Nature-derived, structure and function integrated ultra-thick carbon electrode for high-performance supercapacitors
文献类型：期刊论文
| 作者 | Liu, K; Mo, RW; Dong, WJ; Zhao, W; Huang, FQ |
| 刊名 | JOURNAL OF MATERIALS CHEMISTRY A
 |
| 出版日期 | 2020-10-14 |
| 期号 | 38页码:20072 |
| ISSN号 | 2050-7488 |
| DOI | 10.1039/d0ta06108e |
| 文献子类 | Article |
| 英文摘要 | The design of ultra-thick electrodes for energy storage has the potential to significantly increase the device-level energy density, but still faces major challenges of low mechanical stability and slow charge kinetics. Herein, inspired by the hierarchical structure and lignocellulosic component of natural wood, we developed a structure-engineered and heteroatom-functionalized carbon slice, leveraging selective delignification and hydrogen bonding chemistryviapyrolyzing the as-modified porous cellulose following a one-pot chemical treatment of natural wood. When explored as a binder-free, conductive-additive-free, and self-supporting ultra-thick electrode, the electrode shows outstanding areal and gravimetric capacitance of 2980 mF cm(-2)and 183 F g(-1), respectively. Moreover, the as-assembled quasi-solid-state symmetric supercapacitor yields high areal, gravimetric and volumetric energy densities of 0.3 mW h cm(-2), 9.68 W h kg(-1), and 0.63 mW h cm(-3), respectively. The excellent electrochemical properties can be attributed to the synergistic effect of dual heteroatom-containing groups and well-aligned channels. This work provides a new design strategy for ultra-thick electrodes toward next-generation, high-performance energy storage devices. |
| WOS关键词 | GRAPHENE AEROGELS ; WOOD ; NITROGEN |
| WOS研究方向 | Chemistry ; Energy & Fuels ; Materials Science |
| 语种 | 英语 |
| 出版者 | ROYAL SOC CHEMISTRY |
| 源URL | [http://ir.sic.ac.cn/handle/331005/27692]  |
| 专题 | 中国科学院上海硅酸盐研究所 |
| 推荐引用方式 GB/T 7714 | Liu, K,Mo, RW,Dong, WJ,et al. Nature-derived, structure and function integrated ultra-thick carbon electrode for high-performance supercapacitors[J]. JOURNAL OF MATERIALS CHEMISTRY A,2020(38):20072. |
| APA | Liu, K,Mo, RW,Dong, WJ,Zhao, W,&Huang, FQ.(2020).Nature-derived, structure and function integrated ultra-thick carbon electrode for high-performance supercapacitors.JOURNAL OF MATERIALS CHEMISTRY A(38),20072. |
| MLA | Liu, K,et al."Nature-derived, structure and function integrated ultra-thick carbon electrode for high-performance supercapacitors".JOURNAL OF MATERIALS CHEMISTRY A .38(2020):20072. |
入库方式： OAI收割
来源：上海硅酸盐研究所
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