The Effect of CO2 Partial Pressure on CH4 Recovery in CH4-CO2 Swap with Simulated IGCC Syngas
文献类型：期刊论文
| 作者 | Ding, Ya-Long4,5; Wang, Hua-Qin4; Xu, Chun-Gang1,2,3,5; Li, Xiao-Sen1,2,3,5
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| 刊名 | ENERGIES
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| 出版日期 | 2020-03-01 |
| 卷号 | 13期号:5页码:11 |
| 关键词 | CH4 hydrate replacement IGCC syngas in-situ Raman |
| DOI | 10.3390/en13051017 |
| 通讯作者 | Li, Xiao-Sen(lixs@ms.giec.ac.cn) |
| 英文摘要 | To investigate the influence of CO2 partial pressure on efficiency of CH4-CO2 swap from natural gas hydrates (NGHs), the replacement of CH4 from natural gas hydrate (NGH) is carried out with simulated Integrated Gasification Combined Cycle (IGCC) syngas under different pressures, and the gas chromatography (GC), in-situ Raman, and powder X-ray diffraction (PXRD) are employed to analyze the hydrate compositions and hydrate structures. The results show that with the P-T (pressure and temperature) condition shifting from that above the hydrate equilibrium curve of IGCC syngas to that below the hydrate equilibrium curve of IGCC syngas, the rate of CH4 recovery drastically rises from 32% to 71%. The presence of water can be clearly observed when P-T condition is above the hydrate equilibrium curve of IGCC syngas; however the presence of water only occurs at the interface between gas phase and hydrate phase. No H-2 is found to present in the final hydrate phase at the end of process of CH4-CO2 swap with IGCC syngas. |
| WOS关键词 | CARBON-DIOXIDE ; METHANE HYDRATE ; PHASE-EQUILIBRIA ; GAS HYDRATE ; ENERGY ; EXPLOITATION ; REPLACEMENT ; CONVERSION |
| 资助项目 | National Natural Science Fund of Guangdong Province, China[2019A1515011490] ; Key Program of National Natural Science Foundation of China[51736009] ; Special project for marine economy development of Guangdong Province[GDME-2018D002] ; Key Research Program of Frontier Sciences, CAS[ZDBS-LY-SLH041] ; CAS Science and Technology Apparatus Development Program[YZ201619] ; Frontier Sciences Key Research Program of the Chinese Academy of Sciences[QYZDJ-SSW-JSC033] |
| WOS研究方向 | Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:000524318700004 |
| 出版者 | MDPI |
| 资助机构 | National Natural Science Fund of Guangdong Province, China ; Key Program of National Natural Science Foundation of China ; Special project for marine economy development of Guangdong Province ; Key Research Program of Frontier Sciences, CAS ; CAS Science and Technology Apparatus Development Program ; Frontier Sciences Key Research Program of the Chinese Academy of Sciences |
| 源URL | [http://ir.giec.ac.cn/handle/344007/27031]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Li, Xiao-Sen |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou 510640, Peoples R China 2.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 3.CAS Key Lab Gas Hydrate, Guangzhou 510640, Peoples R China 4.Huanghuai Univ, Coll Chem & Pharmaceut Engn, Zhumadian 463000, Peoples R China 5.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510641, Guangdong, Peoples R China |
| 推荐引用方式 GB/T 7714 | Ding, Ya-Long,Wang, Hua-Qin,Xu, Chun-Gang,et al. The Effect of CO2 Partial Pressure on CH4 Recovery in CH4-CO2 Swap with Simulated IGCC Syngas[J]. ENERGIES,2020,13(5):11. |
| APA | Ding, Ya-Long,Wang, Hua-Qin,Xu, Chun-Gang,&Li, Xiao-Sen.(2020).The Effect of CO2 Partial Pressure on CH4 Recovery in CH4-CO2 Swap with Simulated IGCC Syngas.ENERGIES,13(5),11. |
| MLA | Ding, Ya-Long,et al."The Effect of CO2 Partial Pressure on CH4 Recovery in CH4-CO2 Swap with Simulated IGCC Syngas".ENERGIES 13.5(2020):11. |
入库方式： OAI收割
来源：广州能源研究所
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