Improved photocatalytic activity of porous ZnO nanosheets by thermal deposition graphene-like g-C3N4 for CO2 reduction with H2O vapor
文献类型：期刊论文
| 作者 | Guo, Qiang; Fu, Liming; Yan, Tao; Tian, Wen; Ma, Danfeng; Li, Jiaming; Jiang, Yanan; Wang, Xitao |
| 刊名 | APPLIED SURFACE SCIENCE
 |
| 出版日期 | 2020 |
| 卷号 | 509 |
| 关键词 | CARBON NITRIDE NANOSHEETS VISIBLE-LIGHT FACILE SYNTHESIS ZNO/G-C3N4 COMPOSITES CHARGE SEPARATION DECORATED G-C3N4 EFFICIENT DEGRADATION FABRICATION TIO2 |
| DOI | 10.1016/j.apsusc.2019.144773 |
| 英文摘要 | Porous ZnO nanosheets (PNS-ZnO) were prepared by calcining ZnS(en)(0.5) (en = ethylenediamine) nanosheets in air, and g-C3N4 (g-CN) nanofilms were coated on the surface of PNS-ZnO by thermal deposition using bulk g-C3N4 as precursor. Experimental results showed that the graphene-like g-C3N4 could be deposited on the surface of ZnO to form nanocomposites with core/shell structure. After the loading of g-CN, the light absorption and chemical adsorption of CO2 over PNS-ZnO were improved obviously and the recombination of photogenerated electron and hole was greatly depressed due to the formation of heterojunction between PNS-ZnO and g-CN. All PNS-ZnO@g-CN nanocomposites exhibited much higher photocatalytic activity for CO2 reduction with H2O vapor when compared to pure PNS-ZnO and bulk g-CN. The loading amount of g-CN had significant influence on the light absorption and photocatalytic activity, and PNS-ZnO@g-CN-0.4 exhibited the best photocatalytic performance, for which H-2, CH4 and CO production rates of 22.7, 30.5 and 16.8 mu mol/g(cat)/h can be obtained, respectively. |
| 学科主题 | Chemistry ; Materials Science ; Physics |
| 源URL | [http://ir.nimte.ac.cn/handle/174433/19794]  |
| 专题 | 2020专题 2020专题_期刊论文 |
| 作者单位 | Wang, XT (corresponding author), Tianjin Univ, Coll Chem Engn & Technol, Collaborat Innovat Ctr Chem Sci & Engn, Tianjin Key Lab Appl Catalysis Sci & Technol, Tianjin 300072, Peoples R China. |
| 推荐引用方式 GB/T 7714 | Guo, Qiang,Fu, Liming,Yan, Tao,et al. Improved photocatalytic activity of porous ZnO nanosheets by thermal deposition graphene-like g-C3N4 for CO2 reduction with H2O vapor[J]. APPLIED SURFACE SCIENCE,2020,509. |
| APA | Guo, Qiang.,Fu, Liming.,Yan, Tao.,Tian, Wen.,Ma, Danfeng.,...&Wang, Xitao.(2020).Improved photocatalytic activity of porous ZnO nanosheets by thermal deposition graphene-like g-C3N4 for CO2 reduction with H2O vapor.APPLIED SURFACE SCIENCE,509. |
| MLA | Guo, Qiang,et al."Improved photocatalytic activity of porous ZnO nanosheets by thermal deposition graphene-like g-C3N4 for CO2 reduction with H2O vapor".APPLIED SURFACE SCIENCE 509(2020). |
入库方式： OAI收割
来源：宁波材料技术与工程研究所
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