Fe2O3 modification promotes the photocatalytic performance of TiO2 nanotube confined Pd nanoparticles
文献类型:期刊论文
作者 | Peng, Quanming2,3; Peng, Guiming1; Wu, Liangpeng2![]() ![]() ![]() |
刊名 | JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY
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出版日期 | 2019-07-01 |
卷号 | 380页码:7 |
关键词 | Photocatalytic degradation TiO2 nanotube Confined Pd Fe2O3 Confinement effect |
ISSN号 | 1010-6030 |
DOI | 10.1016/j.jphotochem.2019.111865 |
通讯作者 | Li, Xinjun(lixj@ms.giec.ac.cn) |
英文摘要 | It is revealed that TiO2 nanotube confined Pd nanoparticles (Pd-in-TiO2NT) processed better photocatalytic degradation activity than Pd nanoparticles loaded on outer wall of TiO2 nanotube (Pd-out-TiO2NT). Moreover, by anchoring Fe2O3 nanoparticles on Pd-in-TiO2NT (Pd-in/Fe2O3-TiO2NT), the photocatalytic activity is dramatically improved as evidenced by the accelerated photocatalytic degradation of methyl orange. As measured by photoluminescence and electrochemical impedance spectroscopy, the separation efficiency of photogenerated electron-hole pairs is significantly improved when the outside surface of TiO2NT was modified by Fe2O3. X-ray photoelectron spectroscopy informs that the Fe2O3 modification can efficiently modulate the electron density distribution of the TiO2 nanotube, thus improves the catalytic oxidation of Pd in Pd-in/Fe2O3-TiO2NT. This work provides a novel method to construct high active catalysts for environmental prevention by the modulation of electronic state on TiO2 nanotube confinement effect. |
WOS关键词 | CATALYTIC COMBUSTION ; CARBON NANOTUBES ; IRON ; HYDRODECHLORINATION |
资助项目 | Science and Technology Program of Guangzhou, China[201803030019] ; Science and Technology Plan Project of Guangdong Province[2017A050501044] ; National Natural Science Foundation of China[51802305] ; National Natural Science Foundation of China[51802043] ; Analytical & Testing Center, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, China |
WOS研究方向 | Chemistry |
语种 | 英语 |
WOS记录号 | WOS:000474320400013 |
出版者 | ELSEVIER SCIENCE SA |
资助机构 | Science and Technology Program of Guangzhou, China ; Science and Technology Plan Project of Guangdong Province ; National Natural Science Foundation of China ; Analytical & Testing Center, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, China |
源URL | [http://ir.giec.ac.cn/handle/344007/25284] ![]() |
专题 | 中国科学院广州能源研究所 |
通讯作者 | Li, Xinjun |
作者单位 | 1.Guangdong Univ Technol, Sch Mat & Energy, Guangzhou 510006, Guangdong, Peoples R China 2.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China 3.Univ Chinese Acad Sci, Coll Mat Sci & Optoelect Technol, Beijing 100049, Peoples R China 4.Guangzhou Nanfeng Environm Technol Co Ltd, Guangzhou 510335, Guangdong, Peoples R China |
推荐引用方式 GB/T 7714 | Peng, Quanming,Peng, Guiming,Wu, Liangpeng,et al. Fe2O3 modification promotes the photocatalytic performance of TiO2 nanotube confined Pd nanoparticles[J]. JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY,2019,380:7. |
APA | Peng, Quanming.,Peng, Guiming.,Wu, Liangpeng.,Li, Juan.,Wang, Xiaoyang.,...&Li, Xinjun.(2019).Fe2O3 modification promotes the photocatalytic performance of TiO2 nanotube confined Pd nanoparticles.JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY,380,7. |
MLA | Peng, Quanming,et al."Fe2O3 modification promotes the photocatalytic performance of TiO2 nanotube confined Pd nanoparticles".JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY 380(2019):7. |
入库方式: OAI收割
来源:广州能源研究所
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