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Selective Conversion of Cellulose to Hydroxyacetone and 1-Hydroxy-2-Butanone with Sn-Ni Bimetallic Catalysts

文献类型：期刊论文

作者Wang, Haiyong1,2,3,4; Zhu, Changhui1,2,3,4; Liu, Qiying1,2,3,5; Tan, Jin1,2,3; Wang, Chenguang1,2,3; Liang, Zheng1,2,3; Ma, Longlong1,2,3
刊名CHEMSUSCHEM
出版日期2019-05-21
卷号12期号:10页码:2154-2160
关键词biomass cellulose hydroxyacetone intermetallic keto-alcohols
ISSN号1864-5631
DOI10.1002/cssc.201900172
通讯作者Liu, Qiying(liuqy@ms.giec.ac.cn) ; Ma, Longlong(mall@ms.giec.ac.cn)
英文摘要The high-value-added chemicals hydroxyacetone (HA) and 1-hydroxy-2-butanone (HB) were produced from agricultural waste over a Ni3Sn4-SnOx catalyst. The Sn-Ni intermetallic compound and SnOx acted as the active sites for HA and HB production by selectively cleaving the target C-C and C-O bonds. Approximately 70% of the total HA and HB yield was obtained by selective hydrogenolysis of cellulose. This strategy expands the application of cellulose towards renewable production of high-value C-3 and C-4 keto-alcohols from cellulosic biomass.
WOS关键词ETHYLENE-GLYCOL ; PLATFORM MOLECULES ; AEROBIC OXIDATION ; BIOMASS ; CHEMICALS ; GLYCEROL ; POLYOLS ; HYDROGENOLYSIS ; EFFICIENT ; SORBITOL
资助项目National Natural Science Foundation of China[51576199] ; National Natural Science Foundation of China[51536009] ; DNL Cooperation Fund, CAS[DNL180302] ; Natural Science Foundation of Guangdong Province[2017A030308010] ; Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program[2017BT01N092]
WOS研究方向Chemistry ; Science & Technology - Other Topics
语种英语
WOS记录号WOS:000472806800008
出版者WILEY-V C H VERLAG GMBH
资助机构National Natural Science Foundation of China ; DNL Cooperation Fund, CAS ; Natural Science Foundation of Guangdong Province ; Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program
源URL[http://ir.giec.ac.cn/handle/344007/25263]  
专题中国科学院广州能源研究所
通讯作者Liu, Qiying; Ma, Longlong
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
3.Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Guangdong, Peoples R China
4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
5.Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714		 Wang, Haiyong,Zhu, Changhui,Liu, Qiying,et al. Selective Conversion of Cellulose to Hydroxyacetone and 1-Hydroxy-2-Butanone with Sn-Ni Bimetallic Catalysts[J]. CHEMSUSCHEM,2019,12(10):2154-2160.
APA Wang, Haiyong.,Zhu, Changhui.,Liu, Qiying.,Tan, Jin.,Wang, Chenguang.,...&Ma, Longlong.(2019).Selective Conversion of Cellulose to Hydroxyacetone and 1-Hydroxy-2-Butanone with Sn-Ni Bimetallic Catalysts.CHEMSUSCHEM,12(10),2154-2160.
MLA Wang, Haiyong,et al."Selective Conversion of Cellulose to Hydroxyacetone and 1-Hydroxy-2-Butanone with Sn-Ni Bimetallic Catalysts".CHEMSUSCHEM 12.10(2019):2154-2160.

入库方式： OAI收割

来源：广州能源研究所

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