Pyrolytic conversion of biowaste-derived hydrochar: Decomposition mechanism of specific components
文献类型：期刊论文
| 作者 | Zhuang, Xiuzheng1,4; Song, Yanpei1,4; Zhan, Hao2,3; Bi, Xiaotao T.5,6; Yin, Xiuli1 ; Wu, Chuangzhi1,4
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| 刊名 | FUEL
 |
| 出版日期 | 2020-04-15 |
| 卷号 | 266页码:13 |
| ISSN号 | 0016-2361 |
| 关键词 | Industrial biowaste Hydrothermal carbonization Pyrolysis behavior Multi-parallel kinetic model Gaseous component |
| DOI | 10.1016/j.fuel.2020.117106 |
| 通讯作者 | Yin, Xiuli(xlyin@ms.giec.ac.cn) |
| 英文摘要 | Hydrothermal carbonization (HTC) coupled with subsequent downstream conversion is a new concept for the utilization of industrial biowastes for energy production. In this work, three representative biowastes (i.e., lignocellulosic, non-lignocellulosic and ash-rich samples) were selected for HTC pretreatment, and the subsequent pyrolysis of the derived hydrochars was evaluated using multiple kinetic models and combined instrumental analyses. Results showed that the thermal weight loss peak for each biowaste was progressively shifted to a higher temperature after HTC pretreatment, while the maximum value of weight loss was reduced compared to that of the original feedstock. This change was shown to be caused by the shift in biowaste compositions to a more stable one in the hydrothermal stage, but the dissimilarity of evolution pathways among specific components affected the rate and degree of pyrolysis of the hydrochars to different extent. In addition, fewer volatile compounds were released during the pyrolysis of the hydrochars, and the composition of pyrolytic volatiles was found to be mainly dependent on the types of biowaste and HTC conditions. These findings not only provide essential information on the pyrolytic capability of HTC-derived hydrochars, but can also help in designing, optimizing and scaling up the thermochemical conversion of industrial biowastes. |
| WOS关键词 | HYDROTHERMAL CARBONIZATION HTC ; SEWAGE-SLUDGE ; TG-FTIR ; GASIFICATION CHARACTERISTICS ; INDUSTRIAL BIOWASTES ; SOLID-FUEL ; KINETICS ; COMBUSTION ; BEHAVIOR ; BIOMASS |
| 资助项目 | National Natural Science Foundation of China[51676195] ; Science and Technology Program of Guangdong Province[2018A050506068] ; Science and Technology Program of Guangzhou[201803030006] ; Shanghai Tongji Gao Tingyao Environmental Science & Technology Development Foundation |
| WOS研究方向 | Energy & Fuels ; Engineering |
| 语种 | 英语 |
| 出版者 | ELSEVIER SCI LTD |
| WOS记录号 | WOS:000510603500075 |
| 资助机构 | National Natural Science Foundation of China ; Science and Technology Program of Guangdong Province ; Science and Technology Program of Guangzhou ; Shanghai Tongji Gao Tingyao Environmental Science & Technology Development Foundation |
| 源URL | [http://ir.giec.ac.cn/handle/344007/26513]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Yin, Xiuli |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangdong Key Lab New & Renewable Energy Res & De, Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China 3.Chinese Acad Sci, Guangzhou Inst Geochem, Guangdong Key Lab Environm Protect & Resources Ut, Guangzhou 510640, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 5.Univ British Columbia, Clean Energy Res Ctr, Vancouver, BC V6T 1Z3, Canada 6.Univ British Columbia, Dept Chem & Biol Engn, Vancouver, BC V6T 1Z3, Canada |
| 推荐引用方式 GB/T 7714 | Zhuang, Xiuzheng,Song, Yanpei,Zhan, Hao,et al. Pyrolytic conversion of biowaste-derived hydrochar: Decomposition mechanism of specific components[J]. FUEL,2020,266:13. |
| APA | Zhuang, Xiuzheng,Song, Yanpei,Zhan, Hao,Bi, Xiaotao T.,Yin, Xiuli,&Wu, Chuangzhi.(2020).Pyrolytic conversion of biowaste-derived hydrochar: Decomposition mechanism of specific components.FUEL,266,13. |
| MLA | Zhuang, Xiuzheng,et al."Pyrolytic conversion of biowaste-derived hydrochar: Decomposition mechanism of specific components".FUEL 266(2020):13. |
入库方式： OAI收割
来源：广州能源研究所
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