A skeletal n-butane mechanism with integrated simplification method
文献类型：期刊论文
| 作者 | Li, Fan4,5; Yang, Haolin2,3,4 ; Jiang, Liqiao2,3,4; Huo, Jiepeng1,2,3,4; Wang, Xiaohan2,3,4; Zhao, Daiqing2,3,4
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| 刊名 | JOURNAL OF THE ENERGY INSTITUTE
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| 出版日期 | 2020-08-01 |
| 卷号 | 93期号:4页码:1559-1570 |
| 关键词 | n-Butane fuel Skeletal mechanism Directed relation graph method Reaction path analysis Sensitivity analysis |
| ISSN号 | 1743-9671 |
| DOI | 10.1016/j.joei.2020.01.018 |
| 通讯作者 | Yang, Haolin(yanghl@ms.giec.ac.cn) ; Zhao, Daiqing(zhaodq@ms.giec.ac.cn) |
| 英文摘要 | A new skeletal mechanism of n-butane is developed for describing its ignition and combustion characteristics applicable over a wide range of conditions: initial temperature 690-1430 K, pressure 1-30 atm, and equivalence ratio 0.5-2.0. Starting with a detailed chemical reaction kinetic model of 230 species and 1328 reactions (Healy et al., Combust. Flame, 2010), the directed relation graph method is applied as the first step to derive a semi-detailed mechanism with 134 species. Then, the reaction path analysis in conjunction with temperature sensitivity analysis is used to remove the redundant species and reaction paths simultaneously under the condition of low-temperature and moderate-to-high temperatures, respectively. Finally, a skeletal n-butane mechanism consisting of 86 species and 373 reactions can be obtained. Mechanism validation indicates that the new developed skeletal mechanism is in good agreement with the detailed mechanism in predicting the global ignition and combustion characteristics. The new skeletal mechanism is further validated using extensive available literature data including rapid pressure machine ignition delay time, shock-tube ignition delay time, laminar flame speed, and jet-stirred reaction oxidation, covering a large range of temperatures, pressures, and equivalence ratios. The comparison results demonstrate that a satisfactory agreement between predictions and experimental measurements is achieved. (C) 2020 Energy Institute. Published by Elsevier Ltd. All rights reserved. |
| WOS关键词 | LAMINAR FLAME SPEEDS ; IGNITION DELAY TIMES ; BURNING VELOCITY ; SHOCK-TUBE ; HYDROGEN ADDITION ; COMBUSTION ; TEMPERATURE ; HYDROCARBON ; OXIDATION ; PRESSURE |
| 资助项目 | National Natural Science Foundation of China[51006109] ; National Natural Science Foundation of China[51336010] ; National Basic Research Program of China (973 program)[2014CB239601] |
| WOS研究方向 | Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:000539488400031 |
| 出版者 | ELSEVIER SCI LTD |
| 资助机构 | National Natural Science Foundation of China ; National Basic Research Program of China (973 program) |
| 源URL | [http://ir.giec.ac.cn/handle/344007/27238]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Yang, Haolin; Zhao, Daiqing |
| 作者单位 | 1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 2.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 3.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 4.Chinese Acad Sci, Guangzhou Inst Energy Convers, 2 Nengyuan Rd, Guangzhou 510640, Peoples R China 5.Nanjing Univ Aeronaut & Astronaut, Coll Energy & Power Engn, Nanjing 210016, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Fan,Yang, Haolin,Jiang, Liqiao,et al. A skeletal n-butane mechanism with integrated simplification method[J]. JOURNAL OF THE ENERGY INSTITUTE,2020,93(4):1559-1570. |
| APA | Li, Fan,Yang, Haolin,Jiang, Liqiao,Huo, Jiepeng,Wang, Xiaohan,&Zhao, Daiqing.(2020).A skeletal n-butane mechanism with integrated simplification method.JOURNAL OF THE ENERGY INSTITUTE,93(4),1559-1570. |
| MLA | Li, Fan,et al."A skeletal n-butane mechanism with integrated simplification method".JOURNAL OF THE ENERGY INSTITUTE 93.4(2020):1559-1570. |
入库方式： OAI收割
来源：广州能源研究所
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