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Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method

文献类型：期刊论文

作者Mei, Qun1,2; Wei, Xiangqian2; Sun, Weitao2; Zhang, Xinghua1; Li, Wenzhi2; Ma, Longlong1
刊名RSC ADVANCES
出版日期2019
卷号9期号:23页码:12846-12853
ISSN号2046-2069
DOI10.1039/c9ra02090j
通讯作者Li, Wenzhi(liwenzhi@ustc.edu.cn) ; Ma, Longlong(mall@ms.giec.ac.cn)
英文摘要Conversion of cellulose to 5-hydroxymethylfurfural (HMF) is an important means of biomass utilization. However, simulation of hydrolysis of cellulose and species transport in multiphase systems is still missing. In this paper, a multiphase lattice Boltzmann method of the Shan-Chen model has been applied for simulating the complex chemical reactions and interphase mass transfer in a liquid membrane catalytic reactor. For the sake of simplification, a single particle liquid membrane catalytic model is developed to simulate the hydrolysis of cellulose into HMF and its side reactions, which include the adsorption of cellulose particles on the liquid membrane, the complex chemical reactions inside the liquid membrane and the interphase transfer of HMF. This simulation presents the results of hydrolysis of cellulose and the HMF transport process. Additionally, the results show that the thinner liquid membrane thickness is beneficial for increasing the yield of HMF.
WOS关键词BIOMASS FAST PYROLYSIS ; MASS-TRANSFER ; SIMULATION ; DEHYDRATION ; CONVERSION ; FRUCTOSE ; ZEOLITE ; FLOW
资助项目National Natural Science Foundation of China[51576198] ; National Natural Science Foundation of China[51536009] ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences[XDA21060102]
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000468636000008
出版者ROYAL SOC CHEMISTRY
资助机构National Natural Science Foundation of China ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences
源URL[http://ir.giec.ac.cn/handle/344007/24978]  
专题中国科学院广州能源研究所
通讯作者Li, Wenzhi; Ma, Longlong
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
2.Univ Sci & Technol China, Dept Thermal Sci & Energy Engn, Lab Basic Res Biomass Convers & Utilizat, Hefei 230026, Anhui, Peoples R China
推荐引用方式
GB/T 7714		 Mei, Qun,Wei, Xiangqian,Sun, Weitao,et al. Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method[J]. RSC ADVANCES,2019,9(23):12846-12853.
APA Mei, Qun,Wei, Xiangqian,Sun, Weitao,Zhang, Xinghua,Li, Wenzhi,&Ma, Longlong.(2019).Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method.RSC ADVANCES,9(23),12846-12853.
MLA Mei, Qun,et al."Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method".RSC ADVANCES 9.23(2019):12846-12853.

入库方式： OAI收割

来源：广州能源研究所

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