中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Effects of the joint application of phosphate rock, ferric nitrate and plant ash on the immobility of As, Pb and Cd in soils

文献类型:期刊论文

作者Li, Qiqi4; Zhong, Huiqiong3; Cao, Yan1,2,3,4
刊名JOURNAL OF ENVIRONMENTAL MANAGEMENT
出版日期2020-07-01
卷号265页码:7
关键词Multi-metal(loid)s contaminations Immobility Phosphate rock Ferric nitrate Grass ash SAR leaching
ISSN号0301-4797
DOI10.1016/j.jenvman.2020.110576
通讯作者Cao, Yan(caoyan@ms.giec.ac.cn)
英文摘要Phosphate rock (PR) and ferric salts have been frequently used to immobilize heavy metal(loid)s in soils, but in varied efficiencies referring to different metal(loid) pollutants. This study explored the effective application of plant ash (PA) to the previous formula of phosphate rock (PR) and ferric salts (Fe(NO3)(3)) (PR + Fe3++PA), compared to only PR, on the bioavailability and immobility of multi-metal(loid)s of selected arsenic (As), lead (Pb) and cadmium (Cd) in soils. Results from NaHCO3-extraction and toxicity characteristic leaching procedure (TCLP) implied the increase of the As mobility in soils by 7.0% and 2.6% using PR only, but the significant reduction of the As mobility by 24.2% and 82.4% jointly using PR + Fe3++PA. Meanwhile, the application of either PR alone or PR + Fe3++PA in soil significantly decreased Pb and Cd extracting in diethylene triamine pentacetate acid (DTPA) and TCLP, particularly, the immobilization effect of PR + Fe3+ +PA was better than that of PR. The leaching column test further confirmed the high durability of PR + Fe3++PA on the immobilization of As and Pb under the continuous acid exposure, but likely slightly increased the mobility of Cd (the accumulated concentration of Cd, 5.88 mu g/L) compared to that (3.16 mu g/L) in the untreated column (UN-column), which were both much lower than the level V (100 mu g/L) of the Chinese National Quality Standard for Surface Water (GB 3838-2002). Therefore, PR + Fe3++PA exhibited the significant enhancement on the immobilization of As, Pb and Cd under simulated acid rain (SAR) leaching.
WOS关键词CONTAMINATED SOILS ; ARSENIC UPTAKE ; CADMIUM ; ADSORPTION ; MOBILITY ; METALS ; LEAD ; CU ; HYPERACCUMULATOR ; STABILIZATION
资助项目National Natural Science Foundation of China[21676001] ; National Key Research and Development program of China-Intergovernmental International Scientific and Technological Innovation Cooperation[2017YFE0105500]
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000533526800019
出版者ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD
资助机构National Natural Science Foundation of China ; National Key Research and Development program of China-Intergovernmental International Scientific and Technological Innovation Cooperation
源URL[http://ir.giec.ac.cn/handle/344007/27125]  
专题中国科学院广州能源研究所
通讯作者Cao, Yan
作者单位1.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China
2.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
4.Anhui Univ, Coll Chem & Chem Engn, Hefei 230601, Peoples R China
推荐引用方式
GB/T 7714
Li, Qiqi,Zhong, Huiqiong,Cao, Yan. Effects of the joint application of phosphate rock, ferric nitrate and plant ash on the immobility of As, Pb and Cd in soils[J]. JOURNAL OF ENVIRONMENTAL MANAGEMENT,2020,265:7.
APA Li, Qiqi,Zhong, Huiqiong,&Cao, Yan.(2020).Effects of the joint application of phosphate rock, ferric nitrate and plant ash on the immobility of As, Pb and Cd in soils.JOURNAL OF ENVIRONMENTAL MANAGEMENT,265,7.
MLA Li, Qiqi,et al."Effects of the joint application of phosphate rock, ferric nitrate and plant ash on the immobility of As, Pb and Cd in soils".JOURNAL OF ENVIRONMENTAL MANAGEMENT 265(2020):7.

入库方式: OAI收割

来源:广州能源研究所

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