pH-Responsive Superwettability Surface: The Study of Oil Dewetting Ability from Air to Water on a Rough Surface and Selective Oil-Water Separation
文献类型：期刊论文
| 作者 | Tang, Lei; Zeng, Zhixiang; Wang, Gang; Shen, Luli; Zhu, Lijing; Zhang, Yingxin; Xue, Qunji |
| 刊名 | ADVANCED MATERIALS INTERFACES
 |
| 出版日期 | 2020 |
| 关键词 | SWITCHABLE WETTABILITY SUPERHYDROPHOBIC SURFACE OIL/WATER SEPARATION COATINGS BEHAVIOR FABRICATION MONOLAYERS MEMBRANES DESIGN DRIVEN |
| DOI | 10.1002/admi.202001147 |
| 英文摘要 | Responsive smart surfaces with controllable wettability have a high potential application in self-cleaning and oil-water separation. In this work, a new and simple method is reported to fabricate a pH-responsive superwettability surface. And the self-cleaning performance from air to water after oil contamination in a dry state is studied. Wettability regulation can be achieved by controlling the ratio of carboxyl groups with protonation or deprotonation state in acid or basic solutions. Rough surface with 40% carboxyl content (X-COOH = 0.4) shows the most significant response. The surface is superoleophilic underwater after wetted in acid solution in advance but superoleophobic underwater with basic solution pre-wetted. Oil desorption can be achieved under the superoleophobic state to realize the self-cleaning effect on a rough surface with a complex process. The dynamic self-cleaning process can be achieved by changing the pH value of the solution. This pH-responsive surface also has a good self-cleaning effect for the common water and solid pollutants. Moreover, a smart separation system with the ability to realize selective oil-water separation under two different states is prepared. It is believed that the results reported could broaden the understanding of self-cleaning systems and open a new perspective in controlling wettability. |
| 学科主题 | Chemistry ; Materials Science |
| 源URL | [http://ir.nimte.ac.cn/handle/174433/20476]  |
| 专题 | 2020专题 2020专题_期刊论文 |
| 作者单位 | 1.Zeng, ZX 2.Wang, G (corresponding author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Zhejiang Key Lab Marine Mat & Protect Technol, Key Lab Marine Mat & Related Technol, Ningbo 315201, Peoples R China. |
| 推荐引用方式 GB/T 7714 | Tang, Lei,Zeng, Zhixiang,Wang, Gang,et al. pH-Responsive Superwettability Surface: The Study of Oil Dewetting Ability from Air to Water on a Rough Surface and Selective Oil-Water Separation[J]. ADVANCED MATERIALS INTERFACES,2020. |
| APA | Tang, Lei.,Zeng, Zhixiang.,Wang, Gang.,Shen, Luli.,Zhu, Lijing.,...&Xue, Qunji.(2020).pH-Responsive Superwettability Surface: The Study of Oil Dewetting Ability from Air to Water on a Rough Surface and Selective Oil-Water Separation.ADVANCED MATERIALS INTERFACES. |
| MLA | Tang, Lei,et al."pH-Responsive Superwettability Surface: The Study of Oil Dewetting Ability from Air to Water on a Rough Surface and Selective Oil-Water Separation".ADVANCED MATERIALS INTERFACES (2020). |
入库方式： OAI收割
来源：宁波材料技术与工程研究所
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