Converting Co2+-impregnated g-C3N4 into N-doped CNTs-confined Co nanoparticles for efficient hydrogenation rearrangement reactions of furanic aldehydes
文献类型：期刊论文
| 作者 | Wang, Dongdong1,2; Al-Mamun, Mohammad3; Gong, Wanbing1; Lv, Yang1,2; Chen, Chun1 ; Lin, Yue4; Wang, Guozhong1; Zhang, Haimin1; Zhao, Huijun1,3
|
| 刊名 | NANO RESEARCH
 |
| 出版日期 | 2021-01-05 |
| 关键词 | g-C3N4 Co nanoparticles carbon nanotubes hydrogenation rearrangement furanic aldehydes |
| ISSN号 | 1998-0124 |
| DOI | 10.1007/s12274-021-3298-y |
| 通讯作者 | Gong, Wanbing(wbgong@issp.ac.cn) ; Zhao, Huijun(h.zhao@griffith.edu.au) |
| 英文摘要 | The cyclopentanone and derivatives are a class of crucial fine chemicals for various industries and currently produced by conventional petrochemical synthetic routes. Here, we demonstrated a new synthetic approach to directly fabricate N-doped carbon nanotube (N-CNTs) networks with confined Co nanoparticles from Co2+-impregnated bulk g-C3N4 as high performance hydrogenation rearrangement (HR) catalyst to efficiently convert a wide spectrum of biomass-derived furanic aldehydes to the corresponding cyclopentanones in water under a record-low H-2 pressure of 0.5 MPa and mild temperature. We unveiled a Co-catalysed bulk g-C3N4 decomposition/carbonisation CNTs formation mechanism. A new HR pathway was also unveiled. |
| WOS关键词 | SELECTIVE HYDROGENATION ; CARBON NANOTUBES ; CYCLOPENTANONE ; CATALYSTS ; CONVERSION ; PERFORMANCE ; HYBRIDS ; BOND |
| 资助项目 | National Natural Science Foundation of China[51871209] ; National Natural Science Foundation of China[51902311] ; Postdoctoral Science Foundation of China[2019M652223] |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| 语种 | 英语 |
| WOS记录号 | WOS:000605145200005 |
| 出版者 | TSINGHUA UNIV PRESS |
| 资助机构 | National Natural Science Foundation of China ; Postdoctoral Science Foundation of China |
| 源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/119962]  |
| 专题 | 中国科学院合肥物质科学研究院 |
| 通讯作者 | Gong, Wanbing; Zhao, Huijun |
| 作者单位 | 1.Chinese Acad Sci, Anhui Key Lab Nanomat & Nanotechnol, CAS Ctr Excellence Nanosci,Key Lab Mat Phys, Inst Solid State Phys,Ctr Environm & Energy Nanom, Hefei 230031, Peoples R China 2.Univ Sci & Technol China, Hefei 230026, Peoples R China 3.Griffith Univ, Ctr Clean Environm & Energy, Gold Coast Campus, Brisbane, Qld 4222, Australia 4.Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Dongdong,Al-Mamun, Mohammad,Gong, Wanbing,et al. Converting Co2+-impregnated g-C3N4 into N-doped CNTs-confined Co nanoparticles for efficient hydrogenation rearrangement reactions of furanic aldehydes[J]. NANO RESEARCH,2021. |
| APA | Wang, Dongdong.,Al-Mamun, Mohammad.,Gong, Wanbing.,Lv, Yang.,Chen, Chun.,...&Zhao, Huijun.(2021).Converting Co2+-impregnated g-C3N4 into N-doped CNTs-confined Co nanoparticles for efficient hydrogenation rearrangement reactions of furanic aldehydes.NANO RESEARCH. |
| MLA | Wang, Dongdong,et al."Converting Co2+-impregnated g-C3N4 into N-doped CNTs-confined Co nanoparticles for efficient hydrogenation rearrangement reactions of furanic aldehydes".NANO RESEARCH (2021). |
入库方式： OAI收割
来源：合肥物质科学研究院
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。