Building hierarchical zeolite structure by post-synthesis treatment to promote the conversion of furanic molecules into biofuels
文献类型:期刊论文
作者 | Hu, Danxin; Hu Hualei; Jin, Haitao; Zhang, Pilan; Hu, Yunhan; Ying, Suhua; Li, Xianming; Yang, Yong; Zhang, Jian; Wang, Lei |
刊名 | APPLIED CATALYSIS A-GENERAL |
出版日期 | 2020 |
卷号 | 590 |
关键词 | CATALYTIC TRANSFORMATION EFFICIENT PRODUCTION BENZENE ALKYLATION ZSM-5 ZEOLITES ETHERIFICATION DESILICATION LEWIS MFI PERFORMANCE PLATFORM |
DOI | 10.1016/j.apcata.2019.117338 |
英文摘要 | The highly selective conversion of furanic molecules to biofuels was achieved on the hierarchical catalysts, which were prepared through modifying the commercially microporous zeolites with sequential alkali and acid post-synthesis treatments. The characterization results indicated that the post-synthesis treatment could successfully introduce the mesopores into the microporous ZSM-5 sample as well as adjust its acidity. The yield of three furanic ethers i.e. 2,5-bis(ethoxymethyl)furan, 5-ethoxymethyl-furfural, and ethyl furfuryl ether on the AT(0.50)-OT catalyst were 94.7%, 90.6%, and 58.2%, respectively. The excellent performance could be attributed to the synergic effect of mass transfer efficiency and surface acidity. This work provides a simple route to prepare high-performance catalysts for the production of biofuels from biochemical. |
学科主题 | Chemistry ; Environmental Sciences & Ecology |
源URL | [http://ir.nimte.ac.cn/handle/174433/20136] |
专题 | 2020专题 2020专题_期刊论文 |
作者单位 | 1.Hu, HL 2.Zhang, J 3.Wang, L (corresponding author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, 1219 Zhongguan West Rd, Ningbo 315201, Peoples R China. |
推荐引用方式 GB/T 7714 | Hu, Danxin,Hu Hualei,Jin, Haitao,et al. Building hierarchical zeolite structure by post-synthesis treatment to promote the conversion of furanic molecules into biofuels[J]. APPLIED CATALYSIS A-GENERAL,2020,590. |
APA | Hu, Danxin.,Hu Hualei.,Jin, Haitao.,Zhang, Pilan.,Hu, Yunhan.,...&Wang, Lei.(2020).Building hierarchical zeolite structure by post-synthesis treatment to promote the conversion of furanic molecules into biofuels.APPLIED CATALYSIS A-GENERAL,590. |
MLA | Hu, Danxin,et al."Building hierarchical zeolite structure by post-synthesis treatment to promote the conversion of furanic molecules into biofuels".APPLIED CATALYSIS A-GENERAL 590(2020). |
入库方式: OAI收割
来源:宁波材料技术与工程研究所
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