeneration during CO2 reforming of bio-oil[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2019,44(21):10277-10285. |
| APA | Xu Qingli,Feng Peng,Qi Wei,Huang Kai,Xin Shanzhi,&Yan Yongjie.(2019).Catalyst deactivation and regeneration during CO2 reforming of bio-oil.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,44(21),10277-10285. |
| MLA | Xu Qingli,et al."Catalyst deactivation and regeneration during CO2 reforming of bio-oil".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 44.21(2019):10277-10285. |
入库方式： OAI收割
来源：广州能源研究所
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