Accumulation, temporal variation, source apportionment and risk assessment of heavy metals in agricultural soils from the middle reaches of Fenhe River basin, North China
文献类型:期刊论文
作者 | Liu, Minxia3; Han, Zhiqiang1; Yang, Yuyi2,4 |
刊名 | RSC ADVANCES
![]() |
出版日期 | 2019-07-16 |
卷号 | 9期号:38页码:21893-21902 |
ISSN号 | 2046-2069 |
DOI | 10.1039/c9ra03479j |
英文摘要 | The Fenhe River basin is the main agricultural and industrial developed area in Shanxi province, China. In recent years, agricultural non-point source pollution in the Fenhe River basin intensified, threatening soil quality and safety in the area. Accumulation of eight heavy metals (HMs) including chromium (Cr), nickel (Ni), copper (Cu), zinc (Zn), arsenic (As), cadmium (Cd), lead (Pb) and mercury (Hg) has been detected in soil samples from 50 agricultural sites (0-20 cm) from the middle reaches of the Fenhe River basin. The ecological and human health risk and potential sources of the eight HMs were investigated. In addition, the human health and ecological risks imposed by the possible sources of the eight HMs were quantitatively apportioned. The enrichment factor (EF) values of Cr, Ni, Cu, Pb and Zn were lower than 2, indicating minimal enrichment, while values for As, Cd and Hg were between 2 and 5, exhibiting moderate enrichment. Temporal variation analysis suggested that most HMs in the study area exhibited low concentrations after 2015, except As. The potential ecological risk index was 174.09, indicating low ecological risk. The total hazard index and cancer risk values were 0.395 and 5.35 x 10(-4) for adults and 2.75 and 3.63 x 10(-4) for children, indicating the accepted standard levels were exceeded for non-carcinogenic risk for children and carcinogenic risks for both adults and children. Four potential sources were identified: (1) natural sources, (2) farming activities, (3) coal combustion, and (4) exhaust emissions. Natural sources represented the largest contributor to ecological risk, accounting for 57.42% of the total. Coal combustion was the major contributor to human health risks, accounting for 43.27% and 43.73% of the total non-carcinogenic risk and carcinogenic risk for adults, respectively, and 42.72% and 43.88% for children, respectively. |
资助项目 | Applied Basic Research of Shanxi province of China[201801D221042] ; Science and Technology Innovation Fund of Shanxi Agricultural University[2016YJ13] ; National Natural Science Foundation of China[31500523] |
WOS研究方向 | Chemistry |
语种 | 英语 |
WOS记录号 | WOS:000476751400034 |
出版者 | ROYAL SOC CHEMISTRY |
源URL | [http://202.127.146.157/handle/2RYDP1HH/8354] ![]() |
专题 | 中国科学院武汉植物园 |
通讯作者 | Yang, Yuyi |
作者单位 | 1.Period Press Shanxi Agr Univ, Taigu 030801, Peoples R China 2.Chinese Acad Sci, Key Lab Aquat Bot & Watershed Ecol, Wuhan Bot Garden, Wuhan 430074, Hubei, Peoples R China 3.Shanxi Agr Univ, Coll Forestry, Taigu 030801, Peoples R China 4.Univ Dundee, Sch Life Sci, Dundee DD1 5EH, Scotland |
推荐引用方式 GB/T 7714 | Liu, Minxia,Han, Zhiqiang,Yang, Yuyi. Accumulation, temporal variation, source apportionment and risk assessment of heavy metals in agricultural soils from the middle reaches of Fenhe River basin, North China[J]. RSC ADVANCES,2019,9(38):21893-21902. |
APA | Liu, Minxia,Han, Zhiqiang,&Yang, Yuyi.(2019).Accumulation, temporal variation, source apportionment and risk assessment of heavy metals in agricultural soils from the middle reaches of Fenhe River basin, North China.RSC ADVANCES,9(38),21893-21902. |
MLA | Liu, Minxia,et al."Accumulation, temporal variation, source apportionment and risk assessment of heavy metals in agricultural soils from the middle reaches of Fenhe River basin, North China".RSC ADVANCES 9.38(2019):21893-21902. |
入库方式: OAI收割
来源:武汉植物园
浏览0
下载0
收藏0
其他版本
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。