Flower-shaped nanoscale Na2Mg(CO3)(2): a promising adsorbent for fluoride removal from drinking water
文献类型:期刊论文
作者 | Sun, Bai1,2; Xu, Fangwen2; Liu, Fei2![]() |
刊名 | DESALINATION AND WATER TREATMENT
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出版日期 | 2020-10-01 |
卷号 | 202 |
关键词 | Na2Mg(CO3)(2) Adsorption Defluoridation |
ISSN号 | 1944-3994 |
DOI | 10.5004/dwt.2020.26178 |
通讯作者 | Sun, Bai(bsun@mail.ustc.edu.cn) ; Cai, Xinli(ahcxl@163.com) |
英文摘要 | In this paper, flower-shaped Na2Mg(CO3)(2) nanoparticles were synthesized by a simple hydrothermal method for defluoridation in water. The effects of the initial concentration of fluoride, pH value, and coexisting ions on the removal of fluoride were investigated. Na2Mg(CO3)(2) nanoparticles were characterized by using scanning electron microscopy, X-ray diffraction, Fourier transform infrared spectroscopy, and energy disperse analysis of X-rays. The experimental results show that the adsorption isotherm is consistent with the Freundlich model at pH = 7 and 35 degrees C. When the initial concentration is 200 mg/L, the maximum adsorption capacity calculated by the Langmuir model is up to 113.64 mg/g. The adsorption kinetics is consistent with the pseudo-second-order model, and the adsorption equilibrium can be achieved within 100 min. There is little effect on Na2Mg(CO3)(2) nanoparticles in the wide range of pH values (3-10). The fluoride removal rate reaches up to 92.26% at pH = 7 for the initial fluoride concentration of 5 mg/L, along with the adsorbent dose of 1 g/L. Except for PO43-, SO42-, and HCO3-, other anions don't affect the fluoride adsorption. The experiment results also demonstrate that the prepared adsorbents can be reused for at least six times. Finally, the mechanism for fluoride adsorption by Na2Mg(CO3)(2) nanoparticles is discussed. |
WOS关键词 | AQUEOUS-SOLUTION ; MONTMORILLONITE NANOPARTICLES ; ADSORPTION PERFORMANCE ; LOW-COST ; KINETICS ; EQUILIBRIUM ; COAGULATION ; TEMPERATURE ; MORPHOLOGY ; ISOTHERMS |
资助项目 | Project of National Key Research and Development Program[2019YFC0408503] ; Natural Science Major Research Projects of Anhui Education Department[KJ2017ZD40] ; National Natural Science Foundation of China[61873003] ; National Natural Science Foundation of China[21677001] ; Science and Technology Major projects of Anhui Province[18030801106] ; Science and Technology Major projects of Anhui Province[16030801118] ; Key Research and Development Plan of Anhui Province[201904a07020070] ; Scientific Research Start-up Foundation for Introduction of Talent, Anhui Jianzhu University[2016QD113] |
WOS研究方向 | Engineering ; Water Resources |
语种 | 英语 |
WOS记录号 | WOS:000583308100020 |
出版者 | DESALINATION PUBL |
资助机构 | Project of National Key Research and Development Program ; Natural Science Major Research Projects of Anhui Education Department ; National Natural Science Foundation of China ; Science and Technology Major projects of Anhui Province ; Key Research and Development Plan of Anhui Province ; Scientific Research Start-up Foundation for Introduction of Talent, Anhui Jianzhu University |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/105274] ![]() |
专题 | 中国科学院合肥物质科学研究院 |
通讯作者 | Sun, Bai; Cai, Xinli |
作者单位 | 1.Chinese Acad Sci, Hefei Inst Phys Sci, Nanomat & Environm Detect Lab, Hefei 230031, Peoples R China 2.Anhui Jianzhu Univ, Coll Environm & Energy Engn, Key Lab Water Pollut Control & Wastewater Resourc, Hefei 230601, Peoples R China 3.Anhui Normal Univ, Coll Chem & Mat Sci, Key Lab Funct Mol Solids, Minist Educ, Wuhu 241002, Peoples R China |
推荐引用方式 GB/T 7714 | Sun, Bai,Xu, Fangwen,Liu, Fei,et al. Flower-shaped nanoscale Na2Mg(CO3)(2): a promising adsorbent for fluoride removal from drinking water[J]. DESALINATION AND WATER TREATMENT,2020,202. |
APA | Sun, Bai.,Xu, Fangwen.,Liu, Fei.,Cheng, Yunming.,Zhang, Jie.,...&Cai, Xinli.(2020).Flower-shaped nanoscale Na2Mg(CO3)(2): a promising adsorbent for fluoride removal from drinking water.DESALINATION AND WATER TREATMENT,202. |
MLA | Sun, Bai,et al."Flower-shaped nanoscale Na2Mg(CO3)(2): a promising adsorbent for fluoride removal from drinking water".DESALINATION AND WATER TREATMENT 202(2020). |
入库方式: OAI收割
来源:合肥物质科学研究院
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